全文获取类型
收费全文 | 4267篇 |
免费 | 500篇 |
国内免费 | 391篇 |
专业分类
电工技术 | 914篇 |
综合类 | 323篇 |
化学工业 | 438篇 |
金属工艺 | 115篇 |
机械仪表 | 303篇 |
建筑科学 | 98篇 |
矿业工程 | 59篇 |
能源动力 | 209篇 |
轻工业 | 77篇 |
水利工程 | 94篇 |
石油天然气 | 47篇 |
武器工业 | 28篇 |
无线电 | 1422篇 |
一般工业技术 | 544篇 |
冶金工业 | 33篇 |
原子能技术 | 39篇 |
自动化技术 | 415篇 |
出版年
2024年 | 10篇 |
2023年 | 66篇 |
2022年 | 86篇 |
2021年 | 153篇 |
2020年 | 130篇 |
2019年 | 136篇 |
2018年 | 112篇 |
2017年 | 162篇 |
2016年 | 151篇 |
2015年 | 189篇 |
2014年 | 245篇 |
2013年 | 243篇 |
2012年 | 320篇 |
2011年 | 373篇 |
2010年 | 285篇 |
2009年 | 289篇 |
2008年 | 288篇 |
2007年 | 296篇 |
2006年 | 253篇 |
2005年 | 222篇 |
2004年 | 194篇 |
2003年 | 150篇 |
2002年 | 138篇 |
2001年 | 96篇 |
2000年 | 100篇 |
1999年 | 77篇 |
1998年 | 56篇 |
1997年 | 52篇 |
1996年 | 57篇 |
1995年 | 33篇 |
1994年 | 40篇 |
1993年 | 34篇 |
1992年 | 18篇 |
1991年 | 22篇 |
1990年 | 23篇 |
1989年 | 14篇 |
1988年 | 11篇 |
1987年 | 5篇 |
1986年 | 3篇 |
1985年 | 3篇 |
1984年 | 8篇 |
1983年 | 1篇 |
1982年 | 5篇 |
1981年 | 1篇 |
1980年 | 3篇 |
1979年 | 1篇 |
1978年 | 1篇 |
1977年 | 1篇 |
1975年 | 2篇 |
排序方式: 共有5158条查询结果,搜索用时 31 毫秒
1.
2.
Pengfei Liang Jie Zhu Di Wu Hui Peng Xiaolian Chao Zupei Yang 《Journal of the American Ceramic Society》2021,104(6):2702-2710
Due to the demand of miniaturization and integration for ceramic capacitors in electronic components market, TiO2-based ceramics with colossal permittivity has become a research hotspot in recent years. In this work, we report that Ag+/Nb5+ co-doped (Ag1/4Nb3/4)xTi1−xO2 (ANTOx) ceramics with colossal permittivity over a wide frequency and temperature range were successfully prepared by a traditional solid–state method. Notably, compositions of ANTO0.005 and ANTO0.01 respectively exhibit both low dielectric loss (0.040 and 0.050 at 1 kHz), high dielectric permittivity (9.2 × 103 and 1.6 × 104 at 1 kHz), and good thermal stability, which satisfy the requirements for the temperature range of application of X9R and X8R ceramic capacitors, respectively. The origin of the dielectric behavior was attributed to five dielectric relaxation phenomena, i.e., localized carriers' hopping, electron–pinned defect–dipoles, interfacial polarization, and oxygen vacancies ionization and diffusion, as suggested by dielectric temperature spectra and valence state analysis via XPS; wherein, electron-pinned defect–dipoles and internal barrier layer capacitance are believed to be the main causes for the giant dielectric permittivity in ANTOx ceramics. 相似文献
3.
Abidur Rahman Makoto Kobayashi Kotaro Sugimoto Yuta Endo Manabu Kojima Shigenori Furukawa Takafumi Watanabe Shu Soeda Yuko Hashimoto Keiya Fujimori Hideki Chiba 《International journal of molecular sciences》2021,22(7)
Background: Within the claudin (CLDN) family, CLDN12 mRNA expression is altered in various types of cancer, but its clinicopathological relevance has yet to be established due to the absence of specific antibodies (Abs) with broad applications. Methods: We generated a monoclonal Ab (mAb) against human/mouse CLDN12 and verified its specificity. By performing immunohistochemical staining and semiquantification, we evaluated the relationship between CLDN12 expression and clinicopathological parameters in tissues from 138 cases of cervical cancer. Results: Western blot and immunohistochemical analyses revealed that the established mAb selectively recognized the CLDN12 protein. Twenty six of the 138 cases (18.8%) showed low CLDN12 expression, and the disease-specific survival (DSS) and recurrence-free survival rates were significantly decreased compared with those in the high CLDN12 expression group. We also demonstrated, via univariable and multivariable analyses, that the low CLDN12 expression represents a significant prognostic factor for the DSS of cervical cancer patients (HR 3.412, p = 0.002 and HR 2.615, p = 0.029, respectively). Conclusions: It can be concluded that a reduced CLDN12 expression predicts a poor outcome for cervical cancer. The novel anti-CLDN12 mAb could be a valuable tool to evaluate the biological relevance of the CLDN12 expression in diverse cancer types and other diseases. 相似文献
4.
