Influence of Outer Zirconia Transient Cracking and Spalling on Thermomechanical Behaviour of High Burnup Fuel Rod Submitted to RIA

The French “Institut de Radioprotection et de Sîreté Nucléaire” (IRSN) conducted the REP-Na tests in the CABRI reactor within the framework of its research program on nuclear fuel safety. These tests were devoted to the study of Reactivity Initiated Accident (RIA). Cracking and spalling of the fuel rod zirconia layer were observed after several REP-Na tests. Sometimes, an ovalisation of the rod after the RIA transient is also observed. Metallographic examinations showed that the outer and inner zirconia cracks are regularly spaced and that the crack density is linked to the clad plastic hoop strain. An analogy with brittle thin film layering a ductile substrate submitted to a tensile test is made and helps to understand this specific phenomenon. A numerical simulation evaluates the thermo-mechanical behaviour of the rod, including the zirconia influence during a RIA. This work make it possible both to identify the spalling process and to clarify the preferential spalling along the less corroded azimuths for several tests. The influence of the transient spalling on the boiling crisis occurrence in PWR condition is finally addressed.     

Simple Empirical Expression to Evaluate Effective Dose Equivalent for External Photon Irradiation

In the CABRI-FAST and CABRI-RAFT programs within a collaboration with the Institut de Radioprotection et de Sûreté Nucléaire (IRSN) and Forschungszentrum Karlsruhe (FZK), five pulse-type transient overpower tests were performed in order to study fuel pin behavior and failure condition in the Unprotected Loss-of-Flow (ULOF) accident. In these tests, two types of low-smear-density fuels irradiated in the French Phénix reactor at different burn-up levels were used so that an experimental database extension from the former CABRI-1 and CABRI-2 programs can be obtained. Pin failure took place in three of these tests giving information on the failure threshold. In two tests, no pin failure took place and useful information related to the transient fuel behavior up to failure and failure mechanism was obtained. These test results were interpreted through detailed analysis of experimental data and PAPAS-2S code calculations. In these calculations, pretransient fuel characteristics obtained from the sibling fuels were reflected, such that the uncertainty of the boundary condition can be minimized. Through the comparison among these tests and formerly existing CABRI tests, generalized understanding on the transient fuel behavior was obtained. It was concluded that the low-smear-density fuel mitigates cavity pressurization, thereby enhancing the margin-to-failure. It was also understood that this failure-thresholdenhancing capability is dependent on the type of transient.     

Evaluation of safety of French type B package designs in severe accident environments other than regulatory

Abstract

Packages used to transport radioactive materials in France must be designed to meet the safety performance requirements when subject to the test conditions set forth in the International Atomic Energy Agency (IAEA) Regulations. During actual use, the packages may be subject to quite different accident conditions. The Institut de Radioprotection et de Sûreté Nucléaire (IRSN) has evaluated the behaviour of typical packages designed to transport spent fuel, high activity waste, fresh mixed oxide (MOX) fuel and plutonium oxide powder under realistic conditions of mechanical impact and fire. The studied designs remain safe after impact onto targets present in the real environment of transport. The energy absorption by the package ancillary equipment (transport frame) compensates for the kinetic energy increase by comparison to the energy expended during the regulatory tests. New software was developed to correctly simulate the thermal behaviour of the neutron shielding materials. The studied package designs exhibit large margins of safety concerning resistance to fire. The results obtained have been used to develop tools in support of the appraisal of emergency situations.     

Estimation of the Grain Boundary Gas Inventory in MIMAS/AUC MOX Fuel and Consistency with REP-Na Test Results

In the frame of its research activities on fuel safety, the French “Institut de Radioprotection et de Sûreté Nucléaire” performed the REP-Na program in the CABRI reactor devoted to the study of Reactivity Initiated Accidents. Focused on high burn-up UO2 and MOX fuel behaviour, twelve tests (8 UO2 and 4 MOX) were realized from 1993 to 2000. In all these tests, the influence of grain boundary gas was evidenced and it appeared necessary to perform some estimation of its inventory in irradiated fuel. Such evaluations are presented for the MOX MIMAS/AUC fuel, based on two different approaches: “experimental” and “theoretical.” The fission gas amount located at the grain boundaries increases with burn-up in correlation with the production, but also with the initial Pu enrichment, as soon as the agglomerates have reached the full restructuring threshold for the High Burn-up Structure. The consistency with the REP-Na test results is checked, showing that a significant cladding deformation is needed, clearly higher than for UO2 fuel in order to release all the grain boundary gas in RIA. Furthermore, to the fission gas effect, adds the helium's occluded in the irradiated fuel whose amount increases with burn-up, Pu enrichment and ²⁴¹Pu and ²⁴¹Am initial content.     

