全文获取类型
收费全文 | 2173篇 |
免费 | 149篇 |
国内免费 | 1篇 |
专业分类
电工技术 | 21篇 |
综合类 | 1篇 |
化学工业 | 511篇 |
金属工艺 | 69篇 |
机械仪表 | 128篇 |
建筑科学 | 76篇 |
矿业工程 | 7篇 |
能源动力 | 75篇 |
轻工业 | 305篇 |
水利工程 | 22篇 |
石油天然气 | 24篇 |
无线电 | 146篇 |
一般工业技术 | 331篇 |
冶金工业 | 52篇 |
原子能技术 | 13篇 |
自动化技术 | 542篇 |
出版年
2024年 | 6篇 |
2023年 | 26篇 |
2022年 | 41篇 |
2021年 | 106篇 |
2020年 | 93篇 |
2019年 | 96篇 |
2018年 | 110篇 |
2017年 | 84篇 |
2016年 | 106篇 |
2015年 | 80篇 |
2014年 | 111篇 |
2013年 | 213篇 |
2012年 | 166篇 |
2011年 | 213篇 |
2010年 | 136篇 |
2009年 | 123篇 |
2008年 | 112篇 |
2007年 | 95篇 |
2006年 | 79篇 |
2005年 | 53篇 |
2004年 | 48篇 |
2003年 | 50篇 |
2002年 | 27篇 |
2001年 | 18篇 |
2000年 | 17篇 |
1999年 | 15篇 |
1998年 | 13篇 |
1997年 | 10篇 |
1996年 | 13篇 |
1995年 | 8篇 |
1994年 | 9篇 |
1993年 | 4篇 |
1992年 | 2篇 |
1991年 | 4篇 |
1990年 | 5篇 |
1989年 | 7篇 |
1988年 | 1篇 |
1987年 | 1篇 |
1986年 | 1篇 |
1985年 | 1篇 |
1984年 | 2篇 |
1982年 | 2篇 |
1981年 | 2篇 |
1980年 | 3篇 |
1979年 | 3篇 |
1978年 | 1篇 |
1977年 | 1篇 |
1976年 | 2篇 |
1975年 | 3篇 |
1973年 | 1篇 |
排序方式: 共有2323条查询结果,搜索用时 31 毫秒
1.
Sergey Tkachev Miguel Monteiro João Santos Ernesto Placidi Mohamed Ben Hassine Pedro Marques Paulo Ferreira Pedro Alpuim Andrea Capasso 《Advanced functional materials》2021,31(33):2103287
Graphene-based materials have attracted significant attention in many technological fields, but scaling up graphene-based technologies still faces substantial challenges. High-throughput top-down methods generally require hazardous, toxic, and high-boiling-point solvents. Here, an efficient and inexpensive strategy is proposed to produce graphene dispersions by liquid-phase exfoliation (LPE) through a combination of shear-mixing (SM) and tip sonication (TS) techniques, yielding highly concentrated graphene inks compatible with spray coating. The quality of graphene flakes (e.g., lateral size and thickness) and their concentration in the dispersions are compared using different spectroscopic and microscopy techniques. Several approaches (individual SM and TS, and their combination) are tested in three solvents (N-methyl-2-pyrrolidone, dimethylformamide, and cyrene). Interestingly, the combination of SM and TS in cyrene yields high-quality graphene dispersions, overcoming the environmental issues linked to the other two solvents. Starting from the cyrene dispersion, a graphene-based ink is prepared to spray-coat flexible electrodes and assemble a touch screen prototype. The electrodes feature a low sheet resistance (290 Ω □−1) and high optical transmittance (78%), which provide the prototype with a high signal-to-noise ratio (14 dB) and multi-touch functionality (up to four simultaneous touches). These results illustrate a potential pathway toward the integration of LPE-graphene in commercial flexible electronics. 相似文献
2.
