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排序方式: 共有2886条查询结果,搜索用时 15 毫秒
1.
Stefano Mariani Antonino Amedeo La Mattina Alessandro Paghi Lucanos Strambini Giuseppe Barillaro 《Advanced functional materials》2021,31(26):2100774
Here, a fluoride-assisted route for the controlled in-situ synthesis of metal nanoparticles (NPs) (i.e., AgNPs, AuNPs) on polydimethylsiloxane (PDMS) is reported. The size and coverage of the NPs on the PDMS surface are modulated with time and over space during the synthetic process, leveraging the improved yield (10×) and faster kinetics (100×) of NP formation in the presence of F− ions, compared to fluoride-free approaches. This enables the maskless preparation of both linear and step gradients and patterns of NPs in 1D and 2D on the PDMS surface. As an application in flexible plasmonics/photonics, continuous and step-wise spatial modulations of the plasmonic features of PDMS slabs with 1D and 2D AgNP gradients on the surface are demonstrated. An excellent spatially resolved tuning of key optical parameters, namely, optical density from zero to 5 and extinction ratio up to 100 dB, is achieved with AgNP gradients prepared in AgF solution for 12 minutes; the performance are comparable to those of commercial dielectric/interference filters. When used as a rejection filter in optical fluorescence microscopy, the AgNP-PDMS slabs are able to reject the excitation laser at 405 nm and retain the green fluorescence of microbeads (100 µm) used as test cases. 相似文献
2.
Marcus Weyd Christian Pflieger Andy Vogel Hannes Richter Volker Prehn Christiane Günther Frank Splittgerber Alessa Gäbler Daniel Kaulbars Patrick Bräutigam Marcus Franke Samira Lambertz Julian Schlechtweg Ingolf Voigt 《化学,工程师,技术》2021,93(9):1432-1439
Reducing micropollutant pollution of water bodies is an important objective of water management and an integral part of environmental policy. Ceramic nanofiltration membranes were developed as multichannel membranes of increased membrane area and rotating disk filters. The membranes developed show retention of over 80 % for PEG 400. The membranes are currently being tested for the separation of micropollutants from wastewater contaminated with pharmaceuticals. With the help of a downstream oxidative process, the trace substances remaining in the permeate are degraded. 相似文献
3.
Peng Li Haibin Jiang Ariel Barr Zhichu Ren Rui Gao Hua Wang Weiwei Fan Meifang Zhu Guiyin Xu Ju Li 《Advanced functional materials》2021,31(51):2105845
Mercury, lead, and cadmium are among the most toxic and carcinogenic heavy metal ions (HMIs), posing serious threats to the sustainability of aquatic ecosystems and public health. There is an urgent need to remove these ions from water by a cheap but green process. Traditional methods have insufficient removal efficiency and reusability. Structurally robust, large surface-area adsorbents functionalized with high-selectivity affinity to HMIs are attractive filter materials. Here, an adsorbent prepared by vulcanization of polyacrylonitrile (PAN), a nitrogen-rich polymer, is reported, giving rise to PAN-S nanoparticles with cyclic π-conjugated backbone and electronic conductivity. PAN-S can be coated on ultra-robust melamine (ML) foam by simple dipping and drying. In agreement with hard/soft acid/base theory, N- and S-containing soft Lewis bases have strong binding to Hg2+, Pb2+, Cu2+, and Cd2+, with extraordinary capture efficiency and performance stability. Furthermore, the used filters, when collected and electrochemically biased in a recycling bath, can release the HMIs into the bath and electrodeposit on the counter-electrode as metallic Hg0, Pb0, Cu0, and Cd0, and the PAN-S@ML filter can then be reused at least 6 times as new. The electronically conductive PAN-S@ML filter can be fabricated cheaply and holds promise for scale-up applications. 相似文献
4.
Chemical filters are the most important devices for removing gas-phase pollutants in clean rooms. However, the testing concentration of chemical filters is too high for reflecting their performance in a real clean room environment. This study tested the adsorption performance of chemical filters in the two most commonly used shapes at different concentrations. Then, the Langmuir equation and Wheeler-Jonas kinetic equation were combined to establish an adsorption performance prediction model of chemical filters under actual conditions. The predicted values of the model were in good agreement with the experimental results, which indicated the high accuracy of the prediction model. The model does not need to test the microscopic parameters of the adsorbent and can maintain high accuracy at low concentrations. A fast method for calculating the service life of chemical filters was also presented. Based on this model, the total cost of using a chemical filter with a high carbon content in microelectronic clean rooms could be decreased by 45% due to decreasing the number of filter replacements over 3 months. So a chemical filter with a high carbon content should be preferred over a filter with low resistance in microelectronic clean rooms. 相似文献
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7.
