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61.
《International Journal of Hydrogen Energy》2021,46(75):37333-37339
Water electrolysis is an efficient approach for high-purity hydrogen production. However, the anodic sluggish oxygen evolution reaction (OER) always needs high overpotential and thus brings about superfluous electricity cost of water electrolysis. Therefore, exploiting highly efficient OER electrocatalysts with small overpotential especially at high current density will undoubtedly boost the development of industrial water electrolysis. Herein, we used a simple hydrothermal method to prepare a novel FeOOH–CoS nanocomposite on nickel foam (NF). The as-prepared FeOOH–CoS/NF catalyst displays an excellent OER performance with extremely low overpotentials of 306 and 329 mV at 500 and 1000 mA cm−2 in 1.0 M KOH, respectively. In addition, the FeOOH–CoS/NF catalyst can maintain excellent catalytic stability for more than 50 h, and the OER catalytic activity shows almost no attenuation no matter after 1000 repeated CV cycles or 50 h of stability test. The high catalytic activity and stability have exceeded most non-noble metal electrocatalysts reported in literature, which makes the FeOOH–CoS/NF composite catalyst have promising applications in the industrial water electrolysis. 相似文献
62.
《Journal of the European Ceramic Society》2020,40(8):3348-3353
Large transduction coefficient () is difficult to obtain in piezoelectric ceramics because these two parameters show opposite trends with compositional modifications. Herein, the Pb(Zr0.53Ti0.47)O3 ceramic powders were calcinated under different temperatures (A:830 °C, B:860 °C, and C:890 °C), and then mixed together according to different weight ratios (1A:1B:1C, 1A:2B:1C, 1A:2B:3C and 3A:2B:1C) for ceramics preparation. Both d33 and g33 are improved successfully, and the transduction coefficient with the weight ratio of 1A:2B:3C reaches up to 17,500 × 10−15 m2/N, which is 60 % higher than that with the powders calcinated under 830 °C, and at least twice those of commercial PZT-4, PZT-5A and PZT-8 ceramics. The improved transduction coefficient is owing to the enhanced piezoelectric constant and spontaneous polarization resulted from the increased grain size, relative density and the fraction of tetragonal phase. These results indicate that this is a simple but effective way to tailor the transduction coefficient in piezoelectric ceramics. 相似文献
63.
Many models of spoken word recognition posit the existence of lexical and sublexical representations, with excitatory and inhibitory mechanisms used to affect the activation levels of such representations. Bottom-up evidence provides excitatory input, and inhibition from phonetically similar representations leads to lexical competition. In such a system, long words should produce stronger lexical activation than short words, for 2 reasons: Long words provide more bottom-up evidence than short words, and short words are subject to greater inhibition due to the existence of more similar words. Four experiments provide evidence for this view. In addition, reaction-time-based partitioning of the data shows that long words generate greater activation that is available both earlier and for a longer time than is the case for short words. As a result, lexical influences on phoneme identification are extremely robust for long words but are quite fragile and condition-dependent for short words. Models of word recognition must consider words of all lengths to capture the true dynamics of lexical activation. (PsycINFO Database Record (c) 2010 APA, all rights reserved) 相似文献
64.
Reports an error in "Tradeoffs and Theory: The Double-Mediation Model" by Marc Scholten and Steven J. Sherman (Journal of Experimental Psychology: General, 2006 May, Vol 135[2], 237-261). This article was inadvertently printed with the incorrect title. The original title was "Tradeoffs and Conflict: The Double-Mediation Model." This title highlights the relation between tradeoffs and conflict as investigated by the authors and accounted for by their model. However, readers are asked to refer to the article by the title with which it was printed to facilitate its retrieval.. (The following abstract of the original article appeared in record 2006-06642-006.) Most theories of decision making suggest that, when options imply tradeoffs between their attributes, conflict increases as tradeoff size increases, because greater sacrifices are to be incurred in choosing one option instead of another. An alternative view is that conflict decreases as tradeoff size increases, because stronger arguments can be made for any decision. The authors propose a unified model, the double-mediation model, which combines the mediating effects of sacrifice and argumentation. Our model generally predicts an inverse U-shaped relation between tradeoff size and conflict. Results support this prediction. Also, when the decision situation increases the mediating effect of sacrifice relative to that of argumentation, the relation between tradeoff size and conflict changes in an upward direction; conversely, when the decision situation increases the mediating effect of argumentation relative to that of sacrifice, the relation changes in a downward direction. Results support these predictions as well. Commonalities and differences between our model and other formulations are discussed. (PsycINFO Database Record (c) 2010 APA, all rights reserved) 相似文献
65.
SO4^2-/ZrO2固体超强酸的制备及其催化合成ETBE的研究 总被引:5,自引:2,他引:3
采用沉淀一浸渍法制备了负载型SO4^2-/ZrO2固体超强酸催化剂,运用IR、XRD等方法表征所制备催化剂的物化性质。结果表明,所制备的催化剂具有固体超强酸催化剂的特征,酸性与焙烧温度有关,适当提高焙烧温度有利于样品酸强度的提高,但焙烧温度过高会导致脱硫;浸渍液H2SO4浓度高有利于提高催化剂的硫含量,但是浓度过高,会在催化剂上形成硫酸盐,从而降低催化剂的比表面积和酸性。采用制备的催化剂气相催化乙醇与叔丁醇合成乙基叔丁基醚反应,乙基叔丁基醚的选择性为54.71%。 相似文献
66.
67.
醇解技术在制备皮革加脂剂方面的研究进展 总被引:1,自引:0,他引:1
本文介绍了醇解反应的动力学、影响醇解反应收率的因素以及醇解反应在合成加脂剂方面的应用。 相似文献
68.
分析了长距离管输后3号喷气燃料电导率严重衰减的原因和补加抗静电剂后对3号喷气燃料电导率和水反应指标的影响。对比了成品油长距离管输和喷气燃料馏分长距离管输对3号喷气燃料电导率和水反应指标的影响,并对比了两种管输方式的优缺点,提出对3号喷气燃料的管输建议。3号喷气燃料的长距离管输,优先采用喷气燃料馏分油管输在末端加注抗静电剂的方式;需兼顾汽运时,宜采用成品油管输并在末端根据电导率衰减情况,最小量补加抗静电剂的方式,以获得较高的成功率和较好的经济效益。 相似文献
69.
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