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1.
Novel organic dyes containing N-bridged oligothiophene coplanar cores for dye-sensitized solar cells
Three novel organic dyes adopting fully-fused coplanar heteroarene as the donor moieties end-capped with two cyanoacrylic acids as acceptors and anchoring groups have been synthesized, characterized, and used as the sensitizers for dye-sensitized solar cells (DSSCs). The photophysical and electrochemical properties of the novel dyes and the characteristics of the DSSCs based on the novel organic dyes were investigated. The incorporation of the coplanar cores with electron-donating N-bridges are beneficial for the better intramolecular charge transfer (ICT), giving these new dyes good light-harvesting capability. The LUMO energy levels of these coplanar heteroacene-based dyes are sufficiently high for the efficient electron injection to TiO2 upon photo-excitation, while the suitable HOMOs allow the regeneration of oxidized dyes with the electrolyte redox (I−/I3−). The structural features of the coplanar cores (penta vs. hexa heteroarene) as well as the alkyl substitutions play crucial roles in governing the physical properties and device performance. Among these three novel organic sensitizers, the EHTt dye composed of a fully fused hexa-arene core and less bulky N-alkyl groups caused the DSSC to show the best photovoltaic performance with an open-circuit voltage (VOC) of 0.58 V, a short-circuit photocurrent density (JSC) of 13.72 mA/cm2, and a fill factor (FF) of 0.69, yielding an overall power conversion efficiency (PCE) of 5.52% under AM 1.5G solar irradiation. 相似文献
2.
A double optimal projection method that involves projections for intra-cluster and inter-cluster dimensionality reduction are proposed for video fingerprinting. The video is initially set as a graph with frames as its vertices in a high-dimensional space. A similarity measure that can compute the weights of the edges is then proposed. Subsequently, the video frames are partitioned into different clusters based on the graph model. Double optimal projection is used to explore the optimal mapping points in a low-dimensional space to reduce the video dimensions. The statistics and geometrical fingerprints are generated to determine whether a query video is copied from one of the videos in the database. During matching, the video can be roughly matched by utilizing the statistics fingerprint. Further matching is thereafter performed in the corresponding group using geometrical fingerprints. Experimental results show the good performance of the proposed video fingerprinting method in robustness and discrimination. 相似文献
3.
基于扩展分形和CFAR特征融合的SAR图像目标识别 总被引:3,自引:0,他引:3
研究了多信息融合技术在SAR图像目标识别中的应用。将扩展分形特征(Extended Fractal)与双参数恒虚警特征(Double Parameter CFAR)形成的多信息进行融合处理。运用Dempster-Shafer证据理论,在决策层对SAR图像中的像素进行识别分类。实验结果表明通过融合对像素分类的准确性明显好于单特征的检测结果,减少了虚警概率,提高了系统的识别能力。 相似文献
4.
一种基于三次样条函数求离子浓度的自动算法 总被引:1,自引:0,他引:1
本文提出了一种用三次样条函数模拟双次标准加入法测量方程,直接求解离子浓度的自动算法。比较了三咱不同边界条件下用要池数计算离子浓度的结果。造出节点区间两极端点的二阶导数为零时的三次样条函数为最佳模拟函数。并讨论了该方法在实际分析中误差的来源及消除办法。经对一系列文献数据的验算对比,表明本法完全可代替传统的迭代法和查图法,且能方便地设置在智能化的电位分析系统中。 相似文献
5.
On the basis of the experimental data, we show that the difference between the macroscopic and microscopic fatigue crack growth rates in the second section of the kinetic diagram of fatigue fracture is caused by the effect of crack closure within the limits of its existence. We establish the relationships between the macroscopic and microscopic fatigue crack growth rates and the structure of the material in the second section of the diagram for various values of the load ratio with regard for the effect of crack closure and propose a procedure of examination of the fracture processes in structural materials based on the analysis of microscopic and macroscopic fatigue crack growth rates. 相似文献
6.
针对单轴传动滚切式双边剪生产过程中出现的薄钢板经双边剪剪后出现“错牙”及“飞边”的问题,从多个方面入手对薄钢板出现“错牙”及“飞边”的原因进行了分析对比,提出了相应的解决方案,对今后滚切式双边剪的设计、制造及安装调试有借鉴和参考价值。 相似文献
7.
中国火灾与社会经济因素的关系 总被引:22,自引:2,他引:20
对中国的火灾统计数据与社会经济数据之间的关系进行了研究,发现中国火灾与社会经济因素的关系和国外相反:中国的火灾形势在经济越发达的地方越严重,并且随着经济的发展更趋严重。讨论了火灾与经济水平及教育水平的关系,提出了火灾和经济的更为全面的关系,即随着经济的发展,火灾形势是先严重后趋缓和。根据所讨论的结果对中国未来一段时期的火灾情况做出了一些预测。 相似文献
8.
We apply a bifurcation-theoretic approach to the standard Moore–Greitzer compressor model in effort to understand a curious phenomenon. When one forces the actuator to respond sluggishly to commanded inputs, performance of the controller improves dramatically. We show that the behavior can be explained via Hopf–Hopf interactions of surge and rotating stall. Also, we argue that there is a broad class of controllers which possess the general dynamic features responsible for the surprising effectiveness of sluggish actuators. 相似文献
9.
CHENSheng-ping LUKe-cheng LIYi-gang LIJia-fang ZHUJian-ping FENGMing LIJing 《半导体光子学与技术》2004,10(2):122-126
The effects of the variations in fiber length, fiber mirror reflectance on efficiency and output power are experimentally investigated for erbium-doped double pass backward superfluorescent fiber sources (SFSs). The influence of fiber length on mean wavelength stability (MWS) has also been demonstrated. By incorporating a short section of un-pumped erbium-doped fiber (EDF) at the output port, the pump power dependent on MWS becomes independent of pumped EDF length. This is a novel phenomenon that hasn‘t been reported up to now,and should be helpful to SFS fabrication and theory analysis. By using a fiber Michelson interferometer as spectrum slicing component,a multi-wavelength fiber source (MWFS) with ~20 channels (from 1542nm to 1559nm) is got. The MWFS has a channel spacing of ~0. 8 nm which satisfies ITUstandard. The intensity fluctuation among channels is less than 0.5dB,and the extinction ratio of all channels is above 14dB. This kind of MWFS should be useful to wavelength division multiplexing systems. 相似文献
10.
Hitsman Brian; Borrelli Belinda; McChargue Dennis E.; Spring Bonnie; Niaura Raymond 《Canadian Metallurgical Quarterly》2003,71(4):657
The authors conducted a meta-analysis of published studies to (a) evaluate the premise that a history of major depression is associated with failure to quit smoking and (b) identify factors that moderate the relationship between history of depression and cessation outcome. Fifteen studies met the selection requirements and were coded for various study methodology and treatment characteristics. DSTAT was used to calculate individual study effect sizes, determine the mean effect size across studies. and test for moderator effects. No differences in either short-term (≤ 3 months) or long-term abstinence rates (≥ 6 months) were observed between smokers positive versus negative for history of depression. Lifetime history of major depression does not appear to be an independent risk factor for cessation failure in smoking cessation treatment. (PsycINFO Database Record (c) 2010 APA, all rights reserved) 相似文献