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针铁矿是分布广泛、储量丰富的铁氧化物,其主要成分为α-羟基氧化铁(α-FeOOH)。为了探究针铁矿在催化H2O2烟气脱硝反应中的性能,本文通过沉淀-水解法制备了α-FeOOH,并在自行搭建的实验台上开展了α-FeOOH催化H2O2的低温烟气脱硝实验研究,深入分析了H2O2流量、H2O2浓度、汽化温度、反应温度和共存气体浓度等工况参数对脱硝性能的影响。采用离子色谱(IC)分析了单独脱硝反应和同时脱硫脱硝反应后的含氧酸成分,结合各项表征分析技术考察了催化剂反应前后的理化特性和稳定性。实验结果显示,随着汽化温度和反应温度的升高,NO的脱除效率先增加后降低;增加H2O2浓度对脱硝效率有明显的促进作用。当汽化温度为140℃、反应温度为160℃时,以2.5mL/h注入10mol/L的H2O2脱硝效率达到80%。当SO2浓度为1000μL/L时,脱硝效率提高至86.4%。离子色谱分析结果显示,单独脱硝反应和同时脱硫脱硝反应后含氧酸产物为HNO3和H2SO4。反应前后催化剂的表征结果显示,α-FeOOH在脱硝反应后依然具有良好的稳定性,显示出针铁矿在低温烟气脱硝工艺中的潜在应用前景。 相似文献
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为研究含齿形裂隙岩石在单轴压缩下的破坏特征及强度特性,制作了含不同裂隙倾角和起伏角的齿形裂隙类岩石材料试件,并采用岩石力学伺服试验机进行单轴压缩试验。试验结果表明:(1)试件主要产生拉伸、剪切和拉剪复合裂纹,且根据裂纹的扩展路径可划分为A型(拉伸破坏)、B型(剪切破坏)、C型(复合破坏)3种破坏模式,裂隙倾角对试件最终破坏模式影响显著;(2)当裂隙倾角较小时,试件应力—应变曲线为多峰曲线,随着裂隙倾角的增大,曲线呈单峰形式,表现为延性减弱,脆性增强,而裂隙倾角相同但起伏角不同的试件应力—应变曲线大致相同;(3)当裂隙起伏角相同时,试件当量峰值强度随裂隙倾角的增大呈先减小后增大的规律,且裂隙起伏角对试件当量峰值强度的影响小于裂隙倾角。 相似文献
15.
Tatsuro Tanaka Yoshifumi Maeda Shinji Yamamoto Toru Iwao 《Electrical Engineering in Japan》2019,207(1):15-23
The arc welding has been used in various welding methods because it is inexpensive and high in strength after welding. However, it is a problem that accidents such as collapse of the bridge occur because of the welding defects. The welding of low cost and high productivity is required without the welding defects. The pulsed TIG welding is inexpensive and capable of high‐quality welding. The electromagnetic force contributing to penetration changes because the transient response of arc temperature and iron vapor generated from anode occurs. However, the analysis of pulsed TIG welding with metal vapor has been elucidated only metal vapor concentration near anode with transient phenomenon and heat flux. Thus, the theoretical elucidation of penetration depth with control factor has not been researched. In this paper, the contribution of metal vapor mass at the periphery part of pulsed arc to the electromagnetic force in the weld pool is elucidated. As a result, the iron vapor mass at periphery part decreased with increasing the frequency. The iron vapor was stagnated at axial center within one cycle. The electromagnetic force to the penetration depth direction in weld pool increased at axial center. Therefore, the metal vapor mass at periphery part plays an important role for the electromagnetic force increment at axial center. 相似文献
16.
《International Journal of Hydrogen Energy》2019,44(2):587-593
A solid-state photoelectrochemical (SSPEC) cell is an attractive approach for solar water splitting, especially when it comes to monolithic device design. In a SSPEC cell the electrodes distance is minimized, while the use of polymer-based membranes alleviates the need for liquid electrolytes, and at the same time they can separate the anode from the cathode. In this work, we have made and tested, firstly, a SSPEC cell with a Pt/C electrocatalyst as the cathode electrode, under purely gaseous conditions. The anode was supplied with air of 80% relative humidity (RH) and the cathode with argon. Secondly, we replaced the Pt/C cathode with a photocathode consisting of 2D photocatalytic g-C3N4, which was placed in tandem with the photoanode (tandem-SSPEC). The tandem configuration showed a three-fold enhancement in the obtained photovoltage and a steady-state photocurrent density. The mechanism of operation is discussed in view of recent advances in surface proton conduction in absorbed water layers. The presented SSPEC cell is based on earth-abundant materials and provides a way towards systems of artificial photosynthesis, especially for areas where water sources are scarce and electrical grid infrastructure is limited or nonexistent. The only requirements to make hydrogen are humidity and sunlight. 相似文献
17.
