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991.
The Influence of Carbon Nitride Nanosheets Doping on the Crystalline Formation of MIL‐88B(Fe) and the Photocatalytic Activities 下载免费PDF全文
Zhen‐Dong Lei Yuan‐Cheng Xue Wen‐Qian Chen Lin Li Wen‐Hui Qiu Yong Zhang Liang Tang 《Small (Weinheim an der Bergstrasse, Germany)》2018,14(35)
In this research, bulk graphitic carbon nitride (g‐C3N4) is exfoliated and transferred to the carbon nitride nanosheets (CNNSs), which are then coupled with MIL‐88B(Fe) to form the hybrid. From the results of the powder X‐ray diffraction, scanning electronic microscopy and thermogravimetric analysis, it is found that the doping of CNNSs on the surface of MIL‐88(Fe) could maintain the basic structure of MIL‐88B(Fe), and the smaller dimension of CNNSs might influence the crystallization process of metal‐organic frameworks (MOFs) compared to bulk g‐C3N4. Besides, the effects of the CNNSs incorporation on photocatalysis are also investigated. Through the photoluminescence spectra, electrochemical measurements, and photocatalytic experiments, the hybrid containing 6% CNNSs is certified to possess the highest catalytic activity to degrade methylene blue and reduce Cr(VI) under visible light. The improvement of the photocatalytic performance can be attributed to the matched energy level which favors the formation of the heterojunctions. Besides, it promotes the charge migration such that the contact between MOFs and CNNSs is more intimate, which can be inferred from the electronic microscopy images. Finally, a possible photocatalytic mechanism is put forward by the relative calculation and the employment of the scavengers to trap the active species. 相似文献
992.
Yiru Wang Tinghui Yin Zhenwei Su Chen Qiu Yong Wang Rongqin Zheng Meiwan Chen Xintao Shuai 《Nano Research》2018,11(7):3710-3721
Although gas-filled microbubbles with high echogenicity are widely applied inclinical ultrasonography, the micron scale particle size impedes their use in the treatment of solid tumors,which are accessible to objects less than several hundred nanometers. We herein propose an unusual approach involving apH-induced core–shell micelle-to-vesicle transition to prepare ultrasound-sensitive polymeric nanospheres (polymersomes in structure) possessing multiple features, including nanosize, monodispersity, and incorporation of a phase-transitional imaging agent into the aqueous lumen. These features are not achievable via the conventional double-emulsion method for polymersome preparation. The nanospheres were constructed based on a novel triblock copolymer with dual pH sensitivity. The liquid-to-gas phase transition of the imaging agent induced by external low-frequency ultrasound may destroy the nanospheres for a rapid drug release, with simultaneous tissue-penetrating drug delivery inside a tumor. These effects may provide new opportunities for the development of an effective cancer therapy with few adverse effects. 相似文献
993.
Botao Liu Kowsalya Vellingiri Sang-Hee Jo Pawan Kumar Yong Sik Ok Ki-Hyun Kim 《Nano Research》2018,11(9):4441-4467
Advances in metal-organic frameworks (MOFs) resulted in significant contributions to diverse applications such as carbon capture, gas storage, heat transformation and separation along with emerging applications toward catalysis, medical imaging, drug delivery, and sensing. The unique in situ and ex situ structural features of MOFs can be tailored by conceptual selection of the organic (e.g., ligand) and inorganic (e.g., metal) components. Here, we provide a comprehensive review on the synthesis and characterization of MOFs, particularly with respect to controlling their size and morphology. A better understanding of the specific size and morphological parameters of MOFs will help initiate a new era for their real-world applications. Most importantly, this assessment will help develop novel synthesis methods for MOFs and their hybrid/porous materials counterparts with considerably improved properties in targeted applications. 相似文献
994.
随着电力、电气设备的日益复杂化,对于其安全性能也有了更高的要求,数字兆欧表作为测量绝缘阻值的重要工具,已在工业领域中广泛应用;为了满足测量精度以及兆欧表的可靠性,通过基于S3C2440的嵌入式平台,提出了一种基于数字兆欧表的自动切换档位的实现方案,以达到更加精确的测量;此方案通过判断采集到的电压值选择相应的采样电阻来实现,并结合硬件平台和软件设计,分别介绍了驱动程序和应用程序的编写与测试,并很好地应用到了实际电路中;经测试,能够达到预期的效果,测量精度高,测量误差控制在±2%。 相似文献
995.
Shijie Hu Xiaoyu Li Jiayu Bai Hang Lei Weizhong Qian Sunqiang Hu Cong Zhang Akpatsa Samuel Kofi Qian Qiu Yong Zhou Shan Yang 《计算机、材料和连续体(英文)》2023,74(2):2803-2815
When the Transformer proposed by Google in 2017, it was first used for machine translation tasks and achieved the state of the art at that time. Although the current neural machine translation model can generate high quality translation results, there are still mistranslations and omissions in the translation of key information of long sentences. On the other hand, the most important part in traditional translation tasks is the translation of key information. In the translation results, as long as the key information is translated accurately and completely, even if other parts of the results are translated incorrect, the final translation results’ quality can still be guaranteed. In order to solve the problem of mistranslation and missed translation effectively, and improve the accuracy and completeness of long sentence translation in machine translation, this paper proposes a key information fused neural machine translation model based on Transformer. The model proposed in this paper extracts the keywords of the source language text separately as the input of the encoder. After the same encoding as the source language text, it is fused with the output of the source language text encoded by the encoder, then the key information is processed and input into the decoder. With incorporating keyword information from the source language sentence, the model’s performance in the task of translating long sentences is very reliable. In order to verify the effectiveness of the method of fusion of key information proposed in this paper, a series of experiments were carried out on the verification set. The experimental results show that the Bilingual Evaluation Understudy (BLEU) score of the model proposed in this paper on the Workshop on Machine Translation (WMT) 2017 test dataset is higher than the BLEU score of Transformer proposed by Google on the WMT2017 test dataset. The experimental results show the advantages of the model proposed in this paper. 相似文献
996.
