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1.
The coupling of reaction and diffusion between neighboring active sites in the catalyst pore leads to the spatiotemporal fluctuation in component concentration, which is very important to catalyst performance and hence its optimal design. Molecular dynamics simulation with hard-sphere and pseudo-particle modeling has previously revealed the non-stochastic concentration fluctuation of the reactant/product near isolated active site due to such coupling, using a simple model reaction of A → B in 2D pores. The topic is further developed in this work by studying the concentration fluctuation due to such coupling between neighboring active sites in 3D pores. Two 3D pore models containing an isolated active site and two adjacent active sites were constructed, respectively. For the isolated site, the concentration fluctuation intensifies for larger pores, but the product yield decreases, and for a given pore size, the product yield reaches a peak at a certain reactant concentration. For two neighboring sites, their distance (d) is found to have little effect on the reaction, but significant to the diffusion. For the same reaction competing at both sites, larger d leads to more efficient diffusion and better overall performance. However, for sequential reactions at the two sites, higher overall performance presents at a smaller d. The results should be helpful to the catalyst design and reaction control in the relevant processes. 相似文献
2.
《International Journal of Hydrogen Energy》2022,47(59):25007-25021
Fluid sloshing usually causes serious safety issues on the dynamic stability and propellant thermal management during the powered-flight phase of launch vehicle. With the wide using of cryogenic propellants, the coupled thermo-mechanical performance during fluid sloshing becomes more prominent. In the present study, one numerical model is established to simulate fluid sloshing by using the VOF method coupled with the mesh motion treatment. The phase change occurring within the tank is considered. Both the experimental validation and mesh sensitivity analysis are made. It shows that present numerical model is acceptable. Based on the developed numerical model, the effect of different super gravity accelerations on fluid sloshing hydrodynamic characteristic is numerically researched. The fluid pressure variation, the sloshing force and sloshing moment, the interface dynamic response and the interface shape variation are investigated, respectively. It shows that the gravity acceleration has caused obvious influences on fluid sloshing characteristic. When the gravity acceleration is higher than 4g0, fluid sloshing becomes more obvious and must be paid enough attention. With some valuable conclusions obtained, the present work is of great significance for in-depth understanding of fluid sloshing mechanism. 相似文献
3.
Yixuan ZHOU Huajie WANG Yi YU Yihang CHEN Rui KE Min XU Chijie XIAO Zhanhui WANG Jiquan LI Xuru DUAN Minyou YE 《等离子体科学和技术》2021,23(7):75105-52
In this article, we present the optical design of a novel diagnostic on the HL-2 A tokamak, i.e. the20-channel edge Lyman-alpha beam emission spectroscopy, which is a promising solution for edge density turbulence research on tokamaks, as it offers the possibility of density fluctuation measurement with a 3.3 mm spatial resolution while maintains a high temporal resolution of1 μs. The optical path, including the reflective collection optics, the high-dispersion spectrometer, and the linear detector array, is carefully optimized to obtain a good image quality and a high throughput. The maximum root mean square radius of the collection optics is 64 μm.The detected photon flux is estimated to be about 10~(11) photons/s/channel. 相似文献
4.
针对现有掘进机截割头载荷特性研究方法采用单一影响因素不能全面反映截割头载荷及其波动变化规律的问题,通过分析截割头瞬时载荷,确定了纵轴式掘进机在水平截割工况下截割头载荷的主要影响因素有截割岩石特性、截割头掏槽深度、截割头吃刀深度、截割头转速和截割臂摆速。针对某纵轴式掘进机水平截割工况,采用Matlab对影响截割头载荷的多种因素进行仿真分析,得到了各向载荷及其波动随各因素的变化规律:截割头载荷随着岩壁普氏系数的增大而增加,其中横向阻力增加尤为明显,横向阻力波动程度高于其他方向载荷,且随着岩壁普氏系数的增大呈减小趋势;随着截割头掏槽深度的增加,截割头各向载荷近似呈线性增加,其中升力增加幅度最大,各向载荷波动则随着截割头掏槽深度的增大而减小;随着吃刀深度的增加,截割头载荷总体呈增大趋势,载荷波动程度则随之减小;在截割头转速一定的情况下,截割头载荷均随着截割臂摆速的增加而增大,在同一摆速下,截割头载荷随着截割头转速的减小而增大,横向阻力波动明显高于升力和推进阻力波动,横向阻力和推进阻力波动按截割头载荷规律变化,升力波动则与之相反。截割头载荷波动变化规律与截割头载荷变化规律不尽一致,有时甚至相互冲突。因此,掘进机作业过程中应合理选择截割头掏槽深度、吃刀深度等操作参数和截割头转速、截割臂摆速等运动参数,使各参数相互匹配,以减小掘进机振动,延长使用寿命。 相似文献
5.
