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51.
Nobuyuki Gokon Yusuke Osawa Daisuke Nakazawa Tatsuya Kodama 《International Journal of Hydrogen Energy》2009
Ni–Cr–Al metallic foam absorber with high porosity was catalytically activated using a Ru/γ-Al2O3 catalyst, and was subsequently tested with respect to CO2 reforming of methane in a small-scale volumetric receiver-reactor by using a sun-simulator. A chemical storage efficiency of 37% was obtained for a mean light flux of 325 kW m−2. Furthermore, the activity and the stability of the metallic foam absorber were compared with those of a SiC foam absorber activated with the same Ru/γ-Al2O3 catalyst for 50 h of light irradiation, and it was found that the metallic foam absorber has superior catalytic stability in comparison to the SiC form absorber. In addition, unlike ceramic foams such as SiC, metallic foams feature superior plasticity, which prevents the emergence of cracks caused by mechanical or thermal shock. 相似文献
52.
Wet dispersion mechanism of fine aggregates in multiphase flow with solid beads under simple shear 下载免费PDF全文
Daisuke Nishiura Hide Sakaguchi Atsuko Shimosaka 《American Institute of Chemical Engineers》2014,60(12):4076-4085
Clarifying the disintegration mechanism of aggregates in multiphase fluid flow coupled with beads and particulates is important for the optimum design of a wet dispersion process using a stirred media mill. Thus, we develop a numerical method for simulating multiphase flow with beads and particulates using a discrete element method and computational fluid dynamics, and we use the four‐way coupling simulation to study the fluid‐bead‐particulate‐coupled phenomenon that occurs in a simple shear box. The results show that the dominant force causing aggregate disintegration is the fluid force, rather than the bead contact force, because aggregates rarely collide with beads, contact force of which is too small to disintegrate aggregates. Furthermore, aggregates with strong aggregation force are effectively disintegrated by the fluid flow with a dominant high pure‐shear rate induced near the bead surfaces by the expansive force, rather than the compressive force. © 2014 American Institute of Chemical Engineers AIChE J 60: 4076–4085, 2014 相似文献
53.
各种引气剂以及抑泡剂对混凝土经时变化状态等的影响 总被引:1,自引:0,他引:1
众所周知,采用粉煤灰制备混凝土,因粉煤灰成分中含有未燃炭等微粒子,容易造成阴离子型引气剂吸附在这些微粒子上,导致含气量经时损失.同时在混凝土的制备、运输过程中,因受采用的材料、拌和状态等物理因素影响,还会发生含气量经时增加的现象.所以在制备、管理混凝土时,如何保证出机初期一定的含气量、缓解含气量的经时损失或经时增加,是一项极其关键的技术.本文将就采用能改善上述状态的引气剂、抑泡剂拌和混凝土,对混凝土的经时变化以及抗冻融性等特征产生的影响进行论述. 相似文献
54.
55.
Hideki Tanaka Daisuke Noguchi Akiko Yuzawa Tetsuya Kodaira Hirofumi Kanoh Katsumi Kaneko 《Journal of Low Temperature Physics》2009,157(3-4):352-373
We have investigated the applicability of simulations and theoretical techniques for exploring the selectivities of hydrogen isotopes. We have simulated the adsorption isotherms of H2 in an idealized carbon slit pore at 77 K by using the grand canonical Monte Carlo simulations with the Feynman-Hibbs effective potential (FH-GCMC) and the rigorous path integral method (PI-GCMC), and we obtained good agreement between the isotherms from both simulations. This suggests that FH-GCMC, which uses the approximative Feynman-Hibbs treatment, is as useful as PI-GCMC for exploring H2 adsorption at 77 K. Moreover, we show that the ideal adsorption solution theory (IAST) can predict the selectivity of D2 over H2 in the interstices of single-wall carbon nanotube (SWNT) bundles at 77 K (below 0.1 MPa) very well by comparing the obtained results with the mixture adsorption FH-GCMC simulations. This indicates that IAST is also applicable to the estimation of the selectivity of D2 over H2 at moderate pressures and at 77 K from experimental single-component adsorption isotherms. We also demonstrate that the FH-GCMC simulation can reproduce the experimental adsorption isotherms of H2 and D2 in aluminophosphate AlPO4-5 at 77 K. Finally, we analyze the selectivity of D2 over H2 by IAST with the experimental single-component adsorption isotherms of H2 and D2 at 77 K for a variety of adsorbents: AlPO4-5, activated carbon fibers (ACFs), HiPco SWNT, and SWNHs. The selectivities predicted by the experimental adsorption data based on the results from the FH-GCMC simulations are presented and discussed. 相似文献
56.
