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Rong Zhang Hailong Hu Hai Chen Siqi Li Cheng Ying Shuai Huang Qingting Liu Xudong Fu Shengfei Hu Ching-Ping Wong 《应用聚合物科学杂志》2020,137(39):49186
Recently, thermal interface materials (TIMs) are in great demands for modern electronics. For mechanically mixed polymer composite TIMs, the thermal conductivity and the mechanical properties are generally lower than expected values due to the sharply increased viscosity and poor filler dispersion. This work shows that addition of a small amount of polyester-based hyperbranched polymer (HBP) avoided the trade-off in mechanically mixed ABS/hexagonal boron nitride (h-BN) composites. After adding 0.5 wt% HBP, the maximum h-BN content in the composites increased from 50 to 60 wt%. The out-of-plane, in-plane thermal conductivity, and tensile strength of ABS/h-BN with 50 wt% h-BN were 0.408, 0.517 W/mK, and 18 MPa, respectively, and were increased to 0.729, 0.847 W/mK, and 32 MPa by adding 0.5 wt% HBP, while 0.972, 1.12 W/mK, and 29.5 MPa were achieved for ABS/h-BN/HBP with 60 wt% h-BN. The morphological and rheological results proved that these enhancements are due to the improved h-BN dispersion by decreasing viscosity of composites during mixing. Theoretical modeling based on the modified effective medium theory confirmed such results and showed that the interfacial thermal resistance also decreased slightly. Thus, this work demonstrates a facile and scalable method for simultaneously improving the thermal conductivity and mechanical properties of thermoplastic-based TIMs. 相似文献
23.
Chuntao Lan Haiyang Zou Longfei Wang Meng Zhang Shuang Pan Ying Ma Yiping Qiu Zhong Lin Wang Zhiqun Lin 《Advanced materials (Deerfield Beach, Fla.)》2020,32(47):2005481
Despite recent rapid advances in metal halide perovskites for use in optoelectronics, the fundamental understanding of the electrical-poling-induced ion migration, accounting for many unusual attributes and thus performance in perovskite-based devices, remain comparatively elusive. Herein, the electrical-poling-promoted polarization potential is reported for rendering hybrid organic–inorganic perovskite photodetectors with high photocurrent and fast response time, displaying a tenfold enhancement in the photocurrent and a twofold decrease in the response time after an external electric field poling. First, a robust meniscus-assisted solution-printing strategy is employed to facilitate the oriented perovskite crystals over a large area. Subsequently, the electrical poling invokes the ion migration within perovskite crystals, thus inducing a polarization potential, as substantiated by the surface potential change assessed by Kelvin probe force microscopy. Such electrical-poling-induced polarization potential is responsible for the markedly enhanced photocurrent and largely shortened response time. This work presents new insights into the electrical-poling-triggered ion migration and, in turn, polarization potential as well as into the implication of the latter for optoelectronic devices with greater performance. As such, the utilization of ion-migration-produced polarization potential may represent an important endeavor toward a wide range of high-performance perovskite-based photodetectors, solar cells, transistors, scintillators, etc. 相似文献
24.
Qi Yang Qilong Wu Yang Liu Shuiping Luo Xiaotong Wu Xixia Zhao Haiyuan Zou Baihua Long Wen Chen Yujia Liao Lanxi Li Pei Kang Shen Lele Duan Zewei Quan 《Advanced materials (Deerfield Beach, Fla.)》2020,32(36):2002822
Engineering novel Sn-based bimetallic materials could provide intriguing catalytic properties to boost the electrochemical CO2 reduction. Herein, the first synthesis of homogeneous Sn1−xBix alloy nanoparticles (x up to 0.20) with native Bi-doped amorphous SnOx shells for efficient CO2 reduction is reported. The Bi-SnOx nanoshells boost the production of formate with high Faradaic efficiencies (>90%) over a wide potential window (−0.67 to −0.92 V vs RHE) with low overpotentials, outperforming current tin oxide catalysts. The state-of-the-art Bi-SnOx nanoshells derived from Sn0.80Bi0.20 alloy nanoparticles exhibit a great partial current density of 74.6 mA cm−2 and high Faradaic efficiency of 95.8%. The detailed electrocatalytic analyses and corresponding density functional theory calculations simultaneously reveal that the incorporation of Bi atoms into Sn species facilitates formate production by suppressing the formation of H2 and CO. 相似文献
25.
Wireless Personal Communications - The existing long term evolution networks originally designed for human-to-human communications are hard to tackle numerous and bursty random access requests from... 相似文献
26.
Thermoresponsive behavior and rheology of SiO2–hyaluronic acid/poly(N‐isopropylacrylamide) (NaHA/PNIPAm) core–shell structured microparticles 下载免费PDF全文
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通过对氨汽提尿素装置高压系统合成操作压力的理论分析,结合实际工况降低高压系统操作压力,使装置的设备运转状况得到有效改善。 相似文献
29.
采用CO2激光点火装置联合高速摄影系统及扫描电子显微镜等凝聚相燃烧产物分析技术,研究了高氯酸铵(AP)含量对高Al富燃料推进剂中重要组分AP/Al一次燃烧过程中燃烧现象、引燃时间、燃烧扩散时间、燃尽时间、燃烧效率、颗粒团聚及凝聚相燃烧产物的表面形貌、粒径及其分布的影响。结果表明,各AP/Al混合粉体的燃烧过程均可分为表面引燃、燃烧扩散和火焰熄灭3个阶段,但各样品在不同燃烧阶段的燃烧现象存在明显差异。AP含量由10wt%增至30wt%,样品燃烧剧烈程度增强,燃烧过程中固相颗粒的溅射现象越加明显;在火焰熄灭阶段,各样品燃烧由以停留在样品燃面处的燃烧为主逐渐变为以溅射颗粒的燃烧为主,且随反应进行,燃面已燃固相颗粒最先熄灭,各样品表面引燃时间、燃烧扩散时间、燃烧持续时间均缩短,即燃烧反应速率逐渐加快。在AP/Al混合物中,铝粉的燃烧效率、凝聚相燃烧产物粒度及其团聚程度随AP含量增加而增加。 相似文献
30.
考虑旋流衰减的影响,对气液螺旋环状流的压降特性进行研究并推导出了螺旋环状流压降预测模型。定义压降旋-直比系数为气液两相螺旋环状流和气液两相直流的压降之比,以此来表征旋流衰减对压降的影响。基于量纲分析的方法对压降旋-直比系数进行分析,推导出其表达式,压降旋-直比系数依赖于Lockhart-Martinelli 参数和气相Froude数变化。最终,得出了气液两相螺旋环状流的压降预测模型。在50 mm内径的水平管内对螺旋环状流的压降特性进行了实验研究,其中气相表观流速变化范围为10~16 m/s,体积含液率(LVF)变化范围为0.6%~4.8%。通过与实验数据进行对比,压降预测模型的相对误差在±15%以内,为工程应用提供了参考。 相似文献