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L. Birry P. Mehta F. Jaouen J.-P. Dodelet S.R. Guiot B. Tartakovsky 《Electrochimica acta》2011,(3):1505
Catalysts for the oxygen reduction reaction (ORR) in a microbial fuel cell (MFC) were prepared by the impregnation on carbon black of FeII acetate (FeAc), Cl–FeIII tetramethoxyphenyl porphyrin (ClFeTMPP), and FeII phthalocyanine (FePc). These materials were subsequently pyrolyzed at a high temperature. The ORR activity of all Fe-based catalysts was measured at pH 7 with a rotating disk electrode (RDE) and their performance for electricity production was then verified in a continuous flow MFC. Catalysts prepared with FeAc and pyrolyzed in NH3 showed poor activity in RDE tests as well as a poor performance in a MFC. The ORR activity and fuel cell performance for catalysts prepared with ClFeTMPP and FePc and pyrolyzed in Ar were significantly higher and comparable for both precursors. The iron loading was optimized for FePc-based catalysts. With a constant catalyst load of 2 mg cm−2 in a MFC, the highest power output (550–590 mW/m2) was observed when the Fe content was 0.5–0.8 wt%, corresponding to only 0.01–016 mg Fe/cm2. A similar power output was observed using a Pt-based carbon cloth cathode containing 0.5 mg Pt/cm2. Long-term stability of the Fe-based cathode (0.5 wt% Fe) was confirmed over 20 days of MFC testing. 相似文献
13.
柔性结构与周围流体的耦合作用机制广泛应用于仿生机器人、水下航行器、精密仪器及生命医疗等领域。具有驱动变形大、防水性好且柔韧性好的压电宏纤维(Macro fiber composite,MFC)致动器是水下柔性结构变形控制的首选。建立MFC内部致动弯矩和水动力载荷共同作用下柔性结构的流固耦合动力学模型。对粘贴MFC致动器的柔性结构特征截面进行计算流体动力学(Computational fluid dynamics,CFD)分析,得到不同振动特征频率下柔性结构周围流场、压力分布及所受水动力载荷,分别拟合得到MFC致动柔性结构水动力函数的实部和虚部表达式。结果表明柔性结构水动力载荷的附加质量和阻尼效应都随着振动频率的增加而减小。在等振动特征频率下,MFC致动梁结构水动力函数的实部大于匀质等截面梁的实部;在高振动频率下其水动力函数虚部同样大于匀质等截面梁。试验测试了MFC致动柔性结构的水下振动特性,试验所得MFC激励下柔性结构末端稳定振动的幅频特性和相频特性与建立的耦合动力模型相吻合,证实了所建立MFC致动柔性结构的水动力函数及流固耦合振动模型的有效性。 相似文献
14.
利用机构学的方法对双曲肘合模机构进行了运动分析,并确立了合模行程、各肘杆尺寸及最大启模角等参数间的关联关系。通过使用Pro/E二次开发技术,讨论了应用Pro/toolkit进行菜单开发及零件参数化实现的方法;以MFC对话框设计技术和VC++建立了双曲肘合模机构参数驱动自动生成技术,开发出了与Pro/E 4.0系统集成的合模机构零件参数化设计系统。 相似文献
15.
Hajie-Banoo Khalili Davod Mohebbi-Kalhori Mahdi Shafiee Afarani 《International Journal of Hydrogen Energy》2017,42(12):8233-8241
This study aimed to evaluate the influence of commercially available unglazed wall ceramic (UGWC) and unglazed floor ceramic (UGFC) separators with different thickness and porosity on the performance of dual-chamber microbial fuel cells (MFCs). These MFCs were operated under continuous condition using domestic wastewater. The UGWC-based MFC produced higher maximum power density (321 mW/m2 with a thickness of 9 mm) than UGFC-based MFC (106.89 mW/m2 with a thickness of 3 mm) due to lower internal resistance. Power generation using both types of separators was lower than that of obtained using the Nafion 117 membrane as control (602 mW/m2). The maximum average coulombic efficiencies (CE) of the UGWC-based MFCs (with thickness levels of 6 and 9 mm) were 58% and 68%, respectively, which was more than that of UGFC-based MFCs and also control MFC (53%). Voltammetric analysis revealed that the maximum peak current of 6 mA was obtained for UGWC-based MFC which was in the order of control MFC (5.9 mA). The UGWC separators exhibited smaller ohmic and diffusion resistances of 57, 65 and 87 Ω in MFCs at the thickness levels of 3, 6 and 9 mm, respectively, compared to the UGFC separators with that of 164.27 and 366.23 Ω in MFCs at the thickness levels of 3 and 6 mm, respectively. UGWC separators because of their low production cost, high mechanical strength and increased output power density of the MFC proved to be a suitable alternative to replace with a costly polymeric membrane such as Nafion 117. 相似文献
16.