Mechanical characteristics of fuel rod claddings in transport conditions

Abstract

A synthesis on the mechanical characteristics of unirradiated and irradiated fuel rod claddings was performed by the French Institut de Radioprotection et de Sûreté Nucléaire (IRSN) in order to have reference data for the assessment of the safety demonstrations in normal and accident conditions of transport required by the procedure of package licensing. Indeed, the transport conditions correspond to a range of cladding temperatures (200–550°C) which is only partly covered by the data acquired within the framework of the safety demonstration relative to the reactor normal operating conditions, especially beyond 400°C. This work concerned Zircaloy-4 cladding material (Zry-4) and M5^TM. Data about mechanical properties (elastic and ductile properties, creep behaviour), oxidation (in reactor and under air during transport), hydrides and fracture toughness have been collected and synthesised. The laws presented in the document can be used to obtain orders of magnitude of oxide layer thickness, hydrogen content and creep deformation rate. The following phenomena which could influence the mechanical behaviour of the cladding were more particularly studied: oxidation which could become very important during transport in case of cladding temperatures of ～500°C; creep for which only a few data ～500°C are available and which depends in particular on the internal pressure of the rods, the cladding oxidation and the presence of the hydrides; and recrystallisation of Zry-4 at ～500°C, which could have consequences on the mechanical properties of the cladding after cooling during the storage. For other topics of interest for the study of the mechanical behaviour of the cladding, such as the fracture toughness for example, it was identified that the data available is scarce.     

Behaviour of package for transport of spent fuel assemblies exposed to beyond regulation fires

Abstract

Institut de Radioprotection et de Sûreté Nucléaire (IRSN) performed a study relative to the thermal behaviour of a new TN International package design for transport of spent fuel assemblies called TN®112. The aim of this study is to evaluate the behaviour of the package exposed to fires, with durations and temperatures different from those required in the IAEA regulation TS-R-1 (respectively 30 min and 800°C). Its main objective is to provide quantitative data available for safety assessment in emergency situations involving fires. Moreover it can also be used for a cross comparison with the analysis of the thermal behaviour of the package during the IAEA regulatory fire test presented by the applicant in the package design safety analysis report. This study is based on numerical calculations performed with the code THERMX-PROTEE. The three-dimensional model used represents a quarter of the upper half of the package, where the closure system is located. The thermal behaviour of the neutron-shielding resin located in the cavity plug, the trunnions and the packaging body was modelled to allow simulation of endothermic reactions of vaporisation. During the heating phase of the fire test, the water vapour produced in the heated resin components is transferred and condensed in the nearby colder elements; the associated thermal transfers can rapidly increase the temperature of the colder elements. The part of the vapour which cannot be condensed when most of the nearby resin elements reach a temperature above 100°C is evacuated through the holes that are distributed throughout the external envelope of the packaging and closed by fusible plugs under normal conditions. A specific calculation module has been developed to take into account the corresponding energy transfers. This module was qualified by comparison with the results of experimental fire tests. The calculations performed in the framework of this study cover fire temperatures between 400 and 1000°C. One of the results of those calculations is the time necessary to reach the maximum allowable temperature of the elastomer gaskets.     

External loads applied to packages during routine transport

Abstract

Packages carrying radioactive material experience a range of environmental conditions during routine transport including temperatures, pressures and shocks. Concerning the mechanical loadings, the packages are subjected to, the advisory material TS-G-1·1 indicates that, ‘due to the differences in transport infrastructures and practices, the recommended acceleration factors, which represent the package inertial effects, could differ from one country to another and that the package designer should confirm the acceptability of those factors’. In this context, the Institut de radioprotection et de sûreté nucléaire (IRSN) performed a bibliographical study relative to accelerations measured on packages during transport. This study shows some variations with the acceleration factors mentioned in TS-G-1·1. It also highlights areas where data are missing. In these areas, further measurement campaigns should be performed. An international project under the auspices of IAEA could provide opportunities for collecting a large set of results and facilitate the needed international consultation.     