Carla C. B. Brasil Cristiano R. de Menezes Eduardo Jacob-Lopes Juliano Smanioto Barin Leila Queiroz Zepka Paulo Cezar Bastianello Campagnol Roger Wagner Alexandre José Cichoski 《International Journal of Food Science & Technology》2020,55(3):1136-1144
This study investigated the effect of the combination of basic electrolysed water (BEW) and slightly acid electrolysed water (SAEW) with ultrasound (US) for cleaning and sanitation of the knives used in slaughtering processes. The knives were sonicated in a US bath using two modes of operation (normal and sweep) in two steps: (i) 5 min with BEW and (ii) 10 min with SAEW at 35 °C. The microbiological counts and the possible changes in the physical structure of the knives were evaluated. The association BEW + SAEW + US, in the sweep mode, provided lower mesophilic, enterobacterial, Staphylococcus aureus and yeast counts when compared to the values recommended by the international legislation. In addition, these conditions removed all organic residues from the knife blades and promoted the highest migration rate of the residues to the US water bath (12.35 mg/L·min), without modifications in the knife blades. Thus, cleaning and sanitation of knives was feasible with the association of BEW + SAEW + US, which could be a useful alternative for the meat industry. 相似文献
3.
4.
Marcos Antônio Klunk Nattan Roberto Caetano Rommulo Vieira Conceição Paulo Roberto Wander Sudipta Dasgupta 《The International journal of environmental studies》2020,77(3):492-509
ABSTRACT Several Carbon Capture and Storage (CCS) techniques have been studied including injections of carbon dioxide (CO2) into the mature and/or depleted hydrocarbon reservoirs and deep saline aquifers. This work aims to test storing CO2 into the magnesium-rich evaporite strata and also into the stratigraphic intervals containing Mg-rich brines. The test simulates Mg-carbonation of the synthetic solution obtained from the Mg-evaporite mineral, bischofite – both experimentally in the laboratory condition and also through computerised geochemical simulation. The laboratory experiments, which resulted in the crystallisation of anhydrous magnesite, were analysed. The TOUGHREACTTM, Geochemist’s WorkbenchTM (GWB) and PHREEQCTM software simulated the experiments as computerised geochemical model and tested the results for natural geological conditions. The geochemical simulations successfully demonstrate the immense CCS potential for the Mg-evaporite (as well as the sedimentary strata charged with Mg-evaporitic brine) at their subsurface geological occurrences at elevated pressure-temperature and high salinity. 相似文献
5.
6.
Lopez Daniel Andres Sanchez Chagas Luciana Gomes Batista Aline Domingues Guaita Maria Gabriella Detone Amorin Luís Henrique Cardozo da Silva Paulo Rogério Catarini Yamanishi Gustavo Zaia Dimas Augusto Morozin de Santana Henrique Urbano Alexandre 《Journal of Materials Science: Materials in Electronics》2021,32(13):17462-17472
Journal of Materials Science: Materials in Electronics - The increasing demand for lithium-ion batteries has stimulated the investigation of new compounds in order to reduce the costs and the... 相似文献
7.
Dr. Eduarda Mendes Enrico Cadoni Filipa Carneiro Dr. Marta B. Afonso Hugo Brito Dr. João Lavrado Dr. Daniel J. V. A. dos Santos Dr. Jorge B. Vítor Prof. Stephen Neidle Prof. Cecília M. P. Rodrigues Prof. Alexandra Paulo 《ChemMedChem》2019,14(14):1325-1328
Quadruplex nucleic acids are promising targets for cancer therapy. In this study we used a fragment-based approach to create new flexible G-quadruplex (G4) DNA-interactive small molecules with good calculated oral drug-like properties, based on quinoline and triazole heterocycles. G4 melting temperature and polymerase chain reaction (PCR)-stop assays showed that two of these compounds are selective G4 ligands, as they were able to induce and stabilize G4s in a dose- and DNA sequence-dependent manner. Molecular docking studies have suggested plausible quadruplex binding to both the G-quartet and groove, with the quinoline module playing the major role. Compounds were screened for cytotoxicity against four cancer cell lines, where 4,4′-(4,4′-(1,3-phenylene)bis(1H-1,2,3-triazole-4,1-diyl))bis(1-methylquinolin-1-ium) ( 1 d ) showed the greater activity. Importantly, dose–response curves show that 1 d is cytotoxic in the human colon cancer HT-29 cell line enriched in cancer stem-like cells, a subpopulation of cells implicated in chemoresistance. Overall, this study identified a new small molecule as a promising lead for the development of drugs targeting G4 in cancer stem cells. 相似文献
8.
