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1.
《Advanced Powder Technology》2022,33(9):103722
Through a facile hydrothermal method, we have successfully prepared Ti3C2/Bi2.15WO6 (TC/BWO) composite, and systematically investigated their reactivity for the photocatalytic reduction of Cr(VI) under visible light. X-ray diffraction and Raman analysis confirm the formation of heterostructure between Bi2.15WO6 and Ti3C2. The resultant 7TC/BWO composite exhibits enhanced photoactivity toward Cr(VI) reduction. After 120 min irradiation, the conversion of Cr(VI) reaches 92.5% with the quasi-first-order kinetic constant of k = 0.0145 min?1, which is higher than that of pure BWO (30% and k = 0.0005 min?1). The electrochemical and photoluminescent characterization confirm that the introduction of Ti3C2 is conducive to the separation of carriers, thus significantly improves the photocatalytic performance of TC/BWO. Furthermore, the radical capture experiments verify that the electrons are important for enhancing reduction of Cr(VI) to Cr(III). As a result, this research provides a comprehensive understanding of the reduction of Cr(VI) by TC/BWO composite under visible light. 相似文献
2.
《International Journal of Hydrogen Energy》2022,47(85):36216-36231
The fuel cell/battery durability and hybrid system stability are major considerations for the power management of fuel cell hybrid electric bus (FCHEB) operating on complicated driving conditions. In this paper, a real time nonlinear adaptive control (NAC) with stability analyze is formulated for power management of FCHEB. Firstly, the mathematical model of hybrid power system is analyzed, which is established for control-oriented design. Furthermore, the NAC-based strategy with quadratic Lyapunov function is set up to guarantee the stability of closed-loop power system, and the power split between fuel cell and battery is controlled with the durability consideration. Finally, two real-time power management strategies, state machine control (SMC) and fuzzy logic control (FLC), are implemented to evaluate the performance of NAC-based strategy, and the simulation results suggest that the guaranteed stability of NAC-based strategy can efficiently prolong fuel cell/battery lifespan and provide better fuel consumption economy for FCHEB. 相似文献
3.
《International Journal of Hydrogen Energy》2022,47(67):28782-28793
Highly-efficient and stable non-noble metal electrocatalysts for overcoming the sluggish kinetics of oxygen evolution reaction (OER) is urgent for water electrolysis. Biomass-derived biochar has been considered as promising carbon material because of its advantages such as low-cost, renewable, simple preparation, rich structure, and easy to obtain heteroatom by in-situ doping. Herein, Ni2P–Fe2P bimetallic phosphide spherical nanocages encapsulated in N/P-doped pine needles biochar is prepared via a simple two-step pyrolysis method. Benefiting from the maximum synergistic effects of bimetallic phosphide and biochar, high conductivity of biochar encapsulation, highly exposed active sites of Ni2P–Fe2P spherical nanocages, rapid mass transfer in porous channels with large specific surface area, and the promotion in adsorption of reaction intermediates by high-level heteroatom doping, the (Ni0.75Fe0.25)2P@NP/C demonstrates excellent OER activity with an overpotential of 250 mV and a Tafel slope of 48 mV/dec at 10 mA/cm2 in 1 M KOH. Also it exhibits a long-term durability in 10 h electrolysis and its activity even improves during the electrocatalytic process. The present work provides a favorable strategy for the inexpensive synthesis of biochar-based transition metal electrocatalysts toward OER, and improves the water electrolysis for hydrogen production. 相似文献
4.
用信号发生器产生脉冲宽度调制(pulse width modulation,PWM)信号模拟发动机电控单元驱动电磁阀运行,通过改变PWM信号频率、占空比和车辆运行工况,获得燃油蒸发回收系统不同的输出特性。分析了管容阀系统内气流脉动、结构振动和车内噪声随电磁阀控制信号变化的规律。建立了电磁阀体动力学模型,分析了电磁阀阀门受力情况,并与试验数据进行了综合分析。分析结果表明:电磁阀体振动主要由阀门关闭引起,车内敲击声来自电磁阀阀门关闭后气流脉动敲击炭罐,炭罐振动传递到车身,车身钣金振动辐射噪声。振动噪声随电磁阀PWM频率升高而增大,系统内气压波动幅值随频率升高而减小,相同占空比下,气压时均值随频率升高而增大。在电磁阀线圈两端反向并联整流二极管同时在电磁阀体进气管处设置孔板可以降低电磁阀阀门开闭运动引起的气流脉动及电磁阀和炭罐振动,消除车内敲击声。 相似文献
5.
