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Sergey Tkachev Miguel Monteiro João Santos Ernesto Placidi Mohamed Ben Hassine Pedro Marques Paulo Ferreira Pedro Alpuim Andrea Capasso 《Advanced functional materials》2021,31(33):2103287
Graphene-based materials have attracted significant attention in many technological fields, but scaling up graphene-based technologies still faces substantial challenges. High-throughput top-down methods generally require hazardous, toxic, and high-boiling-point solvents. Here, an efficient and inexpensive strategy is proposed to produce graphene dispersions by liquid-phase exfoliation (LPE) through a combination of shear-mixing (SM) and tip sonication (TS) techniques, yielding highly concentrated graphene inks compatible with spray coating. The quality of graphene flakes (e.g., lateral size and thickness) and their concentration in the dispersions are compared using different spectroscopic and microscopy techniques. Several approaches (individual SM and TS, and their combination) are tested in three solvents (N-methyl-2-pyrrolidone, dimethylformamide, and cyrene). Interestingly, the combination of SM and TS in cyrene yields high-quality graphene dispersions, overcoming the environmental issues linked to the other two solvents. Starting from the cyrene dispersion, a graphene-based ink is prepared to spray-coat flexible electrodes and assemble a touch screen prototype. The electrodes feature a low sheet resistance (290 Ω □−1) and high optical transmittance (78%), which provide the prototype with a high signal-to-noise ratio (14 dB) and multi-touch functionality (up to four simultaneous touches). These results illustrate a potential pathway toward the integration of LPE-graphene in commercial flexible electronics. 相似文献
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针对货运车辆在配送调度过程中产生大量碳排放的问题,建立模型将多种影响碳排放量的因素协同优化。模型中考虑了不同载重量的异质车队,两个节点之间有多条道路的柔性路径,以及车辆重量随卸货而减少的动态负载等因素,以碳排放量、行驶时间和行驶路程为优化目标,并加入了节点需求时间窗、根据速度变化划分路段、交接和卸货时间的约束。提出了一种混合蚁群算法,利用蚁群算法信息素强度更新方式保持群体记忆性,利用粒子群算法的快速收敛特性增加计算效率。通过随机数值算例的仿真优化与对比分析,验证了算法和模型的有效性。 相似文献
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为解决传统纤维表面拉曼增强(SERS)基底所存在的稳定性差、操作不便等问题。介绍了柔性SERS基底的优势,总结了目前各类纤维基SERS基底的研究进展及其在痕量检测领域的应用,简述了电磁增强和化学增强2种表面增强拉曼现象的基本原理。综述了纤维纸基SERS、织物基SERS、散纤维及纳米纤维膜SERS基底的制备方法及其应用,并着重介绍了织物基SERS材料的研究现状及其在在线检测应用方面的挑战与机遇。基于织物基SERS材料高度灵敏及灵活检测的特点,展望了其作为可穿戴传感器件用于即时检测和周身环境监测的前景,为拓展智能纺织品的应用领域开辟了新的思路。 相似文献
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为了实现太赫兹信号的可调谐滤波,设计了一种基于柔性材料的太赫兹可调谐滤波器。通过扭曲特氟龙(Teflon)波导形成环型谐振器,实现了160~200 GHz频段的带阻滤波功能。改变谐振腔长可实现自由频谱范围(FSR)和滤波频点的调谐,实验测试了自由频谱范围在1.9 GHz和2.8 GHz间切换以及相应的滤波特性。研究表明,谐振腔长一定时,改变弯曲半径可实现滤波阻带抑制度的调节,柔性材料太赫兹环型谐振器可用于可调谐滤波,且具有较高的自由度。 相似文献
7.
