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11.
We have studied the effect of size mismatch on the structural, magnetic and electrical properties of Pr0.67Ba0.33MnO3 (PBMO) and Pr0.67Sr0.33MnO3 (PSMO) perovskites with considerable difference in their variance σ2 values. Samples were prepared by ceramic route at 1200 °C. Morphological study, microstructure and chemical composition were examined by scanning electron microscopy, EDX analyses and Rietveld structure refinement. Both compounds exhibit single orthorhombic Pnma crystalline phase and with strongly connected and larger grains for PSMO than for PBMO that gives a beginning of single crystal growth in PSMO case. PBMO with higher variance exhibits distinct intrinsic (due to grains) and extrinsic (due to grain boundaries) transitions in the resistivity behaviour, and with higher transition temperatures than those usually reported in the literature. Extrinsic effects, however, are not observed in the lower σ2 PSMO sample. Both compounds exhibit Curie temperature (TC) values significantly higher than those reported in the literature, and with higher TC for PSMO due to its larger bandwidth W. The experimental paramagnetic effective moment for PSMO is very close to the theoretical one, whereas there is a significant difference between these moments for PBMO sample, probably due to the considerable size mismatch effect between Pr and Ba, and to the ferromagnetic correlations in the paramagnetic state. Ferromagnetic-metallic regime in the two compounds seems to emanate from the electron-(phonon, magnon) scattering processes with a larger effect for PBMO than that for PSMO, due to the prominent role of the grain boundary in PBMO. Above paramagnetic-insulating transition temperature the data were well fitted by both variable range hopping (VRH) and small polaron hopping (SPH) models giving higher density state, and lower activation energy and Mott temperature T0 for PSMO than those for PBMO, essentially due to their considerable difference in their variance values.  相似文献   
12.
The nanosized effects of short-range multimagnon excitation behavior and short-circuit diffusion in NiO nanowalls synthesized using the Ni grid thermal treatment method were observed. The energy dispersive spectroscopy mapping technique was used to characterize the growth mechanism, and confocal Raman scattering was used to probe the antiferromagnetic exchange energy J2 between next-nearest-neighboring Ni ions in NiO nanowalls at various growth temperatures below the Neel temperature. This study shows that short spin correlation leads to an exponential dependence of the growth temperatures and the existence of nickel vacancies during the magnon excitation. Four-magnon configurations were determined from the scattering factor, revealing a lowest state and monotonic change with the growth temperature.PACS: 75.47.Lx; 61.82.Rx; 75.50.Tt; 74.25.nd; 72.10.Di  相似文献   
13.
Microparticles and micrograin ceramics show features distinct from the usual-sized polycrystalline materials. Amorphous state material combined with microparticle size for Pb(Zr0.51 Ti0.49)O3 mimics the dielectric behaviour of crystalline ferroelectricity in ABO3 compounds. Fine-grained Y3Fe5O12 (yig) synthesized by pressure sintering ofyig microparticles exhibit spinwave relaxation due to transit time across grain diameter. Applying microemulsion techniques for microparticle synthesis,γ-Fe2O3 has been synthesized. The phase stability fractionγ-Fe2O3/α-Fe2O3 is found to be a function of particle size. At very small sizesγ-Fe2O3 becomes amorphous, leading to interesting Mössbauer studies.  相似文献   
14.
详细介绍小样品热导率测量装置,用该装置测定了沪产99.9%纯钆的热导率。发现在230K附近轧热导率反常,趋向极小。证实了除电子以外,磁机制对钆电导和热导有较大贡献。  相似文献   
15.
在二维绝缘铁磁系统基础上建立了一个磁振子-声子相互作用模型.利用Matsubara格林函数方法研究了磁振子-声子相互作用下的三角绝缘铁磁体的磁振子谱,计算了布里渊区的主要对称点线上的磁振子色散曲线.发现在布里渊区边界区域磁振子谱的软化和磁振子谱线增宽最明显.比较了纵向声子与横向声子对磁振子谱的软化与磁振子谱线增宽的影响,也讨论了各项参数的变化对磁振子谱的软化与磁振子谱线增宽的影响.  相似文献   
16.
The laser-field induced magnon amplification in a magnetic semiconductor quantum well under an external magnetic field was discussed, it is shown that when the laser frequency is near to the electron cyclotron frequency, no matter how weaker the laser field is, the magnon amplification always occurs. In case of fixed laser frequency, the optical absorption of magnons obeys the definite selection rule to the laser field strength. The rate of change of magnon occupation is calculated, and the amplification condition is given.  相似文献   
17.
为了研究腔磁杂化系统中磁振子分布的量子统计性质,构建了一种单量子源,并利用全量子理论在含有声子模的杂化腔磁系统中研究了磁振子阻塞的操控方案及其物理机制.通过求解主方程得到了磁振子的等时二阶关联函数和平均磁子数,并分析了腔模之间的耦合对磁振子反聚束的影响.数值模拟结果表明,增加隧穿耦合、腔与机械模的耦合、腔与磁子模的耦合可有效增强磁振子的反聚束效应.本方案可为在实验中实现单磁子源提供参考.  相似文献   
18.
The magnon contribution to the specific heat of ferromagnetic terbium is evaluated and the results are compared with the measurements from 90 K down to absolute zero.  相似文献   
19.
As new information carriers, antiferromagnetic magnons have great potential in the fields of spintronics and quantum information. However, the strong exchange interaction between sublattice spins in conventional antiferromagnets results in their frequencies up to the terahertz (THz) range, hindering further exploration of related applications and physics. Recently, emerging van der Waals A-type antiferromagnets with the weak exchange interaction may bring about a change. In this study, it demonstrates two distinct tunable ultrastrong magnonmagnon couplings in the gigahertz (GHz) band using this type of antiferromagnet, CrPS4, with a maximum normalized coupling strength (η) of 0.31. It establishes orthorhombic and monoclinic models for theoretical analyses, unambiguously showing that the ultrastrong coupling strength is caused by unique magnetocrystalline anisotropy rather than exchange enhancement. Furthermore, for the first time, it observes a continuous switching process of sublattice magnon chirality arising from the orthorhombic nature of anisotropy. These findings not only deepen the understanding of antiferromagnetic spin dynamics but also offer a powerful platform for building magnonic quantum systems and chirality-based spintronics.  相似文献   
20.
利用非厄米腔磁学系统研究了相干耦合和耗散耦合对极化子量子性质的影响,并采用主方程数值模拟的方法研究了哈密顿本征能谱的特点.结果表明:在耗散耦合的作用下,本征能谱显示出不同于相干耦合的现象,即实部表现出能级吸引,虚部发生能级排斥.当系统中同时存在相干耦合和耗散耦合时,相干耦合对极化子的演化起主导作用,而耗散耦合仍会影响本征能谱的分布,并且不同相位下的本征能谱分布呈周期性变化.该研究结果可为腔磁学系统的量子信息处理提供理论参考.  相似文献   
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