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Polyfluorene Derivatives are High‐Performance Organic Hole‐Transporting Materials for Inorganic−Organic Hybrid Perovskite Solar Cells 下载免费PDF全文
Zonglong Zhu Yang Bai Harrison Ka Hin Lee Cheng Mu Teng Zhang Lixia Zhang Jiannong Wang He Yan Shu Kong So Shihe Yang 《Advanced functional materials》2014,24(46):7357-7365
Photovoltaics based on organic?inorganic perovskites offer new promise to address the contemporary energy and environmental issues. These solar cells have so far largely relied on small‐molecule hole transport materials such as spiro‐OMeTAD, which commonly suffer from high cost and low mobility. In principle, polyfluorene copolymers can be an ideal alternative to spiro‐OMeTAD, given their low price, high hole mobility and good processability, but this potential has not been explored. Herein, polyfluorene derived polymers‐TFB and PFB, which contain fluorine and arylamine groups, are demonstrated and can indeed rival or even outperform spiro‐OMeTAD as efficient hole‐conducting materials for perovskite solar cells. In particular, under the one‐step perovskite deposition condition, TFB achieves a 10.92% power conversion efficiency that is considerably higher than that with spiro‐OMeTAD (9.78%), while using the two‐step perovskite deposition method, about 13% efficient solar cells with TFB (12.80%) and spiro‐OMeTAD (13.58%) are delivered. Photoluminescence reveals the efficient hole extraction and diffusion at the interface between CH3NH3PbI3 and the hole conducting polymer. Impedance spectroscopy uncovers the higher electrical conductivity and lower series resistance than spiro‐OMeTAD, accounting for the significantly higher fill factor, photocurrent and open‐circuit voltage of the TFB‐derived cells than with spiro‐MeOTAD. 相似文献
73.
Chen J 《Journal of the Optical Society of America. A, Optics, image science, and vision》2007,24(1):84-92
On the basis of expanding a hard-edged aperture function as a finite sum of complex Gaussian functions, an approximate analytical expression for the propagation of an input complex amplitude distribution passing through a general nonsymmetrical apertured double-lens system is derived. Then, the propagation result for two-dimensional flat-topped multi-Gaussian beams is given. It is shown that the apertured Lohmann's symmetrical double-lens system for fractional Fourier transform is a special case of the general apertured double-lens system. The numerical calculation, graphical illustration, and some discussions for the transformation of the two-dimensional flat-topped multi-Gaussian beam in apertured Lohmann's symmetrical double-lens systems are also presented. 相似文献
74.
分析和探讨了立井掘进深孔爆破中的掏槽形式和掏槽参数、周边光面爆破参数和光爆装药结构等技术问题,提出了一些较为切合实际的技术观点. 相似文献
75.
针对在装1 000MW汽轮机组的结构特点,提出了节能降耗的一些改进措施,并在机组安装及调试过程中实施。该机组试运后与已投运的同类型机组相比,节能效果显著,仅高、中压缸效率分别提高1.5%和0.2%。 相似文献
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Hui Cheng Jiannong Cao Xingwei Wang Sajal K. Das Shengxiang Yang 《Wireless Communications and Mobile Computing》2009,9(6):759-771
Clustering can help aggregate the topology information and reduce the size of routing tables in a mobile ad hoc network (MANET). The maintenance of the cluster structure should be as stable as possible to reduce overhead and make the network topology less dynamic. Hence, stability measures the goodness of clustering. However, for a complex system like MANET, one clustering metric is far from reflecting the network dynamics. Some prior works have considered multiple metrics by combining them into one weighted sum, which suffers from intrinsic drawbacks as a scalar objective function to provide solution for multi‐objective optimization. In this paper, we propose a stability‐aware multi‐metric clustering algorithm, which can (1) achieve stable cluster structure by exploiting group mobility and (2) optimize multiple metrics with the help of a multi‐objective evolutionary algorithm (MOEA). Performance evaluation shows that our algorithm can generate a stable clustered topology and also achieve optimal solutions in small‐scale networks. For large‐scale networks, it outperforms the well‐known weighted clustering algorithm (WCA) that uses a weighted sum of multiple metrics. Copyright © 2008 John Wiley & Sons, Ltd. 相似文献
78.
Lei Guo Jiannong Cao Xingwei Wang Dingde Jiang Ting Yang 《Optical Fiber Technology》2010,16(3):162-171
With the number of wavelengths on fibers keeps increasing, the size and the cost of Optical Cross-Connect (OXC) are greatly enhanced and then the control and management of optical switches become more and more complicated. Therefore, the technique called waveband switching is proposed to reduce the size and the cost of OXC; that is, to save the All-Optical (OOO) switching ports in OXC. However, the existing waveband switching algorithms are all limited in single-domain optical networks. Actually, with the scale of optical backbone keeps enlarging, the network is divided to multiple independent domains to perform the hierarchy routing for achieving the scalability. In order to reduce the size and the cost of OXC meanwhile to achieve the scalability in multi-domains, in this paper we propose a new heuristic algorithm called Waveband Grooming with Layered Auxiliary Graph (WGLAG) since the waveband grooming problem is the NP-hard to perform the inter-domain routing based on the virtual topology of multi-domain network and the intra-domain routing based on the physical topology of single-domain network. In intra-domain routing with waveband grooming of each single-domain, we propose the Layered Auxiliary Graph (LAG) that includes one virtual topology layer and multiple waveband-plane layers to compute a single-hop, or multi-hop or hybrid waveband route for each connection request based on the sub-path waveband grooming scheme. Simulation results show that, WGLAG not only can effectively save more switching ports to reduce the cost of OXC but also can obtain lower blocking probability than other algorithm. 相似文献
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