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91.
92.
Pascal Habimana Yanjun Jiang Jing Gao Jean Bernard Ndayambaje Osama M. Darwesh Jean Pierre Mwizerwa Xiaobing Zheng Li Ma 《中国化学工程学报》2022,48(8):66-75
The continuous use of chemical dyes in various industries, and their discharge into industrial effluents, results in severe problems to human life and water pollution. Laccases have the ability to decolorize dyes and toxic chemicals in industrial effluents as green biocatalysts. Their possible industrial applications have been limited by poor reusability, low stability, and loss of free laccase action. In this research, laccase was immobilized on zeolitic imidazolate framework coated multi-walled carbon nanotubes (Laccase@ZIF-8@MWCNTs) via metal affinity adsorption to develop an easy separable and stable enzyme. The optimum reaction conditions for immobilized laccase are at a pH of 3.0 and a temperature of 60?℃. The immobilized laccase was enhanced in storage and thermal stability. The results indicated that Laccase@ZIF-8@MWCNTs still maintained 68% of its original activity after 10 times of repeated use. Most importantly, the biocatalytic system was applied for decolorization of different dyes (20?mg·L?1) without a mediator, and up to 97.4% for Eriochrome black T and 95.6% Acid red 88 was achieved in 25 min. Biocatalysts with these properties may be used in a variety of environmental and industrial applications. 相似文献
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Pascal Steiner Enrico Gnecco Tobin Filleter Nitya Nand Gosvami Sabine Maier Ernst Meyer Roland Bennewitz 《Tribology Letters》2010,39(3):321-327
We review recent friction measurements on ordered superstructures performed by atomic force microscopy. In particular, we
consider ultrathin KBr films on NaCl(001) and Cu(001) surfaces, single and bilayer graphene on SiC(0001), and the herringbone
reconstruction of Au(111). Atomically resolved friction images of these systems show periodic features spanning across several
unit cells. Although the physical mechanisms responsible for the formation of these superstructures are quite different, the
experimental results can be interpreted within the same phenomenological framework. A comparison between experiments and modeling
shows that, in the cases of KBr films on NaCl(001) and of graphene films, the tip-surface interaction is well described by
a potential with the periodicity of the substrate which is modulated or, respectively, superimposed with a potential with
the symmetry of the superstructure. 相似文献
96.
David Morin Yoann Stevenin Cédric Grolleau Pascal Brault 《International Journal of Hydrogen Energy》2018,43(45):21017-21029
Nowadays islanded microgrids mostly rely on diesel generator. In order to reduce greenhouse emissions, two islanded microgrids with hydrogen storage have been installed and are currently working autonomously in Reunion Island and France. Energy management implemented on these stations fall in the myopic control category. This study aims to determine the performance improvement that could be achieve on such stations using model predictive control. Ability to supply to the loads and energy losses minimisation are our main objectives. Lifetime degradation is also taken in consideration. Simulations shows that significant improvement can be brought, with a 76% decrease of the station's defaults time and better fill rate of hydrogen tank and batteries. In the meantime, chemical and electrical losses are reduced by 38 and 11%, and the batteries degradations are decreased by around 1%. The relevance of taking into account the electrolyser and fuel cell degradations depends on the time-step of the control. These results give a performance target in order to implement a real-time model predictive control in the microgrids, and eventually can be used to better sizing of future microgrids with similar architecture. 相似文献
97.
Pascal Suer Jan-Erik Lindqvist Paul Frogner-Kockum 《The Science of the total environment》2009,407(18):5110-5118
Reuse of industrial aggregates is still hindered by concern for their long-term properties. This paper proposes a laboratory method for accelerated ageing of steel slag, to predict environmental and technical properties, starting from fresh slag. Ageing processes in a 10-year old asphalt road with steel slag of electric arc furnace (EAF) type in the subbase were identified by scanning electron microscopy (SEM) and leaching tests. Samples from the road centre and the pavement edge were compared with each other and with samples of fresh slag. It was found that slag from the pavement edge showed traces of carbonation and leaching processes, whereas the road centre material was nearly identical to fresh slag, in spite of an accessible particle structure. Batches of moisturized road centre material exposed to oxygen, nitrogen or carbon dioxide (CO2) were used for accelerated ageing. Time (7-14 days), temperature (20-40 °C) and initial slag moisture content (8-20%) were varied to achieve the carbonation (decrease in pH) and leaching that was observed in the pavement edge material. After ageing, water was added to assess leaching of metals and macroelements. 12% moisture, CO2 and seven days at 40 °C gave the lowest pH value. This also reproduced the observed ageing effect for Ca, Cu, Ba, Fe, Mn, Pb, Ca (decreased leaching) and for V, Si, and Al (increased leaching). However, ageing effects on SO4, DOC and Cr were not reproduced. 相似文献
98.