Reactor cooling systems thermal-hydraulic assessment of the ASTEC V1.3 code in support of the French IRSN PSA-2 on the 1300 MWe PWRs

The French Institut de Radioprotection et de Sûreté Nucléaire (IRSN) is performing a level 2 Probabilistic Safety Assessment (PSA-2) on the French 1300 MWe PWRs. This PSA-2 study is relying on the ASTEC integral computer code, jointly developed by IRSN and GRS (Germany). In order to assess the reliability and the quality of physical results of the ASTEC V1.3 code as well as the PWR 1300 MWe reference input deck, a wide-ranging series of comparisons with the French best-estimate thermal-hydraulic code CATHARE 2 V2.5 has been performed on 14 different severe-accident scenarios. The present paper details 4 out of the 14 studied scenarios: a 12-in. cold leg Loss of Coolant Accident (LOCA), a 2-tube Steam Generator Tube Rupture (SGTR), a 12-in. Steam Line Break (SLB) and a total Loss of Feed Water scenario (LFW). The thermal-hydraulic behavior of the primary and secondary circuits is thoroughly investigated and compared to the CATAHRE 2 V2.5 results. The ASTEC results of the core degradation phase are also presented. Overall, the thermal-hydraulic behavior given by the ASTEC V1.3 is in very good agreement with the CATHARE 2 V2.5 results.     

A preliminary assessment of beryllium dust oxidation during a wet bypass accident in a fusion reactor

A beryllium dust oxidation model has been developed at the Idaho National Laboratory (INL) by the Fusion Safety Program (FSP) for the MELCOR safety computer code. The purpose of this model is to investigate hydrogen production from beryllium dust layers on hot surfaces inside a fusion reactor vacuum vessel (VV) during in-vessel loss-of-cooling accidents (LOCAs). This beryllium dust oxidation model accounts for the diffusion of steam into a beryllium dust layer, the oxidation of the dust particles inside this layer based on the beryllium–steam oxidation equations developed at the INL, and the effective thermal conductivity of this beryllium dust layer. This paper details this oxidation model and presents the results of the application of this model to a wet bypass accident scenario in the ITER device.     

Experimental and numerical approaches of aerosol removal in spray conditions for containment application

TOSQAN is an experimental program undertaken by the Institut de Radioprotection et de Sûreté Nucléaire (IRSN) in order to perform thermal hydraulic containment studies. The TOSQAN facility is a large enclosure devoted to simulate typical accidental thermal hydraulic flow conditions in nuclear pressurized water reactor (PWR) containment. The TOSQAN facility, which is highly instrumented with non-intrusive optical diagnostics, is particularly adapted to nuclear safety code validation. The present work is devoted to study a water spray injection used as a mitigation means in order to washout aerosol fission products.     

Experimental investigation in the TOSQAN facility of heat and mass transfers in a spray for containment application

TOSQAN is an experimental program undertaken by the Institut de Radioprotection et de Sûreté Nucléaire (IRSN) in order to perform thermal hydraulic containment studies. The TOSQAN facility is a large enclosure devoted to simulate typical accidental thermal hydraulic flow conditions in nuclear-pressurized water reactor (PWR) containment. The TOSQAN facility which is highly instrumented with non-intrusive optical diagnostics is particularly adapted to nuclear safety CFD code validation. The present work is devoted to studying the interaction of a water spray injection used as a mitigation means in order to reduce the gas pressure and temperature in the containment, to produce gases mixing and washout of fission products. In order to have a better understanding of heat and mass transfers between spray droplets and the gas mixture, and to analyze mixing effects due to spray activation, we perform detailed characterization of the two-phase flow.     

