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1.
Xiao-Ya Shangguan Bao-Lun Fang Chen-Xiao Xu Yuan Tan Yan-Gang Chen Zhi-Jun Xia Wei Chen 《Ceramics International》2021,47(5):6318-6328
A series of direct Z-scheme FeIn2S4/Bi2WO6 hierarchical heterostructures with intimate interface contacts were synthesized by in-situ growth route and characterized by systematical analyses. All as-prepared FeIn2S4/Bi2WO6 nanocomposites showed significantly enhanced photocatalytic activity towards photodegradation for the removal of tetracycline hydrochloride (TCH) in comparison with individual FeIn2S4 and Bi2WO6. Meanwhile, the highest photocatalytic degradation activity can be achieved by modulating adding amount of FeIn2S4 in FeIn2S4/Bi2WO6 nanocomposites and the optimized component ratio of FeIn2S4 to Bi2WO6 is determined to be 10 wt%. The enhanced photocatalytic activity could be ascribed to efficient separation between photogenerated holes and electrons based on the construction of direct Z-scheme system. The high photocatalytic stability of resultant 10 wt% FeIn2S4/Bi2WO6 nanocomposites was revealed through six successive recycling reactions. The main intermediate generated during TCH photodegradation was explored by HPLC-MS. Besides, the direct Z-scheme photocatalytic mechanism was confirmed by band position analysis, electron spin resonance (ESR) and active species capture experiment. 相似文献
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智能工程与控制技术:历史,发展与未来 总被引:3,自引:0,他引:3
本文综述了智能工程和控制技术的发展历程和基本问题。文中着重论述了人工智能在过程控制系统中的必要性及开发实时智能控制系统的步骤;对符号推理系统、耦合推理系统、人工神经网络和集成分布式智能系统的特点和局限进行了比较。最后讨论了计算机集成过程系统(CIPS)的基本问题、基础技术和发展前景。 相似文献
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In the design process of the photocatalytic oxidation (PCO) reactor using TiO2-coated foam nickels, the optimum of catalyst film thickness, light intensity and flow velocity were considered. A model was developed to study the effect of catalyst film thickness on photocatalytic degradation of formaldehyde by a TiO2-coated foam nickel at continuous flow mode. In this model, external mass transfer and internal molecule diffusion-reaction were considered. A first-order kinetics equation was used to account for the photocatalytic reaction. Two exponential equations were employed to describe the distribution of light intensities in foam nickels and catalyst films, respectively. Validated with experimental data, the model can be used to predict the optimal thickness of catalyst films. A method for determining appropriate light intensities was proposed and discussed. The appropriate light intensity can be obtained by giving a margin, regarded as an excess coefficient, to the light intensity calculated based on the assumption of complete use of excited electron–hole pairs. The excess coefficient needs to be determined experimentally. In addition, the optimal flow velocity of PCO reactors could be consistent with the required one by changing the windward area of foam nickels. Based on the theoretical analyses, a novel PCO reactor containing 15 parallel-connected cells was designed. Each reaction cell was composed of an UV lamp and a TiO2-coated tubular foam nickel. The performance of the reactor was tested by degrading gaseous formaldehyde at an indoor concentration level. The results showed that the reactor had low pressure loss and good degradation capability. 相似文献
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瀑布沟水电站导流洞渐变段临时中墩的拆除,采用了微差起爆网络的控制爆破技术,取得了很好的效果。本文着重介绍控制爆破的施工方法、设计依据、设计参数以及爆破方式等。 相似文献
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汽车的NVH(Noise,Vibration and Harshness,即噪声、振动和不平顺性)特性是汽车的五大性能指标之一(另外四个性能指标为:安全性、经济性、环保性和可靠性)。汽车的NVH控制是通过控制汽车中有关 相似文献
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利用CFD软件FLUENT对流体在热管换热器中纵向冲刷方式进行数值模拟,对流场中压降、温度等参数进行了分析。结果表明,在相同情况下纵向冲刷时的流体压降小于横向冲刷,但纵向冲刷时传热效果较差;纵向冲刷时流体压降受管间距与热管长度等因素的影响,并且与热管长度成正比。在热管上加装纵向翅片可有效地改善流体纵向冲刷的换热效果,并且使流场内温度分布更为均匀。 相似文献
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