Irene Merino Jimenez John Greenman Ioannis Ieropoulos 《International Journal of Hydrogen Energy》2017,42(3):1791-1799
The use of ceramics as low cost membrane materials for Microbial Fuel Cells (MFCs) has gained increasing interest, due to improved performance levels in terms of power and catholyte production. The catholyte production in ceramic MFCs can be attributed to a combination of water or hydrogen peroxide formation from the oxygen reduction reaction in the cathode, water diffusion and electroosmotic drag through the ion exchange membrane. This study aims to evaluate, for the first time, the effect of ceramic wall/membrane thickness, in terms of power, as well as catholyte production from MFCs using urine as a feedstock. Cylindrical MFCs were assembled with fine fire clay of different thicknesses (2.5, 5 and 10 mm) as structural and membrane materials. The power generated increased when the membrane thickness decreased, reaching 2.1 ± 0.19 mW per single MFC (2.5 mm), which was 50% higher than that from the MFCs with the thickest membrane (10 mm). The amount of catholyte collected also decreased with the wall thickness, whereas the pH increased. Evidence shows that the catholyte composition varies with the wall thickness of the ceramic membrane. The possibility of producing different quality of catholyte from urine opens a new field of study in water reuse and resource recovery for practical implementation. 相似文献
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在VC+ +6.0平台上利用Windows Media Player控件实现了在程序中播放一段视频和音频的功能.测试结果证明该方法简单易行,极大缩短了程序的开发时间. 相似文献
19.
S. SrikanthT. Pavani P.N. SarmaS. Venkata Mohan 《International Journal of Hydrogen Energy》2011,36(3):2271-2280
Comprehensive study was performed to understand the synergistic interaction between the biocatalyst and anode in terms of electron discharge (ED) pattern and microbial growth by varying electrode (bio-anode) materials viz., graphite, aluminum, brass, copper, nickel and stainless steel. Experiments were performed in bio-electrochemical cell consisting of three electrodes (bio-anode as working electrode, carbon rod as counter electrode and Ag/AgCl(S) as reference electrode) employing anaerobic mixed culture as anodic biocatalyst. Voltammetric and chronoamperometric analysis were used to enumerate the ED and redox reactions. Presence of higher microbial population and dominance of Gram positive bacteria with higher ED supported graphite function as a good bio-anode material. Nickel and stainless steel showed higher ED after graphite associated with dominance of Gram positive bacterial population. Although higher ED was noticed with brass, metal oxidation and decrement in ED with time doesn’t support its function as bio-anode. In spite of higher ED than nickel and stainless steel, aluminum and copper showed significant metal oxidation leading to change in both physical and electrochemical properties along with dominant growth of Gram negative bacteria. This study gives a comprehensive idea on biocatalyst interaction with anode in extracellular electron transfer which is important in improving the anode performance. Juxtaposing the results, it can be deduced that the outcome of the present study can be extended to all bio-electrochemical systems including microbial fuel cell (MFC). 相似文献
20.
Shravankumar B. Kerur 《热应力杂志》2013,36(12):1255-1282
A finite element formulation for geometrically non-linear bending behavior of smart structures integrated with piezoelectric fiber-reinforced composite (AFC/MFC) layer acting as distributed actuator is presented in this article. The formulation of this hygro-thermo-electro-mechanical coupled problem is based on the first-order shear deformation theory (FSDT) and the von Kármán type geometric non-linearity. Resulting non-linear algebraic governing equations are linearized by Newton–Raphson iterative method. A developed finite element formulation is initially solved for validation and comparison with existing results. A wide variety of numerical examples considering cross-ply laminated substrates subjected to combined mechanical, hygrothermal and electrical loads are presented. The effect of piezoelectric fiber orientation in an actuator to counteract non-linear deflections is analyzed. 相似文献