PHEBUS FPT0~FPT2实验堆芯降级过程数值模拟

严重事故下，由于堆芯冷却剂丧失引起的堆芯裸露、过热和熔化过程对后期安全壳完整性、裂变产物行为等具有重要影响。法国辐射防护与核安全研究所主导的PHEBUS-FP研究项目旨在研究轻水堆严重事故下堆芯降级过程以及裂变产物行为。本文使用ATHLET-CD程序对PHEBUS-FP中的FPT0、FPT1和FPT2进行建模计算，主要分析堆芯过热，包壳氧化，堆内材料熔化、迁移及再定位过程。计算结果表明：不同蒸汽流量、不同加热功率将导致不同堆芯降级进程，在趋势上计算值与实验值吻合；模型的限制导致了部分计算值的偏差，本文讨论了包壳氧化与燃料再定位现象中的模型参数。     

ASTEC application to in-vessel corium retention

This paper summarizes the work done in the SARNET European Network of Excellence on Severe Accidents (6th Framework Programme of the European Commission) on the capability of the ASTEC code to simulate in-vessel corium retention (IVR). This code, jointly developed by the French Institut de Radioprotection et de Sûreté Nucléaire (IRSN) and the German Gesellschaft für Anlagen und Reaktorsicherheit mbH (GRS) for simulation of severe accidents, is now considered as the European reference simulation tool.First, the DIVA module of ASTEC code is briefly introduced. This module treats the core degradation and corium thermal behaviour, when relocated in the reactor lower head. Former ASTEC V1.2 version assumed a predefined stratified molten pool configuration with a metallic layer on the top of the volumetrically heated oxide pool. In order to reflect the results of the MASCA project, improved models that enable modelling of more general corium pool configurations were implemented by the CEA (France) into the DIVA module of the ASTEC V1.3 code.In parallel, the CEA was working on ASTEC modelling of the external reactor vessel cooling (ERVC). The capability of the ASTEC CESAR circuit thermal-hydraulics to simulate the ERVC was tested. The conclusions were that the CESAR module is capable of simulating this system although some numerical and physical instabilities can occur. Developments were then made on the coupling between both DIVA and CESAR modules in close collaboration with IRSN. In specific conditions, code oscillations remain and an analysis was made to reduce the numerical part of these oscillations. A comparison of CESAR results of the SULTAN experiments (CEA) showed an agreement on the pressure differences.The ASTEC V1.2 code version was applied to IVR simulation for VVER-440/V213 reactors assuming defined corium mass, composition and decay heat. The external cooling of reactor wall was simulated by applying imposed coolant temperature and heat transfer coefficient (HTC). The obtained results (pool temperatures, heat flux distribution, reactor wall ablation) were compared with available predictions of other codes. The agreement was correct, in particular on the shape and depth of ablation, as well as the maximum heat flux in case of a thick metallic layer, while ASTEC calculated a lower maximum heat flux for a thin metallic layer.     

Analysis of the reference accidental sequence for safety assessment of LLCB TBM system

Safety analysis of the reference accidental sequence has been carried out for Lead Lithium cooled Ceramic Breeder (LLCB) Test Blanket Module (TBM) system; India's prototype of DEMO blanket concept for testing in International Thermonuclear Experimental Reactor (ITER). The accidental event analyzed starts with a Postulated Initiating Event (PIE) of ex-vessel loss of first wall helium coolant due to guillotine rupture of coolant pipe with simultaneous assumed failure of plasma shutdown system. Three different variants of the sequences analyzed include simultaneous additional failures of TBM and ITER first wall, failure of TBM box resulting in to spilling of lead lithium liquid metal in to vacuum vessel and reactor trip on Loss of Coolant Accident (LOCA) signal from TBM system. The analysis address specific reactor safety concerns, such as pressurization of confinement buildings, vacuum vessel pressurization, release of activated products and tritium during these accidental events and hydrogen production from chemical reactions between lead–lithium liquid metal and beryllium with water. An in-house customized computer code is developed and through these deterministic safety analyses the prescribed safety limits are shown to be well within limits for Indian LLCB-TBM design and it also meets overall safety goal for ITER. This paper reports transient analysis results of the safety assessment.     

Analysis of an ex-vessel break in the ITER divertor cooling loop

In the present work the integrated ECART code, developed for severe accident analysis in LWRs, is applied on the analysis of a large ex-vessel break in the divertor cooling loop of the international thermonuclear experimental reactor (ITER). A comparison of the ECART results with those obtained by Studsvik Nuclear AB (S), utilizing the MELCOR code, was also performed in the general framework of the quality assurance program for the ITER accident analyses. This comparison gives a good agreement in the results, both for thermal-hydraulics and the environmental radioactive releases. Mainly these analyses, from the point of view of the ITER safety, confirm that the accidental overpressure inside the vacuum vessel and the Tokamak cooling water system (TWCS) Vault is always well below the design limits and that the radioactive releases are adequately confined below the ITER guidelines.     