《Ceramics International》2022,48(1):656-664
Formation of p-n junction was an effective method to improve the photocatalytic performance due to its built-in electric field. However, the electric field was distributed only on the interface between two semiconductors, which was insufficient in comparison to the entire material. In this work, a multilayer TiO2–CoTiO3 p-n junction was designed and fabricated by atomic layer deposition. The charge transport and photoelectrochemical properties of multilayer TiO2–CoTiO3 films of various thicknesses are thoroughly investigated. The PL and electrochemical tests demonstrate that TiO2–CoTiO3 exhibits enhanced charge separation and transport. Additionally, the extra visible light response was achieved by introduction of CoTiO3. Also, theoretical calculations indicate that the electrons prefer to immigrate from TiO2 to CoTiO3 in a multilayer TiO2–CoTiO3 structure. Benefited from the boosted light absorption and charge transfer, the multilayer TiO2–CoTiO3 composite film exhibits a significantly increased photocurrent, much higher than pure TiO2 and a single TiO2–CoO p-n junction. This multilayer p-n junction structure opens a rational and novel way for nanostructure construction in the energy conversion region. 相似文献
5.
In this paper, the resonance characteristics of aperture type frequency selective surface (FSS) is presented. A systematic investigation is carried out to design the compact FSS. The optimized structure consists of rectangular Archimedean spiral with inter-digital capacitance. Resonance characteristics is verified in both single-layer as well as the double-layer approach by embedding FSS on one side of the dielectric substrate. The performances of the dual-layer are observed by varying air-gap between two FSS layers. The structure offers satisfactory resonance (transmission and reflection) characteristics at optimum air-gap of 7 mm between two layers with the 3 dB cutoff region over a frequency range (3.66–4.66 GHz). Finally, an array of 31 × 31 FSS elements of two layers is fabricated for experimental characterization. A close agreement between simulated and measured results is observed. 相似文献
6.
Yo-Sheng Lin Kai-Siang Lan Ming-Yuan Chuang Yu-Ching Lin 《International Journal of Electronics》2018,105(6):1063-1077
This paper reports a 94 GHz CMOS voltage-controlled oscillator (VCO) using both the negative capacitance (NC) technique and series-peaking output power and phase noise (PN) enhancement technique. NC is achieved by adding two variable LC networks to the source nodes of the active circuit of the VCO. NMOSFET varicaps are adopted as the required capacitors of the LC networks. In comparison with the conventional one, the proposed active circuit substantially decreases the input capacitance (Cin) to zero or even a negative value. This leads to operation (or oscillation) frequency (OF) increase and tuning range (TR) enhancement of the VCO. The VCO dissipates 8.3 mW at 1 V supply. The measured TR of the VCO is 91~96 GHz, close to the simulated (92.1~96.7 GHz) and the calculated one (92.2~98.2 GHz). In addition, at 1 MHz offset from 95.16 GHz, the VCO attains an excellent PN of – 98.3 dBc/Hz. This leads to a figure-of-merit (FOM) of ?188.5 dBc/Hz, a remarkable result for a V- or W-band CMOS VCO. The chip size of the VCO is 0.75 × 0.42 mm2, i.e. 0.315 mm2. 相似文献
7.
关于CaCu3Ti4O12陶瓷的高介电常数机理,目前广泛接受的是非本征的内阻挡层电容模型。该模型认为在多晶中元素变价、缺陷和非化学计量比等导致的半导化晶粒被绝缘晶界层,即内阻挡层所包围。其中内阻挡层的厚度对材料的介电性能影响较大,而扫描电子显微镜(SEM)测试表明样品晶界呈稀烂的果酱状,SEM难以测量晶界区域绝缘内阻挡层厚度。本文采用正电子湮没技术表征其厚度,通过对CaCu3Ti4O12陶瓷共掺不同浓度的Al、Nb(CaCu3Ti4-xAl0.5xNb0.5xO12,x=0.2%、0.5%、5.0%)改变其晶粒和晶界的微观结构,研究CaCu3Ti4O12陶瓷高介电常数机理。正电子湮没结果显示,掺杂样品符合多普勒展宽谱S参数的变化趋势与平均寿命的变化趋势一致。x=0.5%掺杂样品的介电常数最高,其平均寿命、S参数和湮没长寿命成分均最小,阻挡层最薄。实验结果验证了描述CaCu3Ti4O12陶瓷高介电常数机理的内阻挡层电容模型的预测。 相似文献
8.