Ingrid Lessa Leal Yasmin Carolino da Silva Rosa Josenai da Silva Penha Paulo Romano Cruz Correia Pollyana da Silva Melo Danilo Hansen Guimarães Josiane Dantas Viana Barbosa Janice Izabel Druzian Bruna Aparecida Souza Machado 《应用聚合物科学杂志》2019,136(43):48150
In this study, formulations of cassava starch and poly(butylene adipate-co-terephthalate) flexible films were developed, with glycerol, coconut nanocellulose, annatto, and citric acid in different concentrations, as well as the effectiveness of the selected materials in fresh-cut mangoes storage was evaluated. The tensile strength of the different formulations varied from 1.90 (E4) to 6.65 MPa (E3c), and the strain varied from 206.31 (E1c) to 278.41% (E8); this variation was dependent on the percentage of the polymer matrix incorporated. The aw values of the formulations ranged from 0.396 (E2) to 0.569 (E3c). The Formulations E4 and E7 (with additives) presented good properties and were selected to condition mangoes. The micrographs of these films showed regions of micropores that can facilitate the diffusion of water from the packaged product to the surface, allowing decreases in moisture and aw, which is associated with higher color maintenance during fruit storage. E7 presented better barrier properties than E4 (lower values of WVP and water solubility) which may have influenced in a positive way to maintain the stability of the package in the studied period. E7 can be considered as a viable alternative for minimally processed mango storage. © 2019 Wiley Periodicals, Inc. J. Appl. Polym. Sci. 2019 , 136, 48150. 相似文献
9.
Ranulfo Benedito de Paula Miranda Roger Borges Juliana Marchi Nelson Batista de Lima Paulo Francisco Cesar 《International Journal of Applied Ceramic Technology》2019,16(5):1979-1988
The addition of bioactive glasses to a Y:TZP matrix represents a feasible alternative to provide bioactivity to this material and optimize osseointegration. This work evaluated the effect of the BG concentration (0 and 10 wt%) and the sintering temperature (1200°C and 1300°C) on the microstructure, relative density, and flexural strength of the composite Y:TZP/BG. The Y:TZP and Y:TZP/BG powders were uniaxially pressed and sintered at 1200°C or 1300°C for 1 h. The microstructure was characterized by X-ray diffraction analysis, scanning electron microscopy, and energy-dispersive X-ray Spectroscopy. Relative density was calculated from density values obtained using the Archimedes’ principle. For the flexural strength, specimens (n = 6) were fractured in a biaxial flexural setup using a piston-on-three-balls fixture in a universal testing machine. Bioactivity test was performed in simulated body fluid solution. The results suggested that BG addition decreased the grain size of the composite, increased porosity and caused a significant decrease in the relative density and flexural strength. Crystalline phases of calcium stabilized cubic zirconia and sodium zirconium silicate were formed after the addition of BG. Finally, it was concluded that composite specimens sintered at 1300°C showed the highest density values and larger grains compared to those sintered at 1200°C. 相似文献
10.
Lauane G. Moreno Paulo H. Evangelista-Silva Edivânia C. Santos Rodrigo P. Prates Artenizia C. Lima Mateus F. Mendes Vinícius O. Ottone Marcelo H. F. Ottoni Wagner F. Pereira Gustavo E. B. A. Melo Elizabethe A. Esteves 《European Journal of Lipid Science and Technology》2021,123(9):2000332
Inflammatory bowel diseases (IBD) affect the gastrointestinal tract, and the imbalance of intestinal immune homeostasis can trigger them. Pequi oil (PO), a monounsaturated (MUFA) and carotenoid-rich food with nutraceutical potential, could help reshape the intestinal immune response, ameliorating IBD outcomes. This study investigates the effects of a 28 days intake of PO on elements of the intestinal immune response of mice with DSS-induced ulcerative colitis (disease activity index, colonic damage, inflammatory cells and markers). PO reduces body weight, colonic crypt and goblet cell losses and ameliorates diarrhea. In the colon, it increases γδT cells and secretory-IgA and decreases CD8+T cells. In lymphoid organs, it reduces CD8+T cells. Moreover, it also reduces the IL-17 and CRP in plasma. PO oil promotes a less cytotoxic response that may protect mice from immunological injuries caused by an IBD in the intestinal mucosa, improving the disease prognosis. Practical applications: This study demonstrates that the intake of pequi oil contributes to the regulation of immune response and improves clinical and histological signs of DSS-induced ulcerative colitis in mice. Its effects in cytotoxic cell reduction and other inflammatory markers and stimulation of regulatory cells, and preservation of mucus-producing cells, provide news insights about the importance of the regular intake of this food to better prognosis of ulcerative colitis acute episodes. In addition, these findings encourage further studies with foods with a protective potential for the intestinal mucosa. 相似文献