International Working Group for Sabotage Concerns of Transport and Storage Casks

Abstract

The International Working Group for Sabotage Concerns of Transport and Storage Casks (IWGSTSC), gathers multiple organisations from different countries (for US party Department of Energy, Nuclear Regulatory Commission, and Sandia National Laboratories; for German party Gesellschaft für Anlagen- und Reaktorsicherheit and Fraunhofer Institut; for the French party Institut de Radioprotection et de Sûreté Nucléaire). The goal of the IWGSTSC is to continue cooperation to improve the analytic capabilities, through information sharing and collaborative research and development plus modelling, to understand the potential adverse public health effects and environmental impacts of radiological sabotage directed at or associated with the transport and storage of civilian nuclear material or other civilian radioactive materials. The Parties may also undertake collaborative research and development in other areas of the physical protection of civilian nuclear materials or other radioactive materials. Since 2000, the IWGSTSC has conducted an extensive test programme for the assessment of the aerosol source term produced in the case of spent fuel transport sabotage by a high energy density device, after having examined several scenarios. The major goal of this programme is to produce an accurate estimate of the so called spent fuel ratio in the domain of respirable, aerosol particles produced. All the reports prepared by Sandia National Laboratories have precisely emphasised the important efforts they have made from the beginning and the amount of work already accomplished. In parallel, the International Atomic Energy Agency (IAEA), assisted by technical experts from different countries, has provided a draft document promised to become guidance for the security of radioactive or nuclear materials during transport. The IAEA document contains general guidance addressed to anyone who intends to implement or improve the security of material transports, but the text is, as of today, limited to rather general recommendations. Based on all the knowledge accumulated from past experiments and also based on the work carried out in Vienna at the IAEA, the IWGSTSC members have decided to work on the development of a method for the evaluation of the vulnerability and the source term. So for doing that, joint projects for the research, development, testing and evaluation of the consequences of the malevolent actions during transport are being pursued and are described in this paper.     

Real-time measurement of hydrogen generation level during beryllium dust oxidation by steam depending on the dust arrangement geometry

The paper concentrates on the safety issues in the International Thermonuclear Experimental Reactor (ITER) and describes the experiment on the measurement of hydrogen generation rate in case of Ingress of Coolant Event (ICE)—leak inside the vacuum vessel during interaction between water and beryllium (Be) dust. The ICE situation in ITER was simulated in a facility; the active spectroscopy was used to define the hydrogen content by the dynamics of oxidant concentration at a sampling frequency up to 10 Hz. Hydrogen release in time at temperatures of 500-900 °C is investigated, and different versions of dust arrangement are considered, i.e. on the surface and in a slot between armoring tiles at different initial density. The obtained results are compared with the known experiments.     

Tritium Safety-Related Studies at TPL of JAERI

Activities regarding tritium safety technology in the Tritium Process Laboratory (TPL) at Tokai Establishment of Japan Atomic Energy Research Institute are reviewed. Research and development of a new tritium removal system is being carried out by using a gas separation membrane which enable to make the ITER atmosphere detritiation system more compact and cost-effective. Techniques of gas flowing calorimetry and laser Raman spectroscopy are applied to develop new tritium accountancy methods. Studies of tritium-material interaction, such as plasma material interactions, radiochemical reaction of tritium in gas phase, radiolysis of tritiated water, and waste processing are being carried out under ITER/EDA and U.S.-Japan collaboration. Tritium release experiments for research of tritium behavior in confinements and environment and demonstration of safety related components are planned.     

Preliminary experiments: High-energy alpha PIXE in archaeometry

This paper describes the work realized at the “Centre Européen d’Archéométrie” to highlight the utility of high-energy alpha PIXE in the particular field of archaeometry and to introduce the developments done and to be done to complete the knowledge of high-energy alpha PIXE.It starts with the comparison of the yield and the noise background between several alpha particle beams and the comparison between alpha particle and proton beams on different thick and thin references. After, this paper depicts the developments done at the “Institut de Physique Nucléaire, Atomique et Spectroscopie” to perform such high-energy experiments, first on standards and later on cultural heritage objects. Moreover, it introduces the problematics of such beams for the quantification in PIXE by the intermediary of the knowledge of the ionization and X-ray production cross-sections and also the developments done to answer to this serious lack in the databases.