H.L. Zhu X.W. Zhao R.W. Han Q.J. DU Y.X. Qi H.N. Jiang D.W. Huang Y.X. Yang 《Journal of dairy science》2021,104(8):9263-9275
The newborn gut undergoes rapid colonization by commensal microorganisms and possible exposure to pathogens. The contribution of colostrum intake to host protection is well known; however, limited research exists on the intestinal innate immunity corresponding to colostrum intake during the passive immune transfer period in newborn ruminants. The aim of this study was to investigate the changes in bacterial community and expression of genes encoding toll-like receptors (TLR), mucins (MUC), antimicrobial peptides, and tight junctions in the jejunum of lambs that were fed colostrum during the first 24 h of life. Twenty-seven newborn lambs were used in this study, of which 18 lambs were bottle-fed pooled bovine colostrum within the first 2 h after birth to obtain an intake of approximately 8% of body weight. Lambs were slaughtered at 12 (n = 9) and 24 h (n = 9) after birth. The remaining 9 lambs without any feeding were slaughtered at 30 min after birth (0 h). Tissue and ligated segment samples from the jejunum were collected immediately after the lambs were slaughtered. The bacterial profile in the ligated jejunum segment was assessed using amplicon sequencing. The gene expression in the jejunum tissue was determined using quantitative real-time PCR. The relative abundances of Escherichia-Shigella, Lactobacillus, Lactococcus, and Streptococcus increased, whereas those of Sphingomonas, Phyllobacterium, Bradyrhizobium, and Rudaea decreased during the first 24 h of life. Expression of TLR2 and β-defensin 109-like was upregulated at 12 h after birth, but a recovery was detected at 24 h; TLR3, TLR5, LYZ, MUC1, MUC13, MUC20, and CLDN7 showed a higher expression level in samples taken at 24 h than in those taken at 0 h. In addition, expression level of CLDN1, CLDN4, and the junctional adhesion molecule-1 tended to be higher at 24 h than at 0 h after birth. Correlation analysis indicated that TLR2 expression was negatively correlated with the relative abundance of Lactobacillus and Bradyrhizobium, whereas TLR5 expression was positively correlated with the relative abundance of Escherichia-Shigella and Pelagibacterium. These results suggest that TLR, MUC, antimicrobial peptides, and CLDN act together and play an important role in intestinal defense during the passive immune transfer period. They are potentially associated with microbial colonization. The findings from this study provide novel information to elucidate the role of colostrum components in regulating the development of the intestinal mucosal immune barrier in newborn lambs during the passive immune transfer period. 相似文献
9.
A novel CdS/CaFe2O4 (CS/CFO) heterogeneous p-n junction was created by thermal deposition of CaFe2O4 nanoparticles on CdS rods. The CS/CFO hetero-structured photocatalysts exhibited increasingly efficient visible light harvesting compared to the bare CdS. The CS/CFO composites also presented higher photocurrent and slower decay of photoluminescence, suggesting a better separation of the photo-generated electrons and holes. The photocatalytic H2 evolution quantity on the optimized CS/CFO composite from water in the presence of ethanol was up to 2200 μmol after 3-h visible light illumination, which is more than twice that of the pristine CdS. The chemical interaction between CdS and CaFe2O4 was confirmed by the shifts in the XPS peaks, which made it possible for the charge carriers to transfer across the p-n junction interface. This research highlights the importance of forming an interfacial p-n heterojunction between two semiconductors for efficient charge separation and improved photocatalytic performance. 相似文献
10.
Zhongyuan Fu Xinyi Ma Bing Xia Xiaoyun Hu Jun Fan Enzhou Liu 《International Journal of Hydrogen Energy》2021,46(37):19373-19384
Schottky junction and p-n heterojunction are widely employed to enhance the charge transfer during the photocatalysis process. Herein, Cu and Cu3P co-modified TiO2 nanosheet hybrid (Cu–Cu3P/TiO2) was fabricated using an in situ hydrothermal method. The ternary composite achieved the superior H2 evolution rate of 6915.7 μmol g?1 h?1 under simulated sunlight, which was higher than that of Cu/TiO2 (4643.4 μmol g?1 h?1) and Cu3P/TiO2 (6315.8 μmol g?1 h?1) and pure TiO2 (415.7 μmol g?1 h?1). The enhanced activity can be attributed to the collaboration effect of Schottky junction and p-n heterojunction among Cu/TiO2 and Cu3P/TiO2, which can harvest the visible light, reduce the recombination of charge carriers and lower the overpotential of H2 evolution, leading to a fast H2 evolution kinetics. This work develops a feasible method for the exploration of H2 evolution photocatalyst with outstanding charge separation properties. 相似文献