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排序方式: 共有453条查询结果,搜索用时 15 毫秒
1.
Liangtao Yang Liang-Yin Kuo Juan Miguel López del Amo Prasant Kumar Nayak Katherine A. Mazzio Sebastian Maletti Daria Mikhailova Lars Giebeler Payam Kaghazchi Teófilo Rojo Philipp Adelhelm 《Advanced functional materials》2021,31(38):2102939
A known strategy for improving the properties of layered oxide electrodes in sodium-ion batteries is the partial substitution of transition metals by Li. Herein, the role of Li as a defect and its impact on sodium storage in P2-Na0.67Mn0.6Ni0.2Li0.2O2 is discussed. In tandem with electrochemical studies, the electronic and atomic structure are studied using solid-state NMR, operando XRD, and density functional theory (DFT). For the as-synthesized material, Li is located in comparable amounts within the sodium and the transition metal oxide (TMO) layers. Desodiation leads to a redistribution of Li ions within the crystal lattice. During charging, Li ions from the Na layer first migrate to the TMO layer before reversing their course at low Na contents. There is little change in the lattice parameters during charging/discharging, indicating stabilization of the P2 structure. This leads to a solid-solution type storage mechanism (sloping voltage profile) and hence excellent cycle life with a capacity of 110 mAh g-1 after 100 cycles. In contrast, the Li-free compositions Na0.67Mn0.6Ni0.4O2 and Na0.67Mn0.8Ni0.2O2 show phase transitions and a stair-case voltage profile. The capacity is found to originate from mainly Ni3+/Ni4+ and O2-/O2-δ redox processes by DFT, although a small contribution from Mn4+/Mn5+ to the capacity cannot be excluded. 相似文献
2.
《Advances in Engineering Software》2007,38(5):295-300
The paper presents the implementation of an association rules discovery data mining task using Grid technologies. For the mining task we are using the Apriori algorithm on top of the Globus toolkit. The case study presents the design and integration of the data mining algorithm with the Globus services. The paper compares the Grid version with related work in the field and we outline the conclusions and future work. 相似文献
3.
《钢铁研究学报(英文版)》2006
Soft-magnetic ferrite has advantages of high initial magnetic permeability, high electric resistivity, low loss and low cost in the high-frequency alternating field. Considering the characters of soft-magnetic ferrite, this paper uses a soft-magnetic ferrite ring as stator core and presents a novel field-weakening structure of high speed PM motors. Based on this structure, a novel field-weakening method of PM motors can be presented. The equivalent reluctance of permanent magnetic field circuit can be changed by altering saturation degree of soft-magnetic ferrite core in this method. For the convenience of analysis and calculation, considering the magnetic field distribution in the motors, this paper deduces an equivalent two-dimensional finite element model of three-dimensional magnetic field, by which the field-weakening parameters of high speed PM motor can be conveniently analyzed. The simulation results of finite element model prove: the field-weakening structure of high speed PM motor based on soft-magnetic ferrite, presented in this paper, is valid and feasible, offers a valid and applicative method for field-weakening control of high speed PM motor. 相似文献
4.
5.
Rongliang Chen Yuqi Wu Zhengzheng Yan Yubo Zhao Xiao-Chuan Cai 《Journal of scientific computing》2014,58(2):275-289
Numerical simulation of three-dimensional incompressible flows at high Reynolds number using the unsteady Navier–Stokes equations is challenging. In order to obtain accurate simulations, very fine meshes are necessary, and such simulations are increasingly important for modern engineering practices, such as understanding the flow behavior around high speed trains, which is the target application of this research. To avoid the time step size constraint imposed by the CFL number and the fine spacial mesh size, we investigate some fully implicit methods, and focus on how to solve the large nonlinear system of equations at each time step on large scale parallel computers. In most of the existing implicit Navier–Stokes solvers, segregated velocity and pressure treatment is employed. In this paper, we focus on the Newton–Krylov–Schwarz method for solving the monolithic nonlinear system arising from the fully coupled finite element discretization of the Navier–Stokes equations on unstructured meshes. In the subdomain, LU or point-block ILU is used as the local solver. We test the algorithm for some three-dimensional complex unsteady flows, including flows passing a high speed train, on a supercomputer with thousands of processors. Numerical experiments show that the algorithm has superlinear scalability with over three thousand processors for problems with tens of millions of unknowns. 相似文献
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7.
《Diamond and Related Materials》2005,14(10):1673-1677
This paper summarizes the preliminary results obtained from lithium electrochemical intercalation into boron-doped diamond films grown on carbon felt (BDD/CF electrode). BDD films have been grown by Hot Filaments Chemical Vapor Deposition (HFCVD) and have been characterized by Scanning Electron Microscopy (SEM) and Raman Scattering spectroscopy. BDD/CF composite electrodes, which contain a diamond layer, lead to higher conductivity and smaller grain sizes. In turn, they are richer in boundary or sp2 sites, and present a reversible specific capacity that is much larger than that of the substrate alone, indicating that the diamond layer effectively participates in lithium storage. Diamond layers displaying boron doping levels of 1019 and 1021 part cm− 3 provide a specific capacity of 160 and 370 mA h g− 1, respectively, which is associated with lithium storage. 相似文献
8.
我国西南地区地质灾害频发,为了探索该区域地质灾害的分布特征,以内江市为研究区,利用遥感卫星影像及地理国情监测数据,从自然地理、生态条件和基础地质3个方面建立生态地质环境评价指标体系。采用层次分析法(AHP)和二元Logistic回归模型分别确定各评价指标的主、客观权重,再用最小信息熵求出两者的综合权重,在GIS支持下建立地质灾害评价模型,对内江市地质灾害进行风险性评价分级;并通过高权重评价因子与历史地质灾害点的空间结构分析,揭示其空间分布特征及规律。评估结果表明:①内江市地质灾害中高易发区主要分布在西部低山区,占全区总面积的28.93%;②海拔和坡度是导致地质灾害发生的主要影响因子,在海拔较高、坡度较陡地区,且山区公路两旁极易发生地质灾害,沉寂式构造线附近地层相对稳定。 相似文献
9.
《Journal of the European Ceramic Society》2021,41(14):7375-7379
New generation wireless communication systems require characterisations of dielectric permittivity and loss tangent at microwave and terahertz bands. La2Ti2O7 is a candidate material for microwave application. However, all the reported microwave dielectric data are average value from different directions of a single crystal, which could not reflect its anisotropic nature due to the layered crystal structure. Its dielectric properties at the microwave and terahertz bands in a single crystallographic direction have rarely been reported. In this work, a single crystal ferroelectric La2Ti2O7 was prepared by floating zone method and its dielectric properties were characterized from 1 kHz to 1 THz along one single direction. The decrease in dielectric permittivity with increasing frequency is related to dielectric relaxation from radio frequency to microwave then to terahertz band. The capability of characterizing anisotropic dielectric properties of a single crystal in this work opens the feasibility for its microwave and terahertz applications. 相似文献
10.