《Contact lens & anterior eye》2021,44(6):101388
PurposeTo investigate the relationship between the real contact lens imprint into the conjunctival tissue, observed by optical coherence tomography (OCT) and conjunctival staining and contact lens wearing comfort.Methods17 participants (mean age = 26.6 SD ± 3.6 years; 7 females) were fitted with three different contact lenses base curves of the same silicone hydrogel custom lens type (Visell 50; Hecht Contactlinsen, Au, Germany) in a randomised order. One lens was optimally fitted according to the manufacturer's recommendation, one fitted 0.4 mm flatter and one fitted 0.4 mm steeper. After 4 h of lens wear the contact lens edge in the area of the conjunctiva was imaged nasally and temporally using OCT (Optovue iVue SD-OCT). To correct the artefact due to optical distortion with OCT, the imprint of all worn lenses was measured on a glass plate afterwards. Conjunctival staining in the limbal region after 4 h of lens wear was classified using the CCLRU Grading Scale. Comfort scoring was based on visual analog scales from 0 (very poor) to 100 (excellent).ResultsThe mean conjunctival imprint of all contact lens edges was 32.0 ± 8.1 μm before and 7.3 ± 6.5 μm after distortion correction of the OCT images. The distortion corrected conjunctival imprint with the 0.4 mm steeper lens (11.5 ± 6.2 μm) was statistically significantly greater compared to the optimally fitted lens (6.5 ± 5.9 μm) (One-way ANOVA followed Tukey-test; p = 0.017) and greater compared to the 0.4 mm flatter lens (3.9 ± 5.3 μm) (p < 0.001). There was no statistically significant difference between the optimally fitted lens and the 0.4 mm flatter lens (p = 0.209). The nasally measured imprint (11.4 ± 9.0 μm) was significantly greater than the temporally measured (3.3 ± 7.6 μm) (p < 0.001). There was no statistically significant correlation between the amount of conjunctival imprint and the graded conjunctival staining (p = 0.346) or the wearer’s comfort (p = 0.735).ConclusionsContact lens edges imaged by OCT exhibited displacement artefacts. The observed conjunctival imprints are a combination of real conjunctival compression and artefacts. A deeper imprint of the contact lens into the conjunctiva caused by a steeper base curve was not related to clinically significant staining or changes in comfort after 4 h of lens wear. The observed differences between nasal and temporal imprint are likely to be caused by variations of conjunctival thickness and the shape of the underlying sclera. 相似文献
18.
This paper proposes a thermoelectric-assisted vapor compression cycle (TVCC) for applications in air-source heat pump systems which could enhance the heating capacity of the system. Performances of TVCC are calculated and then compared with that of basic vapor compression cycle (BVCC). The simulation results show that when coefficients of performance (COPs) of the two cycles are almost equal, the TVCC under maximum COP condition of the thermoelectric modules still performs better than BVCC by 13.0% in heating capacity through selecting the appropriate intermediate temperature. In addition, the TVCC can also achieve an improvement of 16.4%–21.7% in both the heating COP and capacity when compared with the BVCC with an assistant electric heater that is provided with the equivalent power input of thermoelectric heat exchanger. Thus, the TVCC could be beneficial to the applications in small heat pumps if there is always need for auxiliary electric heat. 相似文献
19.
Mauro D. Santos Ivonne Delgadillo Jorge A. Saraiva 《International Journal of Food Science & Technology》2020,55(3):1171-1179
Hyperbaric storage (HS) was evaluated as a new food preservation methodology at room temperature (RT) for beef and pork meat, both minced and in pieces, and compared to refrigeration (RF) storage. The meat samples were stored at 50, 75 and 100 MPa and variable RT up to 60 days. HS at 75 and 100 MPa could not only inhibit microbial growth but also inactivate microorganisms. Regarding physicochemical analyses, an overall equal to better pH maintenance in HS samples was achieved, and similar colour differences between HS and RF were observed. Generally, similarities in moisture content and drip loss between HS (mostly 75 and 100 MPa) and RF were detected (tendency for lower values in the former and higher values in the latter for the higher pressure level). Protein solubility revealed a decrease of sarcoplasmic protein values during storage with a pressure level dependency in some samples. 相似文献
20.
针对在高太阳辐射地区,柴油车驾驶室内使用车载空调会增加车辆发动机的耗油量、降低柴油车经济效益的问题,搭建了一套由发动机尾气余热驱动的吸附式车载空调系统。系统由填充有氯化钙/氯化锰/硫化膨胀石墨复合吸附剂的吸附床、蒸发器、冷凝器、储液罐和阀门组成,使用氨作为制冷剂,利用车辆在行驶时接触到的自然风为吸附床冷却,在发动机尾气余热的驱动下,为驾驶室内提供连续的制冷效果。结合仿真和实验测试,对所设计系统的制冷性能进行了分析,仿真结果表明,系统最优循环时间为45 min,系统的理论平均制冷功率可达3.5 kW以上,系统COP处于0.2~0.25之间。实验结果表明,在230℃的尾气温度条件下,系统能产生3 kW的平均制冷量。在40℃环境温度条件下,系统在蒸发器进出口处的平均温差为6.5℃,平均制冷量为3.2 kW。 相似文献