为解决现有瓦斯抽采钻孔封孔工艺的封孔效果较差、导致瓦斯抽放效果不佳的问题,研究提出了新的瓦斯抽采钻孔密封关键工艺,在胡底煤业13091巷进行了瓦斯抽采现场试验。试验结果显示,应用该工艺后瓦斯抽采浓度、瓦斯抽采量均有大幅提高,取得了显著的瓦斯抽采效果和经济社会效益。 相似文献
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7.
从时空角度研究长江经济带的水环境污染状况,探究异质性环境规制对水环境污染的影响,为促进水资源合理利用与绿色发展提供参考。基于2009—2019年长江经济带11个省市的面板数据,研究长江经济带水环境污染的时空特征,用Moran's I指数研究水环境污染的空间自相关性,再通过空间杜宾模型探究异质性环境规制对水环境污染的空间溢出效应。研究表明:1)总体来看,长江经济带水环境污染呈上升趋势,其中上游地区水环境污染增速较快,下游和中游地区有所放缓,水环境污染得到一定控制;2)长江经济带水环境污染严重程度具有明显的空间特征,呈现出下游>中游>上游的趋势;3)从异质性角度来看,命令控制型环境规制能显著抑制水环境污染,在经济矩阵下效果最为显著,市场激励型环境规制具有显著负向作用,而公众自愿型环境规制的作用并不明显;4)从溢出效应来看,命令控制型环境规制对周围省市的水环境污染具有负向的空间溢出效应,市场激励型环境规制也会减轻周围省市的水环境污染严重程度,但没有命令控制型环境规制效果明显,公众自愿型环境规制效果不显著。目前长江经济带水环境污染状况仍不容乐观,需要进一步加强管控。虽然命令控制型环境规制对水环境污染治理效果最好,但公众参与也应该提上日程。各地要因地制宜,选择合适的方式来治理,此外还需要建立空间意识,加强联合治理。 相似文献
8.
本文以工业纯铝和混合稀土RE(Ce和La)为原料,制备出Al-8RE、Al-10RE和Al-15RE中间合金,并探讨了Al-RE中间合金对变形铝合金3102的细化机理。结果表明:Al-RE中间合金由α-Al、Al11RE3(Al11Ce3和Al11La3)、Ce和La组成,不同稀土含量Al-RE中间合金微观组织形貌不同,Al-8RE、Al-10RE和Al-15RE中间合金组织分别为亚共晶组织,伪共晶组织和过共晶组织,随稀土含量增加,Al-RE中间合金中Al11RE3相数量增多,尺寸增大;Al-RE中间合金对3102合金具有显著的细化效果,其中Al-10RE中间合金的细化效果最好;添加Al-RE中间合金可以提高产品性能,当添加10%RE时,性能提升最大。 相似文献
9.
文章以西班牙太阳能烟囱电站为原型,采用太阳射线追踪法加载太阳辐射,对太阳能烟囱电站和风力增压型太阳能烟囱电站进行三维数值模拟,探讨烟囱阴影下系统的流场特性和太阳入射角度对系统性能的影响。研究结果表明:烟囱阴影区蓄热层表面、集热棚表面温度突降,导致热气流与蓄热层表面、集热棚表面进行对流换热,造成热量损失;随着太阳入射角增加,系统轴功率和集热棚效率均明显下降;风力增压装置形成的出口负压可以削弱阴影所造成的气流掺混等不利影响,因而风力增压型太阳能烟囱电站涡轮机轴功率的变化幅度相对常规太阳能烟囱电站较为平缓。 相似文献
10.
Nonintrusive load monitoring (NILM) is crucial for extracting patterns of electricity consumption of household appliance that can guide users’ behavior in using electricity while their privacy is respected. This study proposes an online method based on the transient behavior of individual appliances as well as system steady-state characteristics to estimate the operating states of the appliances. It determines the number of states for each appliance using the density-based spatial clustering of applications with noise (DBSCAN) method and models the transition relationship among different states. The states of the working appliances are identified from aggregated power signals using the Kalman filtering method in the factorial hidden Markov model (FHMM). Thereafter, the identified states are confirmed by the verification of system states, which are the combination of the working states of individual appliances. The verification step involves comparing the total measured power consumption with the total estimated power consumption. The use of transient features can achieve fast state inference and it is suitable for online load disaggregation. The proposed method was tested on a high-resolution data set such as Labeled hIgh-Frequency daTaset for Electricity Disaggregation (LIFTED) and it outperformed other related methods in the literature. 相似文献