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Developing highly active, stable and sustainable electrocatalysts for overall water splitting is of great importance to generate renewable H2 for fuel cells. Herein, we report the synthesis of electrocatalytically active, nickel foam-supported, spherical core-shell Fe-poly(tetraphenylporphyrin)/Ni-poly(tetraphenylporphyrin) microparticles (FeTPP@NiTPP/NF). We also show that FeTPP@NiTPP/NF exhibits efficient bifunctional electrocatalytic properties toward both the oxygen evolution reaction (OER) and the hydrogen evolution reaction (HER). Electrochemical tests in KOH solution (1 M) reveal that FeTPP@NiTPP/NF electrocatalyzes the OER with 100 mA cm−2 at an overpotential of 302 mV and the HER with 10 mA cm−2 at an overpotential of 170 mV. Notably also, its catalytic performance for OER is better than that of RuO2, the benchmark OER catalyst. Although its catalytic activity for HER is slightly lower than that of Pt/C (the benchmark HER electrocatalyst), it shows greater stability than the latter during the reaction. The material also exhibits electrocatalytic activity for overall water splitting reaction at a current density of 10 mA cm−2 with a cell voltage of 1.58 V, along with a good recovery property. Additionally, the work demonstrates a new synthetic strategy to an efficient, noble metal-free-coordinated covalent organic framework (COF)-based, bifunctional electrocatalyst for water splitting.  相似文献   
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Stability training refers to the practice, while the surface is unstable and activation stabilizer muscles of the trunk and goals, which may ignore other forms of exercise. For stability, the train network control system is caused by network latency and packet drop out of school. The current study aimed to analyze the accuracy of necessary shooting skills and check the balanced posture, stability, and rifle shooting performance bracelets. There is no burden on the body in different performance groups. No. Equivalent continuous-time model, proposed account. The train network control system model uses Romanov theory, some new analytical techniques to get in, and less conservative results. It will be completed. The effectiveness of the proposed method of numerical display. The proposed training in the correct use of architecture to shape muscle memory training interns position signal trainee lead to incorrect behavior. Students warned that the recent shooting would be suspended after the retry using the selected function when needed for phase detection of unnecessary or excessive exercise pistol. Combined with real-time biofeedback applications, it can lead to accelerated learning, training the number of shots that poverty can be reduced, thereby saving time and costs.  相似文献   
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Buck变换器又称降压变换器、串联开关稳压电源、三端开关型降压稳压器。广泛用于计算机、家用电器、控制系统和通信系统中的电源几乎都是开关电源,具有超快速负载动态响应、高功率变换效率、高功率密度、低电压、大电流的特性.开关变换器作为它的主要电路,故障率较高,对它故障诊断研究是有意义的。基于强跟踪滤波理论,给出了一种开关变换器电路故障实时诊断的一种方法。该方法以建立一种开关变换器电路状态空间模型为基础,利用强跟踪滤波器对电路状态及元件参数进行估计,当元件参数发生软、硬型故障时,根据强跟踪滤波器对元件参数的跟踪结果及修正的Bayes分类算法,可实时诊断开关变换器电路中的元件故障。仿真结果证明了该方法的有效性。  相似文献   
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PPM模型广泛应用于Web预取技术,但大多数的PPM模型不具有自适应性,不能反映用户浏览模式的改变。通过对标准PPM模型的扩展,提出基于滑动窗口的自适应网页预测模型。该模型仅保留处于滑动窗口之内的最近访问序列,从而反映用户兴趣的变化,同时利用非压缩后缀树增量式添加新的用户请求和删除过时的浏览信息,以提高更新速度。实验表明,该模型能更准确地描述用户在Web上的浏览特征,在预取性能上明显地优于以往的模型。  相似文献   
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随着社会信息化的不断发展,数学和计算机的联系性也日益深化。以计算机为工具,以数学为理论基础去解决现实问题,是当代社会对数学专业学生的一个新的要求,也是高校数学专业人才培养的重要方向。在这种时代背景下,对数学专业学生计算机应用能力的培养变得尤为迫切。该文针对内蒙古民族大学数学专业学生计算机能力的现状,做了深度分析,提出了如何提高数学专业学生计算机应用能力的一些具体措施。  相似文献   
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Chen  Jing  Lu  Hui 《Mobile Networks and Applications》2022,27(3):1262-1270
Mobile Networks and Applications - In order to improve the accuracy and performance of classroom teaching effect evaluation, an intelligent teaching mode classroom teaching effect evaluation method...  相似文献   
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A new fusion algorithm for multi-sensor images based on Self-Generating Neural Network (SGNN) and fuzzy logic is proposed in this paper. This study is an extension of the work described in Qin and Bao (2005). First, the order and frequency modifications for the current McKusick and Langley (M–L) optimization are proposed; next, by combining optimization and pruning together, the Pruning-And-One-Optimization-Composite (PAOOC) processing method is raised; and finally, a modified fuzzy fusion scheme using improved SGNN is put forward. Experimental results demonstrate that the posed fuzzy fusion scheme outperforms region-based fusion using wavelet multi-resolution (MR) segmentation, and region-based fusion using tree-structure wavelet MR segmentation, both in visual effect and objective evaluation criteria. In the meantime, simulations also show the effectiveness of our modifications for the current optimization and pruning methods, visually and objectively.  相似文献   
10.
邢熠  叶新铭 《计算机工程》2009,35(24):36-38
针对一致性测试中的静态需求测试通常采用手工方法而产生的效率低问题,提出一种基于统计学习的方法,包括静态需求的关联规则表示,并对采样的协议数据进行关联规则挖掘,如果得到的规则与需求规则一致,静态需求就可以得到统计上的测试检验。该方法在OSPFv3协议测试中取得了较好的效果。  相似文献   
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