Mourad Ben Amor Pascal Lesage Pierre-Olivier Pineau Réjean Samson 《Renewable & Sustainable Energy Reviews》2010,14(9):2885-2895
Renewable distributed electricity generation can play a significant role in meeting today's energy policy goals, such as reducing greenhouse gas emissions, improving energy security, while adding supply to meet increasing energy demand. However, the exact potential benefits are still a matter of debate. The objective of this study is to evaluate the life cycle implications (environmental, economic and energy) of distributed generation (DG) technologies. A complementary objective is to compare the life cycle implications of DG technologies with the centralized electricity production representing the Northeastern American context. Environmental and energy implications are modeled according to the recommendations in the ISO 14040 standard and this, using different indicators: Human Health; Ecosystem Quality; Climate Change; Resources and Non-Renewable Energy Payback Ratio. Distinctly, economic implications are modeled using conventional life cycle costing. DG technologies include two types of grid-connected photovoltaic panels (3 kWp mono-crystalline and poly-crystalline) and three types of micro-wind turbines (1, 10 and 30 kW) modeled for average, below average and above average climatic conditions in the province of Quebec (Canada). A sensitivity analysis was also performed using different scenarios of centralized energy systems based on average and marginal (short- and long-term) technology approaches. Results show the following. First, climatic conditions (i.e., geographic location) have a significant effect on the results for the environmental, economic and energy indicators. More specifically, it was shown that the 30 kW micro-wind turbine is the best technology for above average conditions, while 3 kWp poly-crystalline photovoltaic panels are preferable for below average conditions. Second, the assessed DG technologies do not show benefits in comparison to the centralized Quebec grid mix (average technology approach). On the other hand, the 30 kW micro-wind turbine shows a potential benefit as long as the Northeastern American electricity market is considered (i.e., oil and coal centralized technologies are affected for the short- and long-term marginal scenarios, respectively). Photovoltaic panels could also become more competitive if the acquisition cost decreased. In conclusion, DG utilization will represent an improvement over centralized electricity production in a Northeastern American context, with respect to the environmental, energy and economic indicators assessed, and under the appropriate conditions discussed (i.e., geographical locations and affected centralized electricity production scenarios). 相似文献
99.
Mohamed Kamel Hadj-Kali Vincent Gerbaud Jean-Marc Borgard Olivier Baudouin Pascal Floquet Xavier Joulia Philippe Carles 《International Journal of Hydrogen Energy》2009
The HIx ternary system (H2O–HI–I2) is the latent source of hydrogen for the Sulfur–Iodine thermo-chemical cycle. After analysis of the literature data and models, a homogeneous approach with the Peng–Robinson equation of state used for both the vapor and liquid phase fugacity calculations is proposed for the first time to describe the phase equilibrium of this system. The MHV2 mixing rule is used, with UNIQUAC activity coefficient model combined with of hydrogen iodide solvation by water. This approach is theoretically consistent for HIx separation processes operating above HI critical temperature. Model estimation is done on selected literature vapor–liquid, liquid–liquid, vapor–liquid–liquid and solid–liquid equilibrium data for the ternary system and the three binaries subsystems. Validation is done on the remaining literature data. Results agree well with the published data, but more experimental effort is needed to improve modeling of the HIx system. 相似文献
100.
Raphaël Faure Fabrice RossignolClaire Bonhomme Alexandre MaîtreGrégory Etchegoyen Pascal Del GalloDaniel Gary 《Journal of the European Ceramic Society》2011,31(3):303-312
The manufacture and the characterisation of alumina foams as alternative catalysts supports for industrial steam reforming processes are presented here. The possibility of use of alumina foams as catalysts supports in such processes is evaluated by studying their resistance toward mechanical and chemical stresses. The alumina foams produced are characterised owing to their processing parameters (slurry infiltration, sintering temperature, template pore size). Their ability to work in hydrothermal atmosphere is assessed by characterising the evolution of microstructures and mechanical strengths upon aging. Thermodynamic studies of the stability of alumina in industrial steam reforming working conditions are performed and correlated to the experiments to demonstrate the stability of such a system. 相似文献