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1.
Lindsey Yue Alicia Bayon Wojciech Lipiński 《American Institute of Chemical Engineers》2021,67(8):e17267
The effects of particle size and carbon dioxide concentration on chemical conversion in engineered spherical particles undergoing calcium oxide looping are investigated. Particles are thermochemically cycled in a furnace under different carbon dioxide concentrations. Changes in composition due to chemical reactions are measured using thermogravimetric analysis. Gas composition at the furnace exit is evaluated with mass spectroscopy. A numerical model of thermal transport phenomena developed previously is adapted to match the physical system investigated in the present study. The model is used to elucidate effects of reacting medium characteristics on particle temperature and reaction extent. Experimental and numerical results show that (1) an increase in particle size results in a decrease in carbonation extent, and (2) the carbonation step consists of fast and slow reaction regimes. The reaction rates in the fast and slow carbonation regimes increase with increasing carbon dioxide concentration. The effect of carbon dioxide concentration and the distinction between the fast and slow regimes become more pronounced with increasing particle size. 相似文献
2.
Yangyang Xu Zhaofu Ding Haibin Zhu Yijun Zhang Stephan Knopf Pu Xiao Jacques Lalevée 《大分子材料与工程》2021,306(3):2000720
The introduction of metallic fillers to polymers via the photopolymerization approach can endow the composite materials with some unique properties, but the relevant research is still scarce due to the issue of light penetration and inner filter effect. Herein, for the first time the fabrication of photocomposites based on fine iron powder (i.e., a typical kind of metallic filler) is reported in this work. The free radical polymerization of two different acrylate monomers, poly(ethylene glycol) diacrylate and trimethylolpropane triacrylate, is performed in the presence of iron filler under mild conditions (i.e., light emitting diode (LED)@405 nm irradiation at room temperature under air). And the real-time Fourier transform infrared spectroscopy reveals remarkable photopolymerization kinetics of acrylates with high final conversions and fast polymerization rates despite the increasing contents of iron filler in the composites. Interestingly, the 3D printing technique is applied to the iron filler-based composites to produce tridimensional patterns with excellent spatial resolution. This work not only paves the way for the investigation of photocomposites based on metallic fillers through photochemical methods, but also broadens the potential application prospects. 相似文献
3.
Lai Wei Ryan McCloy Jie Bao Jesse Cranney 《American Institute of Chemical Engineers》2022,68(11):e17830
Modern chemical processes need to operate around time-varying operating conditions to optimize plant economy, in response to dynamic supply chains (e.g., time-varying specifications of product and energy costs). As such, the process control system needs to handle a wide range of operating conditions whilst optimizing system performance and ensuring stability during transitions. This article presents a reference-flexible nonlinear model predictive control approach using contraction based constraints. Firstly, a contraction condition that ensures convergence to any feasible state trajectories or setpoints is constructed. This condition is then imposed as a constraint on the optimization problem for model predictive control with a general (typically economic) cost function, utilizing Riemannian weighted graphs and shortest path techniques. The result is a reference flexible and fast optimal controller that can trade-off between the rate of target trajectory convergence and economic benefit (away from the desired process objective). The proposed approach is illustrated by a simulation study on a CSTR control problem. 相似文献
4.
We collect a household level panel dataset to estimate the price elasticities of electricity demand for different types of urban households in Bangladesh. We use an instrumental variable estimation strategy which exploits exogenous variation in average electricity prices induced by a value-added-tax shock. The results indicate significant heterogeneity in price elasticities by electricity consumption levels. We conduct a number of simulations under alternative policy scenarios to illustrate how incorporating the heterogeneous nature of price elasticities into pricing policy can help decrease electricity demand-supply mismatch and inequality in electricity consumption. The results have important policy implications for developing countries aiming to address major energy issues by implementing tariff reforms. 相似文献
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Investigation into time dependent long-term performance of Prefabricated Vertical Drains (PVDs) combined with vacuum consolidation in thick deposits of clay has been extremely limited. Predicting both settlements and excess pore pressures in such cases has become increasingly challenging when time duration is long-term, e.g. several years. In discussing such matter, finding a suitable model to predict the long-term performance is inevitable. Elasto-plastic analysis models such as Cam-Clay cannot predict long-term time-dependent deformational behaviour in soft soils. In this technical note, a Biot type fully-coupled creep-based elastic viscoplastic (EVP) finite element (FE) numerical model has been extended for application in vacuum consolidation. The vacuum consolidation section of the embankment constructed in Ballina, New South Wales, Australia (hereafter referred as Ballina embankment), is analysed using the model through a unit cell analysis and the numerical predictions are compared with field performance monitoring data up to 1200 days (>3 years). The proposed analysis method for PVD combined with vacuum consolidation involving an EVP model is found to be capable of predicting both short-term and long-term deformational behaviours. Predictions are improved when an exponential function is used for the secondary compression index in the EVP model. Comparison has also been carried out at another location in the embankment where the foundation clay thickness was different to check the precision of the methodology and for better understanding of ground settlement behaviour. Details of the analysis methodology and its validation against field performance data are presented in this note. 相似文献
9.
Low-light images enhancement is a challenging task because enhancing image brightness and reducing image degradation should be considered simultaneously. Although existing deep learning-based methods improve the visibility of low-light images, many of them tend to lose details or sacrifice naturalness. To address these issues, we present a multi-stage network for low-light image enhancement, which consists of three sub-networks. More specifically, inspired by the Retinex theory and the bilateral grid technique, we first design a reflectance and illumination decomposition network to decompose an image into reflectance and illumination maps efficiently. To increase the brightness while preserving edge information, we then devise an attention-guided illumination adjustment network. The reflectance and the adjusted illumination maps are fused and refined by adversarial learning to reduce image degradation and improve image naturalness. Experiments are conducted on our rebuilt SICE low-light image dataset, which consists of 1380 real paired images and a public dataset LOL, which has 500 real paired images and 1000 synthetic paired images. Experimental results show that the proposed method outperforms state-of-the-art methods quantitatively and qualitatively. 相似文献
10.
Dr. Adarshi P. Welegedara Dr. Ansis Maleckis Ruchira Bandara Dr. Mithun C. Mahawaththa Iresha Dilhani Herath Yi Jiun Tan Dr. Angeliki Giannoulis Prof. Daniella Goldfarb Prof. Gottfried Otting Prof. Thomas Huber 《Chembiochem : a European journal of chemical biology》2021,22(8):1480-1486
The selenol group of selenocysteine is much more nucleophilic than the thiol group of cysteine. Selenocysteine residues in proteins thus offer reactive points for rapid post-translational modification. Herein, we show that selenoproteins can be expressed in high yield and purity by cell-free protein synthesis by global substitution of cysteine by selenocysteine. Complete alkylation of solvent-exposed selenocysteine residues was achieved in 10 minutes with 4-chloromethylene dipicolinic acid (4Cl-MDPA) under conditions that left cysteine residues unchanged even after overnight incubation. GdIII−GdIII distances measured by double electron–electron resonance (DEER) experiments of maltose binding protein (MBP) containing two selenocysteine residues tagged with 4Cl-MDPA-GdIII were indistinguishable from GdIII−GdIII distances measured of MBP containing cysteine reacted with 4Br-MDPA tags. 相似文献