Corrosion characteristics of reduced activation ferritic steel, JLF-1 (8.92Cr–2W) in molten salts Flibe and Flinak 总被引:1,自引:0,他引:1
Masatoshi Kondo Takuya Nagasaka Qi Xu Takeo Muroga Akio Sagara Nobuaki Noda Daisuke Ninomiya Masaru Nagura Akihiro Suzuki Takayuki Terai Naoki Fujii 《Fusion Engineering and Design》2009,84(7-11):1081-1085
Static corrosion tests were performed in molten salts, LiF–BeF2 (Flibe) and LiF–NaF–KF (Flinak), at 500 °C and 600 °C for 1000 h. The purpose is to investigate the corrosion characteristics of reduced activation ferritic steels, JLF-1 (8.92Cr–2W) in the fluids. The concentration of hydrogen fluoride (HF) in the fluids was measured by slurry pH titration method before and after the exposure. The HF concentration determined the fluoridation potential. The corrosion was mainly caused by dissolution of Fe and Cr into the fluids due to fluoridation and/or electrochemical corrosion. Carbon on the surface might be dissolved into the fluids due to the corrosion, and this resulted to the decrease of carbide on the surface. The corrosion depth of the JLF-1 specimen, which was obtained from the weight losses, was 0.637 μm in Flibe at 600 °C and 6.73 μm in Flinak at 600 °C. 相似文献
57.
58.
The effects of accelerating voltage and collection angle on the mean free path for all inelastic electron scattering (lambdap), which is an important parameter for determining specimen thickness by using electron energy-loss spectroscopy, were investigated with crystalline Si and amorphous SiO2. First, thickness of Si film was measured with the convergent-beam electron diffraction method, while thickness of SiO2 particles was estimated from their spherical shape. Then from electron energy-loss spectra, lambdap was evaluated for Si film and SiO2 particles by changing the accelerating voltage (100 to approximately 300 kV) and the collection angle for the scattered electrons. Under the condition of no objective aperture, lambdap for Si film and SiO2 particles was found to increase with the increase of accelerating voltage and to take values of 180+/-6 nm (Si) and 247+/-8 nm (SiO2) at 300 kV. Also, it was found that lambdap in both cases decreases drastically with the increase of collection angle in the range smaller than 25 mrad, while it tends to take a constant value at the collection angle larger than 25 mrad at 200 kV. 相似文献
59.
Determining surface orientations of transparent objects based on polarization degrees in visible and infrared wavelengths 总被引:1,自引:0,他引:1
Miyazaki D Saito M Sato Y Ikeuchi K 《Journal of the Optical Society of America. A, Optics, image science, and vision》2002,19(4):687-694
Techniques for modeling an object through observation are very important in object recognition and virtual reality. A wide variety of techniques have been developed for modeling objects with opaque surfaces, whereas less attention has been paid to objects with transparent surfaces. A transparent surface has only surface reflection; it has little body reflection. We present a new method for obtaining surface orientations of transparent surfaces through analysis of the degree of polarization in surface reflection and emission in visible and far-infrared wavelengths, respectively. This parameter, the polarization degree of reflected light at the visible wavelengths, is used for determining the surface orientation at a surface point. The polarization degree at visible wavelengths provides two possible solutions, and the proposed method uses the polarization degree at far-infrared wavelengths to resolve this ambiguity. 相似文献
60.
Steroid cyclophanes, each having a macrocyclic ring attached to four bile acid moieties via chiral lysine connectors, were synthesized, and the binding of the 2-naphthylphenylketone (guest) to the steroid cyclophanes in water was investigated. The circular dichroism spectra of the steroid cyclophane with cholic acid and L-lysine were significantly affected by the binding of the guest, and the induced circular dichroism based on the absorption of the achiral guest was also observed. The binding of the guest to the steroid cyclophane with cholic acids and D-lysines induced changes in the circular dichroism spectra with the opposite sign of the molecular ellipticities. An induced circular dichroism spectral change was not observed upon binding of the guest to the analogous host without OH sites. These results strongly suggest that the guest is conformationally fixed through hydrogen bonding between the carbonyl group of the guest and the steroidal hydroxyl group of the host. The assembly of only four steroid residues on the macrocyclic ring probably provided a hydrophobic nanocavity for hydrogen bonding. 相似文献