Chenhui Zhang Chen Liu Junwei Zhang Youyou Yuan Yan Wen Yan Li Dongxing Zheng Qiang Zhang Zhipeng Hou Gen Yin Kai Liu Yong Peng Xi-Xiang Zhang 《Advanced materials (Deerfield Beach, Fla.)》2023,35(1):2205967
Room-temperature magnetic skyrmion materials exhibiting robust topological Hall effect (THE) are crucial for novel nano-spintronic devices. However, such skyrmion-hosting materials are rare in nature. In this study, a self-intercalated transition metal dichalcogenide Cr1+xTe2 with a layered crystal structure that hosts room-temperature skyrmions and exhibits large THE is reported. By tuning the self-intercalate concentration, a monotonic control of Curie temperature from 169 to 333 K and a magnetic anisotropy transition from out-of-plane to the in-plane configuration are achieved. Based on the intercalation engineering, room-temperature skyrmions are successfully created in Cr1.53Te2 with a Curie temperature of 295 K and a relatively weak perpendicular magnetic anisotropy. Remarkably, a skyrmion-induced topological Hall resistivity as large as ≈106 nΩ cm is observed at 290 K. Moreover, a sign reversal of THE is also found at low temperatures, which can be ascribed to other topological spin textures having an opposite topological charge to that of the skyrmions. Therefore, chromium telluride can be a new paradigm of the skyrmion material family with promising prospects for future device applications. 相似文献
997.
根据CD级柴油机的模拟实验与台架试验的基础数据,用人工神经网络的反向传播(BP)方法,对两者的关系进行了研究,给出了人工神经网络的学习速率为0.2,动量因子为0.9,对人工神经网络的拓扑结构也进行了研究,得到了合适的5-7-2拓扑结构及各节点间的权重系数。探讨了用模拟实验数据预测台架试验结果的可能性,通过检验,证明了用人工神经网络方法建立的模型能准确预报柴油机油的台架试验结果。 相似文献
998.
动态优化调度走向实用的策略与段落全局优化 总被引:1,自引:1,他引:0
本文在总结动态优化调度在实际系统中应用经验的基础上,提出了动态优化调度走向实用的策略及以段落一局优化算动态化调度的方法,该策略可以较地贯彻电力系统运行“安全,优质,经济”的原则,段落全局优化方法则可以一次性处理各种负荷紧段落,包括单调升降段落及以往方法只有通过反向导引才能够处理的陡升连续等类的段落,具有计算时间短,节省内存等特点,为动态优化调度在电力系统中的进一步实用化打下了坚实的基础。 相似文献
999.
An efficient microfluidic sorter: implementation of double meandering micro striplines for magnetic particles switching 总被引:1,自引:1,他引:0
Tian Fook Kong Huan Shin E Hendrik Santoso Sugiarto Hwi Fen Liew Xinghua Wang Wen Siang Lew Nam-Trung Nguyen Yong Chen 《Microfluidics and nanofluidics》2011,10(5):1069-1078
The ability to trap, manipulate, and separate magnetic beads has become one of the key requirements in realizing an integrated
magnetic lab-on-chip biosensing system. In this article, we present the design and fabrication of an integrated magneto-fluidic
device for sorting magnetic particles with a sorting efficiency of up to 95%. The actuation and manipulation of magnetic beads
are realized using microfabricated square meandering current-carrying micro striplines. The current is alternated between
two neighboring micro striplines to switch the magnetic beads to either one of the two outlets. We performed a series of parametric
study to investigate the effect of applied current, flow rate, and switching frequency on the sorting efficiency. Experimental
results reveal that the sorting efficiency is proportional to the square of current applied to the stripline, and decreases
with increasing buffer flow rate and switching frequency. Such phenomena agree well with our theoretical analysis and simulation
result. The fastest switching rate, which is limited by the microchannel geometry and bead velocity, is 2 Hz. 相似文献
1000.
Soon-Yong Park Sung-In Choi Jaekyoung Moon Jun Kim Yong Woon Park 《International Journal of Control, Automation and Systems》2011,9(5):875-887
A computer vision technique to identify the location of an outdoor unmanned ground vehicle (UGV) is presented. The proposed
technique is based on hybrid 3D registration of 360 degree laser range data to a digital surface model (DSM). Range frames
obtained from 48 laser detectors are aligned with the reference coordinate system of the DSM. Three novel approaches are proposed
for accurate and fast 3D registration of range data and the DSM. First, a two-step hybrid 3D registration technique is proposed.
A pair-wise registration step of two consecutive range frames is followed by a refinement step using a layered DSM. Second,
a fast projection-based pair-wise registration is proposed by employing rasterized 360 degree range frames. Third, a high
elevation DSM is divided into several elevation layers and correspondence search is done near the vehicle’s current elevation.
This reduces the number of matching outliers and facilitates fast localization. Experimental results show that the proposed
approaches yield better performance in 3D localization compared to conventional 3D registration techniques. Error analysis
on five outdoor paths is presented with respect to ground truth. 相似文献