Chafic Saide Régis Lengelle Paul Honeine Cédric Richard Roger Achkar 《International Journal of Adaptive Control and Signal Processing》2015,29(11):1391-1410
Nonlinear adaptive filtering has been extensively studied in the literature, using, for example, Volterra filters or neural networks. Recently, kernel methods have been offering an interesting alternative because they provide a simple extension of linear algorithms to the nonlinear case. The main drawback of online system identification with kernel methods is that the filter complexity increases with time, a limitation resulting from the representer theorem, which states that all past input vectors are required. To overcome this drawback, a particular subset of these input vectors (called dictionary) must be selected to ensure complexity control and good performance. Up to now, all authors considered that, after being introduced into the dictionary, elements stay unchanged even if, because of nonstationarity, they become useless to predict the system output. The objective of this paper is to present an adaptation scheme of dictionary elements, which are considered here as adjustable model parameters, by deriving a gradient‐based method under collinearity constraints. The main interest is to ensure a better tracking performance. To evaluate our approach, dictionary adaptation is introduced into three well‐known kernel‐based adaptive algorithms: kernel recursive least squares, kernel normalized least mean squares, and kernel affine projection. The performance is evaluated on nonlinear adaptive filtering of simulated and real data sets. As confirmed by experiments, our dictionary adaptation scheme allows either complexity reduction or a decrease of the instantaneous quadratic error, or both simultaneously. Copyright © 2015 John Wiley & Sons, Ltd. 相似文献
8.
为实现小型磁环表面细微缺陷图像无监督分割,并提高分割精度与计算效率,本文提出了一种基于改进2D Gabor滤波器组的自适应阈值分割方法。首先,利用多尺度、多方向的Gabor滤波器组对缺陷图像进行滤波降噪处理,抑制目标区域与背景区域内部的噪声污染,同时增强区域间的差异性;然后,通过对处理后图像的灰度统计特性分析,根据缺陷图像的灰度均值及方差构造了灰度阈值计算公式,实现了小型磁环表面细微缺陷图像的自适应分割。实验结果表明,本文算法可快速、准确地分割缺陷并抑制噪声干扰,在分割精度、计算效率等方面也优于传统的选择迭代法、OTSU、最大熵等方法,并能够在先进的SEED-DVS8168平台上实时实现,验证了此算法的可行性与实时性。 相似文献
9.
Francesco Centurelli Pietro Monsurrò Vincenzo Stornelli Gianluca Barile Alessandro Trifiletti 《International Journal of Circuit Theory and Applications》2020,48(4):472-484
A 4th-order Butterworth class-AB current-mode low-pass filter is proposed, based on second-generation Current Conveyors (CCII). Class-AB operation allows high-power efficiency and driving large loads with small quiescent currents. The CCII topology uses the class-AB output buffer with error amplifiers: this topology is known to be sensitive to mismatch errors, which cause offsets in the error amplifiers, affecting the biasing current of the stage. This problem is solved via a control loop, which compensates the effect of mismatches. The technique is shown to be effective in Monte Carlo simulations with process variations and mismatches. Simulations have been carried out in 40 nm CMOS technology. The proposed filter achieves good power efficiency, thanks to the class-AB architecture, and good dynamic range, thanks to the closed-loop output buffer. A cut-off frequency of 6 MHz, with 184 μW of total quiescent power consumption, is achieved, with a THD of -55 dB and a SNR of 49 dB. 相似文献
10.
B. Luchini E. Storti T. Wetzig C. Settgast M. Abendroth J. Hubálková V.C. Pandolfelli C.G. Aneziris 《Journal of the European Ceramic Society》2019,39(8):2760-2769
In this work the influence of the production route and filter dimensions on the mechanical properties of carbon-bonded alumina foam filters was investigated. Features like cold crushing strength and fracture behavior were analyzed and used to compare them. Microfocus computer tomography (μCT) was applied to characterize the geometry of the filters, providing a deep correlation with their fracture behavior. Furthermore, computer-generated filter geometries were used as reference. The results indicated that the centrifugation process is better suited for the production of carbon-bonded alumina filters, and is even more effective when the foam dimensions are increased in the range of those analyzed in this research. Finite element simulations showed the influence of the relative density and strut tapering on the cold crushing strength of filters, providing a correlation between filter structure and its failure mechanism. The attained results provided further insights towards the production of inclusions-free metal parts. 相似文献