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Vitória Mussi Toschi Christine Bogicevic Houssny Bouyanfif Henri Laville Pierre-Eymeric Janolin 《Journal of the American Ceramic Society》2021,104(10):5257-5269
The morphotropic composition of the lead-free solid solution between Na0.5Bi0.5TiO3 and BaTiO3 (0.94 Na0.5Bi0.5TiO3-0.06 BaTiO3 or NBT-6BT) is of particular interest for the next generation of high-temperature capacitors but remains plagued by the diversity of dielectric properties reported in the literature. In order to explain the apparent inconsistencies among the reported dielectric properties of NBT-6BT, we examine the influence of stoichiometry, phase separation, and metallization method. We show that the nominal stoichiometry has a crucial effect, since increasing the nominal Na/Bi ratio increases conductivity and dielectric losses (tan δ). It also increases the real part of the permittivity (ε’) and the frequency dispersion of both ε’ and tan δ, thereby altering the shape of the evolution with temperature of the dielectric properties. Moreover it increases the depolarization temperature (Td) and decreases the temperature of maximum permittivity (Tm). Phase separation also occurs during the synthesis of NBT-6BT as Na evaporation leads to the formation of secondary Ba-containing phases. We report that these phases can have a positive impact on the dielectric properties: a moderate volume fraction (2.5 to 3.0%) and average grain surface (0.9 to 3.0 µm2) of these secondary Ba-containing phases increase the relative permittivity, decrease the dielectric losses, and increase the insulation resistance. We also show that the metallization method impacts the dielectric properties and therefore may contribute to the differences between various reports. The dielectric properties of NBT-6BT samples are measured during successive heating/cooling cycles and reveal that the permittivity value is lower during the first heating when silver paste, even cured, is used. These three components contribute to explaining the diversity of the reported dielectric properties of NBT-6BT. 相似文献
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Gehrig Daniel Rebecq Henri Gallego Guillermo Scaramuzza Davide 《International Journal of Computer Vision》2020,128(3):619-619
International Journal of Computer Vision - The original version of this article was unfortunately omitted to publish the footnote “The best result per row is highlighted in bold” in... 相似文献
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Dr. Mélissa Degardin Dr. Sharon Wein Dr. Jean‐Frédéric Duckert Marjorie Maynadier Dr. Alexandre Guy Dr. Thierry Durand Prof. Roger Escale Dr. Henri Vial Dr. Yen Vo‐Hoang 《ChemMedChem》2014,9(2):300-304
Plasmodium falciparum is responsible of the most severe form of malaria, and new targets and novel chemotherapeutic scaffolds are needed to fight emerging multidrug‐resistant strains of this parasite. Bis‐alkylguanidines have been designed to mimic choline, resulting in the inhibition of plasmodial de novo phosphatidylcholine biosynthesis. Despite potent in vitro antiplasmodial and in vivo antimalarial activities, a major drawback of these compounds for further clinical development is their low oral bioavailability. To solve this issue, various modulations were performed on bis‐alkylguanidines. The introduction of N‐disubstituents on the guanidino motif improved both in vitro and in vivo activities. On the other hand, in vivo pharmacological evaluation in a mouse model showed that the N‐hydroxylated derivatives constitute the first oral bioprecursors in bis‐alkylguanidine series. This study paves the way for bis‐alkylguanidine‐based oral antimalarial agents targeting plasmodial phospholipid metabolism. 相似文献
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亨利·巴瓦先生通过介绍其承担的6个项目(瑞士日内瓦扬特基金会花园、法国尼姆市中学校园庭院设计、混合停车场设计、魔水花园、绿色都市、巴黎市中心集市改造工程),向人们阐述了他的设计观念,他认为土壤是进行设计工作的基质和源泉,园林设计不仅要考虑土壤本身的含义,更要由表及里去考虑各个时期中自然、历史、文化对土壤的影响所形成的地貌物的整体。他通过实例告诉风景园林师要深入挖掘发现设计区域内一些未知的、看不见的东西,从而在整体上把握我们的设计。 相似文献
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Rudi Henri van Els João Nildo de Souza ViannaAntonio Cesar Pinho Brasil Jr. 《Renewable & Sustainable Energy Reviews》2012,16(3):1450-1461
There are at least 607 thousand households in the Brazilian Amazon that need to be attended with some form of regular electricity service. These households are not attended by the electricity sector through its electricity distribution companies and most of them have some form of precarious decentralized electricity generation that is not registered or regulated in the institutional framework. Diverse initiatives were taken by Brazilian government to attend these household through alternatives that relied on locally available renewable energy. This paper accesses this initiatives of rural electrification in the Brazilian Amazon. First an overview of the problems of rural electricity are discussed and its specificities in the Brazilian Amazon. Then the Brazilian institutional framework that organizes the decentralized electricity generation is described with its various limitations. The diverse initiatives undertaken to attend the rural communities in the Amazon since the 1990s are described, as well as how these initiatives are linked to the policies for rural electrification. The results shows that it can be inferred that sole market mechanisms are not sufficient to guarantee economic sustainability of these projects. This can be one of the reasons why traditional electricity distribution companies showed the lack of interest in promoting rural electrification with other means than grid extension. The most successful projects had financed efforts to integrate the generation of electricity into local development initiatives in order to guarantee sustainability and used substantial part of funding for local mobilization and organization. It needs a paradigm chance by treating these initiatives as local development initiatives and promoting alternative ways for its implementation through partnership between local new actors in the electricity sector and government and implementing policy on a local municipal level. 相似文献