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1.
Christian Soize Roger Ghanem 《International journal for numerical methods in engineering》2022,123(1):268-290
The probabilistic learning on manifolds (PLoM) introduced in 2016 has solved difficult supervised problems for the “small data” limit where the number N of points in the training set is small. Many extensions have since been proposed, making it possible to deal with increasingly complex cases. However, the performance limit has been observed and explained for applications for which N is very small and for which the dimension of the diffusion-map basis is close to N. For these cases, we propose a novel extension based on the introduction of a partition in independent random vectors. We take advantage of this development to present improvements of the PLoM such as a simplified algorithm for constructing the diffusion-map basis and a new mathematical result for quantifying the concentration of the probability measure in terms of a probability upper bound. The analysis of the efficiency of this extension is presented through two applications. 相似文献
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《International Journal of Hydrogen Energy》2022,47(36):16121-16131
Ammonia is considered as a promising hydrogen or energy carrier. Ammonia absorption or adsorption is an important aspect for both ammonia removal, storage and separation applications. To these ends, a wide range of solid and liquid sorbents have been investigated. Among these, the deep eutectic solvent (DES) is emerging as a promising class of ammonia absorbers. Herein, we report a novel type of DES, i.e., metal-containing DESs for ammonia absorption. Specifically, the NH3 absorption capacity is enhanced by ca. 18.1–36.9% when a small amount of metal chlorides, such as MgCl2, MnCl2 etc., are added into a DES composed of resorcinol (Res) and ethylene glycol (EG). To our knowledge, the MgCl2/Res/EG (0.1:1:2) DES outperforms most of the reported DESs. The excellent NH3 absorption performances of metal–containing DESs have been attributed to the synergy of Lewis acid–base and hydrogen bonding interactions. Additionally, good reversibility and high NH3/CO2 selectivity are achieved over the MgCl2/Res/EG (0.1:1:2) DES, which enables it to be a potential NH3 absorber for further investigations. 相似文献
3.
《International Journal of Hydrogen Energy》2022,47(61):25511-25521
Metal/carbon composite materials are highly promising electrocatalysts for water electrolysis. In this work, three composites of metal cobalt nanoparticles highly dispersed in N-doped carbon materials were facilely constructed by pyrolysis of different phenylenediamine based Schiff base-Co complexes (PDBs). Interestingly, the composites derived from PDBs based on different phenylenediamine exhibited different morphologies. The superior case is that rodlike composite catalyst was derived from o-phenylenediamine based PDBs. The obtained catalyst exhibited remarkable performances for both cathodic hydrogen evolution reaction (HER) and anodic oxygen evolution reaction (OER), as well as overall water electrolysis. Only 172 and 289 mV of overpotentials and 1.57 V of cell voltage were exhibited at 10 mA cm?2 for HER, OER and water splitting in 1.0 M KOH, respectively. The catalyst also displayed robust stability and high Faraday efficiency, and thus are potential high-performance catalyst for commercial water electrolysis. 相似文献
4.
资源型产业发展为推进国家经济增长和工业化进程提供了重要保障。为深入了解资源型产业的研究情况,以CNKI数据库为数据源,搜集2000—2020年关于资源型产业的核心及以上期刊论文,利用CiteSpace软件从发文作者与研究机构分布、关键词共现网络和时区图谱等方面,绘制知识图谱,进行可视化分析。研究发现:资源型产业领域的研究成果愈加丰富,但研究群体间联系合作较少,且现有的合作研究主要集中在所处地域资源富集和具有学科优势的研究机构及学者;资源型产业领域的研究热点可概括为产业发展、资源型城市、产业集群、产业结构、产业链和产业集聚等方面;针对资源型产业领域未来可从资源型产业相关理论研究、创新发展模式和可持续发展等方面深入展开。 相似文献
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多堆厂址一级概率安全评价(PSA)研究中,机组数目的增加使得建模工作量剧增,给整个核电厂的风险评估带来困难。结合已有基础,本文研究了多堆厂址始发事件分析的筛选方法,提出利用堆芯损伤频率(CDF)上下限值评估方法,分析厂址内不同机组数对厂址CDF的影响。结果表明,双机组厂址适合优先进行具体分析。针对双机组核电站,对多堆厂址内各始发事件进行筛选。结果表明,丧失厂外电、丧失热阱等事件适合建模分析,并对其他筛选结果给出后续分析建议,为多堆厂址一级PSA后续事故序列建模工作提供了重要基础。 相似文献
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分别采用共沉淀法、清洁法制备焙烧态水铝钙石,通过低温N2吸脱附法、CO2-TPD、XRD、DTA和FT-IR表征结构,并将其作为大豆油与甲醇酯交换合成生物柴油的催化剂,探讨制备方法对焙烧态水铝钙石催化合成生物柴油的影响。此外,考察了Ca/Al摩尔比、焙烧温度、甲醇与大豆油摩尔比(醇油比)、催化剂用量和反应时间对酯交换合成生物柴油的影响。结果表明,清洁法制备的焙烧态水铝钙石具有更高的比表面积,强碱中心的表面碱量更大,催化活性更高。当Ca/Al摩尔比为2∶1,焙烧温度为600℃时,制备的Ca2Al O-2-600催化剂的催化活性最高,在醇油比8∶1、催化剂用量3%、反应温度65℃、反应时间4 h的条件下,大豆油转化率达到98. 0%。催化剂经重复使用3次后仍保持较高催化活性。 相似文献
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10.
ABSTRACTFeature selection is an important task to improve the classifier’s accuracy and to decrease the problem size. A number of methodologies have been presented for feature selection problems using metaheuristic algorithms. In this paper, an improved self-adaptive inertia weight particle swarm optimisation with local search and combined with C4.5 classifiers for feature selection algorithm is proposed. In this proposed algorithm, the gradient base local search with its capacity of helping to explore the feature space and an improved self-adaptive inertia weight particle swarm optimisation with its ability to converge a best global solution in the search space. Experimental results have verified that the SIW-APSO-LS performed well compared with other state of art feature selection techniques on a suit of 16 standard data sets. 相似文献