A Smart Flexible Solid State Photovoltaic Device with Interfacial Cooling Recovery Feature through Thermoreversible Polymer Gel Electrolyte 下载免费PDF全文
Quasi‐solid‐state dye‐sensitized solar cells (DSSCs) fabricated with lightweight flexible substrates have a great potential in wearable electronic devices for in situ powering. However, the poor lifespan of these DSSCs limits their practical application. Strong mechanical stresses involved in practical applications cause breakage of the electrode/electrolyte interface in the DSSCs greatly affecting their performance and lifetime. Here, a mechanically robust, low‐cost, long‐lasting, and environment‐friendly quasi‐solid‐state DSSC using a smart thermoreversible water‐based polymer gel electrolyte with self‐healing characteristics at a low temperature (below 0 °C) is demonstrated. When the performance of the flexible DSSC is hindered by strong mechanical stresses (i.e., from multiple bending/twisting/shrinking actions), a simple cooling treatment can regenerate the electrode/electrolyte interface and recover the performance close to the initial level. A performance recovery as high as 94% is proven possible even after 300 cycles of 90° bending. To the best of our knowledge, this is the first aqueous DSSC device with self‐healing behavior, using a smart thermoreversible polymer gel electrolyte, which provides a new perspective in flexible wearable solid‐state photovoltaic devices. 相似文献
8.
针对高面板坝后期变形导致的面板破坏问题,采用大型室内试验测定了大石峡筑坝料流变力学特性,重点研究了后期流变效应对坝体、防渗体应力变形的影响。评估了各期面板浇筑前坝体沉降速率,复核了面板浇筑前预沉降时间的合理性。研究结果表明,该坝各期面板浇筑前设置的预沉降期可将坝顶沉降率控制在5mm/月以内。大坝蓄水运行后面板应力,尤其是轴向应力,较初次蓄水增加明显,存在挤压破坏的风险。论证了在面板受压区设置柔性缝的面板应力改善措施,结果表明该工程措施对削减面板轴向压应力效果明显。总体上,250m级的特高砂砾石面板坝坝体和防渗体应力变形能满足安全控制要求,通过合理的工程措施可保证大坝施工与运行安全。 相似文献
9.
针对牛奶厂人工搅拌不均匀、不充分的问题,应用TRIZ(theory of inventive problem solving)理论对整个储奶罐系统进行创新性设计。通过分析组件间相互作用,得出人工使用铁耙搅拌牛奶作用不足的结论;针对搅拌装置在工作时因高度不同而弯曲程度不同,运用物理矛盾分析,结合时间分离中的发明原理——动态特性,设计出一种电机驱动式、可伸缩的柔性机构。运用solidworks三维软件搭建具体的打耙机构模型,通过试验验证柔性臂工作的可行性。试验结果表明,该柔性臂能完成压缩、伸长、弯曲、扭转等姿态,可实现较大范围的搅拌。 相似文献
10.
Bayar Mohammed Rayya Hassan Nahla Alaswadko 《International Journal of Pavement Engineering》2018,19(12):1096-1110
The purpose of this study is to assess the effect of traffic data source (estimated vs. actual) on predicted progression rates of roughness and rutting for heavy-duty flexible pavements of rural freeways. Progression rates are predicted using calibrated HDM-4 models. The assessment is performed in terms of variations in maintenance intervention timing associated with the variations in progression rates. Time series pavement condition data (covering 3–5 years) have been collected for 7 sections of rural freeways for use in calibrating HDM-4 deterioration models. They range in length from 10 to 60.8 km and cover different traffic volumes, climate zones and subgrade soil types. For these sections, estimated annual average daily traffic (AADT), growth factors and assumed loading have been extracted from relevant database. Only six segments of these sections have Weigh-in-Motion (WIM) sites so relevant actual AADT, growth factors and axle load distributions have been extracted from WIM reports. The results of running the calibrated HDM-4 deterioration models using different traffic data show that actual traffic data from WIM sites result in higher rates of deterioration to that of estimated data for four sites, resulting in earlier intervention timing and higher present value agency cost. The other two sites have lower rates with actual data due to lower traffic loading than estimated. 相似文献