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1.
2021年9月16日,四川省泸县发生6.0级地震,对当地的文化遗产造成了不同程度的损坏。为掌握文化遗产在此次地震中的破坏情况,对古建筑、古桥、渡槽、摩崖造像、古遗址以及可移动文物进行震害调查,分析破坏原因,提出不同文化遗产的震害等级,并统计其在此次地震中破坏占比。研究结果表明:古建筑中木结构的震害较轻,砖木结构和石木结构的损伤较为严重,表现为墙体开裂、倾斜、倒塌和屋面损毁等破坏;古桥的桥面板产生裂缝和起壳,桥头堡基石发生移位;摩崖造像发生开裂、石像脱落,部分岩石发生坠落;古遗址的原有缝隙增大,石砌墙歪闪或倾斜;可移动文物与陈列台连接的金属卡件在地震下崩落。根据震害调查结果,将文化遗产的震害划分为4个等级,并对古建筑的维修与加固、摩崖造像的一体化监测、古桥的维护与应急抢险、可移动文物的隔震保护提出几点建议,为我国文化遗产的抗震保护提供参考。 相似文献
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N. Clament Sagaya Selvam Lijie Du Bao Yu Xia Pil J. Yoo Bo You 《Advanced functional materials》2021,31(12):2008190
Electroreduction of small molecules such as H2O, CO2, and N2 for producing clean fuels or valuable chemicals provides a sustainable approach to meet the increasing global energy demands and to alleviate the concern on climate change resulting from fossil fuel consumption. On the path to implement this purpose, however, several scientific hurdles remain, one of which is the low energy efficiency due to the sluggish kinetics of the paired oxygen evolution reaction (OER). In response, it is highly desirable to synthesize high-performance and cost-effective OER electrocatalysts. Recent advances have witnessed surface reconstruction engineering as a salient tool to significantly improve the catalytic performance of OER electrocatalysts. In this review, recent progress on the reconstructed OER electrocatalysts and future opportunities are discussed. A brief introduction of the fundamentals of OER and the experimental approaches for generating and characterizing the reconstructed active sites in OER nanocatalysts are given first, followed by an expanded discussion of recent advances on the reconstructed OER electrocatalysts with improved activities, with a particular emphasis on understanding the correlation between surface dynamics and activities. Finally, a prospect for clean future energy communities harnessing surface reconstruction-promoted electrochemical water oxidation will be provided. 相似文献
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Liting Yang Xiao Li Ke Pei Wenbin You Xianhu Liu Hui Xia Yonggang Wang Renchao Che 《Advanced functional materials》2021,31(35):2103971
Large interfacial resistance plays a dominant role in the performance of all-solid-state lithium-ion batteries. However, the mechanism of interfacial resistance has been under debate. Here, the Li+ transport at the interfacial region is investigated to reveal the origin of the high Li+ transfer impedance in a LiCoO2(LCO)/LiPON/Pt all-solid-state battery. Both an unexpected nanocrystalline layer and a structurally disordered transition layer are discovered to be inherent to the LCO/LiPON interface. Under electrochemical conditions, the nanocrystalline layer with insufficient electrochemical stability leads to the introduction of voids during electrochemical cycles, which is the origin of the high Li+ transfer impedance at solid electrolyte-electrode interfaces. In addition, at relatively low temperatures, the oxygen vacancies migration in the transition layer results in the formation of Co3O4 nanocrystalline layer with nanovoids, which contributes to the high Li+ transfer impedance. This work sheds light on the mechanism for the high interfacial resistance and promotes overcoming the interfacial issues in all-solid-state batteries. 相似文献
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Rapid advancements in wearable electronics impose the challenge on power supply devices. Herein, a flexible single-electrode triboelectric nanogenerator (SE-TENG) that enables both human motion sensing and biomechanical energy harvesting is reported. The SE-TENG is fabricated by interpenetrating Ag-coated polyethylene terephthalate (PET) nanofibers within a polydimethylsiloxane (PDMS) elastomer. The Ag coating and PDMS are performed as the electrode and dielectric material for the SE-TENG, respectively. The Ag-coated PET nanofibers enlarge the electrode surface area, which is beneficial to increase sensing sensitivity. The flexible SE-TENG sensor shows the capability of outputting alternating electrical signals with an open-circuit voltage up to 50 V and a short-circuit current up to 200 nA in response to externally applied pressure. It is used to sense various types of human motions and harvest electric energy from body motion. The harvested energy can successfully power wearable electronics, such as an electronic watch and light-emitting diode. Therefore, the as-prepared SE-TENG sensor with a pressure response and self-powered capability provides potential applications in wearable sensors or flexible electronics for personal healthcare and human–machine interfaces. 相似文献
