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Angjian Wu Jianhua Yan Hao Zhang Ming Zhang Changming Du Xiaodong Li 《International Journal of Hydrogen Energy》2014
Dry methane reforming (DMR) via rotating gliding arc (RGA) discharge, co-driven by a magnetic field and tangential flow, was investigated in this study. Optical emission spectroscopy (OES) was used to characterize the major active species (energetic electrons, radicals, ions, atoms and excited molecules) in the DMR chemical process. The influence of the operational conditions (applied voltage and CH4/CO2 ratio) on the basic spectroscopic parameters (electron excitation temperature, electron density and rotational temperature) was determined by spectroscopic methods. The rotational and electron excitation temperatures were approximately 1100–1200 K and 1.1–1.7 eV, respectively, indicating the non-thermal equilibrium characteristics of the RGA discharge. The electron density was approximately 5–20 × 1021 m−3 by fitting the line shape of Hα at 656 nm. The conversions of the reactants (CH4 and CO2) and the selectivities of the products (H2, CO and C2 hydrocarbon) were analyzed using a gas chromatograph (GC) under different energy inputs or feed gas proportions. The structure and morphology of carbon black produced during the chemical process was characterized by high-resolution transmission electron microscopy (HRTEM) and Raman spectroscopy, indicating the properties of electrical conductivity and high absorption capacity that can be useful for potential application. 相似文献
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The fundamental algorithm of light beam propagation in high power laser system is investigated and the corresponding computational codes are given. It is shown that the number of modulation ring due to the diffraction is related to the size of the pinhole in spatial filter (in terms of the times of diffraction limitation, i. e. TDL) and the Fresnel number of the laser system; for the complex laser system with multi-spatial filters and free space, the system can be investigated by the reciprocal rule of operators. 相似文献