结晶器吹氩流量对流场分布有明显影响,因此明确吹氩流量对结晶器内流场分布的影响规律对提高铸坯质量有重要意义。通过插钉法工业试验研究了吹氩流量对结晶器内流场分布的影响,并且定量分析了液位波动的变化。结果表明,随着吹氩流量的增大,流场形态从双环流逐步转变为复杂流和单环流。结晶器内流场形态从双环流转变为复杂流和单环流的过程中,水口附近速度逐渐增大,液位逐渐升高,弯月面速度分布逐渐转变为从水口流向窄面,液位波动也相应增大。因此,生产过程中应选择合适的吹氩流量,避免产生复杂流和单环流,以提高铸坯质量。 相似文献
6.
Commonly used flow rate measurement systems provide an accurate and stable output value of the quasi-stationary flow rate. In some pump types as e.g. single-blade pumps significant flow rate fluctuations may occur even in steady operation points due to rotor-stator interaction. For the analysis of the time-resolved flow rate a new measurement and evaluation method is presented based on an electromagnetic flow meter. Internal averaging of the flow meter is deactivated and the raw signal is evaluated directly with a sampling rate of 3 kHz. With ensemble-averaging in combination with an impeller position detection, interfering signals acting on the time-resolved measurement signal are filtered out. Accompanying numerical simulations of the pump flow circuit are carried out with a 1D method of characteristics and validated against well-established time-resolved pressure measurements of the pump flow. Experiment and simulation show a resembling trend of pressure as well as flow rate fluctuations over the entire operation range of the pump. Thus, by the combined utilisation of measurement and simulation technique, we assure the validity of the ensemble-averaged flow rate fluctuation results. We find that the flow rate fluctuations show a consistent phase shift to the pressure fluctuations that increases towards overload. The flow rate amplitude is an order of magnitude smaller than the amplitude of the pressure fluctuations. 相似文献
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9.
Yun Shuai Peng Zhang Xiaoyun Guo Xinyan Wang Zhengliang Huang Yao Yang Jingyuan Sun Meng Li Yan Jiang Jiong Ma Jingdai Wang Yongrong Yang 《American Institute of Chemical Engineers》2020,66(1):e16778
Three gas–liquid dispersion states including flooding, loading, and complete dispersion are observed sequentially in a jet bubbling reactor with an increase of the liquid jet velocity at the nozzle outlet (uj). The gas–liquid dispersion states are identified through the slope (k) of the curve of fluctuation distribution index (FI) versus uj as follows: (a) under the flooding, k = 0; (b) under the loading, k > 0; (c) under the complete dispersion, k < 0. In particular, the uj at the transition points from flooding to loading and from loading to complete dispersion are referred to flooding jet velocity (ujf, the transition point between k = 0 and k > 0) and complete dispersion jet velocity (ujcd, the transition point from k > 0 to k < 0), respectively. The average relative deviations of the uj at the transition points obtained through the acoustic emission measurement and visual observation are less than 5%. 相似文献
10.
《International Journal of Hydrogen Energy》2022,47(91):38682-38689
A body-centered cubic equiatomic TiZrTaNbAl multi-principal element alloy (MPEA) with elemental fluctuations was investigated to further understand the relationship between the microstructure and hydrogen distribution. In this study, a composition dependence of the hydrogen distribution was observed in the TiZrTaNbAl MPEA. An inhomogeneous electron density distribution of the MPEA was revealed by advanced differential phase-contrast scanning electron microscopy (DPC-STEM) for the first time. The results showed that the electron density has a significant effect on the hydrogen distribution in TiZrTaNbAl MPEAs. This work provides new insight into the design of materials with high hydrogen storage capacity and high hydrogen embrittlement resistance. 相似文献