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11.
Liu Chu Jiajia Shi Yue Yu Eduardo Souza De Cursi 《International journal of molecular sciences》2021,22(9)
With the distinguished properties in electronics, thermal conductivity, optical transparence and mechanics, graphene has a powerful potential in nanosensors, nano-resonators, supercapacitors, batteries, etc. The resonant frequency of graphene is an important factor in its application and working environment. However, the random dispersed porosities in graphene evidently change the lattice structure and destroy the integrity and geometrical periodicity. This paper focuses on the effects of random porosities in resonant frequencies of graphene. Monte Carlo simulation is applied to propagate the porosities in the finite element model of pristine graphene. The statistical results and probability density distribution of porous graphene with atomic vacancy defects are computed based on the Monte Carlo finite element model. The results of porous graphene with atomic vacancy defects are compared and discussed with the results of graphene with bond vacancy defects. The enhancement effects of atomic vacancy defects are confirmed in porous graphene. The influences of atomic vacancy defects on displacement and rotation vector sums of porous graphene are more concentrated in local places. 相似文献
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Due to advances in medical research, more and more diseases can be cured nowadays, which largely increases the need for an easy-to-use software in calculating sample size of clinical trials with cure fractions. Current available sample size software, such as PROC POWER in SAS, Survival Analysis module in PASS, powerSurvEpi package in R are all based on the standard proportional hazards (PH) model which is not appropriate to design a clinical trial with cure fractions. Instead of the standard PH model, the PH mixture cure model is an important tool in handling the survival data with possible cure fractions. However, there are no tools available that can help design a trial with cure fractions. Therefore, we develop an R package NPHMC to determine the sample size needed for such study design. 相似文献
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合成氨装置脱碳工段采用NHD脱碳工艺,由于脱碳后的脱碳气中CO2含量偏高,造成H 2损耗较大,为此采用ZUPAC系列双向金属折峰式波纹填料和新型槽盘式液体分布器对脱碳塔进行改造。改造后,脱碳气中CO2体积分数从2.0%降至1.6%,年可增加经济效益1000万元左右。 相似文献
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针对粒子群算法对初始种群敏感和易陷入局部最优解等问题,提出了佳点集理论结合多种群多策略协同进化算法改进的粒子群算法(IMPMSPSO).首先采用佳点集理论生成佳点作为初始种群,使种群分布更均匀而在一定程度上减弱其对位置的敏感性;然后利用协同进化算法,先将种群随机分成若干子种群,各子种群随机选择一种改进的进化策略并行计算,并进行最优位置的共享.经过测试,IMPMSPSO在计算精度和收敛速度上均优于其他算法.最后利用IMPMSPSO优化模糊神经网络初始权值和阈值构造分类预测模型,对雾霾污染等级进行分类预测.结果表明,与其他分类模型相比,该模型在各等级上的准确率均有提高. 相似文献
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聚乙烯薄膜的氟化研究 总被引:1,自引:1,他引:0
为了改善聚乙烯薄膜材料表面的反应性能,对聚乙烯薄膜进行了氟化改性研究。在恒定的温度下,通过改变氟化反应的压强参数值,制备了氟化薄膜改性样品,并采用红外光谱和扫描电镜等对样品进行分析,以探究聚乙烯薄膜氟化的较佳条件。研究结果表明,在氟化温度为60℃,且以氮气为保护气的条件下,进行130,220 mPa压力下的递进氟化,能较好地实现聚乙烯薄膜表面的羧化和氟化改性,提高聚乙烯薄膜表面的反应能力。 相似文献
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Jiajia Yan Teng Zhang Haizheng Tao Hongbing Zhan Yuanzheng Yue 《Journal of the American Ceramic Society》2021,104(6):2560-2570
We study the structure, crystallization, and performances of the sealing glasses with the composition (mol.%) of 12Al2O3·8B2O3·40SiO2·40RO (R = Mg, Ca, Sr) for solid oxide fuel cells (SOFCs) before and after isothermal treatment at 700°C, which is within the operation temperature range (600-800°C) of SOFCs. The crystallization behavior has been investigated by differential scanning calorimetry and X-ray diffraction under both dynamic and isothermal conditions. The structural evolution is probed using the Raman and nuclear magnetic resonance spectroscopies. The performances of the sealing glasses are characterized in terms of the coefficient of thermal expansion, the crystallization-induced stress at glass–steel interface. We find that strong crystallization occurs at the operation temperature (700°C) far below the crystallization onset temperature measured by DSC. The structure origin of this anomalous crystallization is discussed in terms of structural heterogeneity of the three studied glasses. We determine the residual stress at the interface between the Ca-containing glass and the steel after isothermal treatment at 700°C for 48 h, but this stress does not lead to falling off the glass layer from the steel. This indicates that this glass is a good candidate to be applied in SOFCs. 相似文献
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Experimental investigation on evaporation interface temperature and evaporation rate of water in its own vapor at low pressures 下载免费PDF全文
Evaporative phase transitions are widely present in industrial production and daily life such as thin film processes and crystal growth. The evaporation of the liquid layer and the thermocapillary convection affect each other and restrict each other, making the energy transfer mechanism of the evaporation interface very complicated. To understand the evaporation characteristics of water in its low-pressure pure vapor environment, a series of experimental studies were carried out on the temperature distributions and evaporating rate of water evaporation in the annular pool. The cylinder temperature of the annular liquid pool is controlled between 3℃ and 15℃, and the evaporation environment pressure ranges from 394 Pa to 1467 Pa, when the temperature measurement starts, the depth of water is 10 mm. The results show that the temperature of the vapor side on the liquid-vapor interface is higher than that of the liquid side and there is an obvious temperature jump across the vapor-liquid interface. With the decrease of the pressure ratio, the evaporation rate increases, and the interface temperature jump is enlarged. Meanwhile, with the increase of the distance from the cylinder, the local evaporation rate decreases, thus, the temperature jump decreases. At the same pressure ratio, as the cylinder temperature increases, the heat flux from vapor side decreases, the temperature jump decreases at all measurement points. Within the experimental controlled parameters, the maximum temperature jump obtained in the measurements is 2.56℃. Due to the coupling effect of evaporation cooling and thermocapillary convection, there is a uniform temperature layer with a thickness of about 2 mm under the evaporation interface. The thickness of the uniform temperature layer near the cylinder is always larger than that in the middle of the evaporation interface. In the uniform temperature layer, the thermocapillary convection induced by radial temperature gradient transfers heat from the cylinder to the liquid-vapor interface to compensate for the latent heat of evaporation. Below the uniform temperature layer, the temperature rises rapidly due to heat conduction and buoyancy convection. 相似文献
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