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151.
Combined Single-Pass Conversion of Methane Via Oxidative Coupling and Dehydroaromatization 总被引:1,自引:0,他引:1
Yonggang Li Lingling Su Hongxia Wang Hongmei Liu Wenjie Shen Xinhe Bao Yide Xu 《Catalysis Letters》2003,89(3-4):275-279
A new reaction mode, i.e., the combined single-pass conversion of methane via oxidative coupling (OCM) over mixed metal oxide (SLC) catalysts and dehydroaromatization (MDA) over Mo/HZSM-5 catalysts, is reported. With the assistance of an OCM reaction over SLC catalysts in the top layer of the reactor, the deactivation resistance of Mo/HZSM-5 catalysts is remarkably enhanced. Under the selected reaction conditions, the CH4 conversion decreased from 18 to 1% and the aromatics yield decreased from 12.8 to 0.1%, respectively, after running the reaction for 960min on both 6Mo/HZSM-5 and SLC-6Mo/HZSM-5 catalyst system without O2 in the feed. On the other hand, for the SLC-6Mo/HZSM-5 catalyst system with O2 in the feed, the deactivation was improved greatly, and after 960min onstream the CH4 conversion and aromatics yield were still as high as 12.0 and 8.0%, respectively. The promotion effect mainly appears to be associated with in situ formation of CO2 in the OCM layer, which reacts with coke via the reverse Boudouard reaction. 相似文献
152.
本文对高聚合度聚氯乙烯(H-PVC)的发展及其优异的物理机械性能作了简要介绍;着重分析了H-PVC的加工性能和表征方法,并讨论了分子特性和颗料特性及加工组成、加工条件对加工性能的影响,提出了改进H-PVC加工性能的方法。 相似文献
153.
通过IR分析了用顺酐和反酸与聚酯合成不饱和聚酯树脂的反应机理,讨论了二种树脂体系固化放热曲线不同的原因。 相似文献
154.
Under the applied high reaction temperatures (900 K) the Ag surface is restructured and a tightly held oxygen species is formed on the surface (O) apart from O atoms dissolved in the bulk (O). Methanol oxidation to formaldehyde proceeds through this O species as demonstrated by application of a variety of spectroscopic techniques. 相似文献
155.
Bulk silver catalysts were found to be active for the oxidative coupling of methane to ethane and ethylene if operated under oxygen-limited conditions at atmospheric pressure and at temperatures above 1020 K. The addition of small amounts of sodium phosphate as promoter increases markedly the C2 selectivity (to values above 90%) and yield (>10%) by efficient suppression of reaction steps leading to total oxidation. Further improvement of the yields might be achieved by more appropriate reactor design. 相似文献
156.
Variation trends of water resources in the Xiangjiang River Basin over the coming decades have been investigated using the variable infiltration capacity(VIC) model and 14 general circulation models'(GCMs') projections under the representative concentration pathway(RCP4.5) scenario. Results show that the Xiangjiang River Basin will probably experience temperature rises during the period from 2021 to2050, with precipitation decrease in the 2020 s and increase in the 2030 s. The VIC model performs well for monthly discharge simulations with better performance for hydrometric stations on the main stream of the Xiangjiang River than for tributary catchments. The simulated annual discharges are significantly correlated to the recorded annual discharges for all the eight selected target stations. The Xiangjiang River Basin may experience water shortages induced by climate change. Annual water resources of the Xiangjiang River Basin over the period from 2021 to 2050 are projected to decrease by 2.76% on average within the range from-7.81% to 7.40%. It is essential to consider the potential impact of climate change on water resources in future planning for sustainable utilization of water resources. 相似文献
157.
本文介绍了一个微机上运行的注塑模CAD系统,此系统主要解决了四个难点,浇注系统设计,冷却系统分析,型腔,型芯的曲面造型设计,装配图和零件工作图的设计绘制,经厂家实际运用证明,该系统使用方便,结果正确,能提高设计效率,降低生产成本。 相似文献
158.
159.
Modelling trees according to desired shapes is important for many applications. Despite numerous methods having been proposed in tree modelling, it is still a non‐trivial task and challenging. In this paper, we present a new variational computing approach for generating realistic trees in specific shapes. Instead of directly modelling trees from symbolic rules, we formulate the tree modelling as an optimization process, in which a variational cost function is iteratively minimized. This cost function measures the difference between the guidance shape and the target tree crown. In addition, to faithfully capture the branch structure of trees, several botanical factors, including the minimum total branches volume and spatial branches patterns, are considered in the optimization to guide the tree modelling process. We demonstrate that our approach is applicable to generate trees with different shapes, from interactive design and complex polygonal meshes. 相似文献
160.
用金属有机化合物制备铁电薄膜:工艺及进展 总被引:2,自引:0,他引:2
本文概述了以金属有机化合物为原料制备铁电薄膜的工艺过程、工艺特点及最新研究进展,着重介绍了金属有机物化学气相溶积(MOCVD),金属有机物热分解(MOD)以及溶胶-凝胶(Sol-Gel)三种制备技术在铁电薄膜制备领域中的应用。 相似文献