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Matrix Manipulation of Directly-Synthesized PbS Quantum Dot Inks Enabled by Coordination Engineering
Fei Li Yang Liu Guozheng Shi Wei Chen Renjun Guo Dong Liu Yaohong Zhang Yongjie Wang Xing Meng Xuliang Zhang You Lv Wei Deng Qing Zhang Yao Shi Yifan Chen Kai Wang Qing Shen Zeke Liu Peter Müller-Buschbaum Wanli Ma 《Advanced functional materials》2021,31(45):2104457
The direct-synthesis of conductive PbS quantum dot (QD) ink is facile, scalable, and low-cost, boosting the future commercialization of optoelectronics based on colloidal QDs. However, manipulating the QD matrix structures still is a challenge, which limits the corresponding QD solar cell performance. Here, for the first time a coordination-engineering strategy to finely adjust the matrix thickness around the QDs is presented, in which halogen salts are introduced into the reaction to convert the excessive insulating lead iodide into soluble iodoplumbate species. As a result, the obtained QD film exhibits shrunk insulating shells, leading to higher charge carrier transport and superior surface passivation compared to the control devices. A significantly improved power-conversion efficiency from 10.52% to 12.12% can be achieved after the matrix engineering. Therefore, the work shows high significance in promoting the practical application of directly synthesized PbS QD inks in large-area low-cost optoelectronic devices. 相似文献
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30CrMnSiA钢具有较高的强度和良好的韧性,是重要的飞机结构受力部件,常在淬火后不同温度回火处理状态下使用。本研究取淬火态的30CrMnSiA钢在200~700 ℃进行回火,观察其金相组织,并使用超声检测方法对不同回火组织进行检测,分析超声波传播特征(纵波声速、声衰减系数、底波频移)与回火温度、组织变化之间的关系。结果表明:随回火温度提高,30CrMnSiA组织依次为回火马氏体、回火屈氏体、回火索氏体、铁素体+珠光体,硬度逐渐降低;受回火脆性的影响,在540~620 ℃回火得到的回火屈氏体超声检测特征参数值呈大幅度波动;其他回火组织进行超声检测时,随回火温度的升高,超声声速呈增大趋势,底波频移呈下降趋势。 相似文献
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This paper aims to find a reliable, collision-free path in a dynamic environment for highly maneuverable unmanned combat air vehicles (UCAVs). Given the real-time nature of the operational scenario, quick and adaptable reactions of UCAVs are necessary for updates in situational awareness. Therefore, we propose a three dimensional (3D) path planning approach based on the situational space to provide the tactical requirements of UCAVs for tracking targets and avoiding collisions. First, to ensure reliable nonlinear measurements, the interacting multiple model (IMM) algorithm based on a cubature Kalman filter (CKF) is chosen for the tracking and prediction algorithm. A constraint reference frame combining the kinematic model of constant acceleration (CA) is developed to solve the problem of arrival point generation. Second, by analyzing the relative motion between the UCAV and the moving objects, we define the situation space and give the corresponding calculation method. In tracking the moving target, the guidance vector contains the fusion information of displacement and velocity. At the same time, taking advantage of the one-step situation space as the judgment of the threat, we further plan the collision avoidance strategy. Third, as the safety in a practically reachable trajectory of the UCAV possesses the absolute priority, the collision avoidance acceleration accounts for this dominant factor in path planning. Simulations and experimental results prove that the proposed approach can plan a smooth and flyable path in 0.008 s under the premise of soft-landing target tracking. 相似文献