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991.
Highly Efficient Overall Water Splitting Through Optimization of Preparation and Operation Conditions of Layered Perovskite Photocatalysts 总被引:1,自引:0,他引:1
Jindo Kim Dong Won Hwang Hyun Gyu Kim Sang Won Bae Jae Sung Lee Wei Li Se Hyuk Oh 《Topics in Catalysis》2005,35(3-4):295-303
The layered perovskite materials were found to give the high photocatalytic activity in water splitting reaction under UV
irradiation, where the electronic structure of perovskite slab constructing the layered structure (the total cation valency)
was the most crucial factor to the high photocatalytic activity. Both the excessive cation valency and the layered structure
were required for active photocatalysts, while the slab thickness of layered perovskites had an insignificant effect on water-splitting
activity. In order to identify key variables that affected photocatalytic activity and to optimize the performance of (110)
layered perovskite, La2Ti2O7 was modified by various methods. The optimum amount of loaded nickel had a great effect and the amount depended on the surface
area of the perovskite phase. When an alkaline-earth element such as Ba, Sr, and Ca was doped on La2Ti2O7, the photocatalytic activity was enhanced markedly. Introduction of an alkaline hydroxide into the reaction system as an
external additive enhanced the activity further showing extremely high quantum yields close to 50%. 相似文献
992.
薛泷辉 《水动力学研究与进展(A辑)》2017,(2):228-236
该文针对感潮河段魁岐排涝二站?型复杂流道的不利冲刷问题,通过建立整体水工模型,研究城市异形排涝通道消能防冲新技术,提出导流坎、消力坎和消力墩联合消能防冲技术,探索其在宽幅水位变化、多工程交替运行及通航情况下的适应能力,并给出水力设计方法。研究表明,联合消能工对复杂工况适应良好,能有效解决异形排涝通道的消能防冲问题。 相似文献
993.
针对向家坝地面电站,采用三维有限元法分析比较蜗壳不同埋设方式下的流道及其外围混凝土结构的静力特性,为蜗壳埋设方式的选择提供依据。研究表明:直埋方案所需配筋最多,不经济,且可能产生贯穿性裂缝;垫层方案应力普遍较小,垫层沿水流向敷设至蜗壳45°断面的组合方案仅局部区域有较大拉应力。推荐采用垫层埋设方式或垫层敷设至蜗壳45°断面的组合埋设方式,但同时应采取有效工程措施避免局部产生贯穿性裂缝。 相似文献
994.
995.
Permeability characteristics of carbonated concrete considering capillary pore structure 总被引:3,自引:0,他引:3
During carbonation process, the calcium phases present in cement are attacked by CO2 and converted into CaCO3 and the permeability of concrete is changing due to the change in porosity. The rate of carbonation depends upon porosity and moisture content of the concrete. Especially in underground reinforced concrete structures, the interior portion of concrete surface may be exposed to carbonation and the exterior portion of concrete surface exposed to wet soil or underground water. As carbonation proceeds from outer surface into internal portion of concrete, microstructure is also changed continuously from outer surface into internal portion of concrete. Even the deteriorations in the structures due to the carbonation have been reported more, research on permeability characteristics of concrete considering carbonation and micro-structural information is very scarce.In this study, the permeability coefficient in carbonated concrete is derived by applying a capillary pore structure formation model in carbonated cement mortar and assuming that aggregates do not affect carbonation process in early-aged concrete as a function of porosity. The permeability obtained from the micro-level modeling for carbonated concrete is verified with the results of accelerated carbonation test and water penetration test in cement mortar. 相似文献
996.
997.
本文引入基于马赫-曾德(Mech-Zehnder)干涉原理的光纤传感检测系统,成功地进行了FRP混凝土结构的应变和振动检测.本文为光纤传感器应用于复合材料,并向工程结构的力学性能测试提供了新的技术装置,也为智能结构的研究奠定了技术基础. 相似文献
998.
Peter?S.?Piispanen Marcus?Persson Per?Claesson Torbj?rn?NorinEmail author 《Journal of surfactants and detergents》2004,7(2):147-159
Several novel and some previously known, mostly sugar-based, surfactants have been synthesized and some of their surface properties
have been characterized and compared with those of commercial nonylphenol ethoxylates. The surfactant solubility in water,
ethanol, and dodecane was studied. The properties of these compounds as emulsification agents in systems composed of the surfactant
with water/isopropyl myristate, water/rapeseed oil, and water/dodecane are presented. The aqueous solubility of the surfactants
follows the general trend expected from their hydrophilic-lipophilic balance according to Griffin (HLBG), but it is also clear
that the nature of the headgroup and the structure of the nonpolar part affect the solubility in a manner not aptured in the
standard HLBG concept. An ester or amine group as the connecting unit between the hydrophile and the hydrophobe produces a
more water-soluble surfactant than the corresponding amide derivative. Some effective emulsifiers were found. For instance,
the surfactants with a dehydroabietic nonpolar group appear to be promosing emulsifiers. Most sugar-based surfactants were
able to form macroemulsions of up to around 2 wt/vol% of oil. The stability of many of these amulsions was very high, extending
for months. 相似文献
999.
V. P. Samsonov 《Combustion, Explosion, and Shock Waves》2003,39(2):126-129
The papers deals with formation of vortex structures during combustion of a fuel gas–air mixture injected vertically down through a hole in a flat plate. It has been established that the shape, position, and number of vortex cells are determined by the flow rate and composition of the fuel mixture. It is shown that as the flow rate increases from the minimum critical value for which a vortex structure arises, the number of vortex cells decreases from five or six to one. A further increase in the gas flow rate leads to transition to turbulence of the combustion product flow. The presence of a vortex structure increases the critical Reynolds number at which the flow becomes turbulent. Reverse transition to the structure with an increased number of vortex cells occurs with a delay in the gas flow rate (gas discharge hysteresis). Variation in flow rate is accompanied by bifurcation of the number of vortex cells. 相似文献
1000.
Polymeric materials are being developed with renewable resources to promote industrial progress with environmentally friendly technologies. For this reason, polyurethane samples were prepared with 4,4′‐diphenylmethane diisocyanate (NCO/OH = 1), eucalyptus tar pitch (biopitch), castor oil as a polyol, and dibutyltin dilaurate as a catalyst. These materials were reinforced with different contents of short sisal fibers (0, 2.5, 5.0, 7.5, and 10.0%) and were prepared by resin‐transfer molding. The composites were characterized by IR absorption spectroscopy, thermal analysis (thermogravimetry and differential scanning calorimetry), impact resistance, scanning electron microscopy, and water absorption resistance. These materials showed hydrophobic characteristics, despite the addition of sisal fibers. © 2003 Wiley Periodicals, Inc. J Appl Polym Sci 89: 3797–3802, 2003 相似文献