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1.
Long-term chemical durability of borosilicate glasses that makes them a widely accepted form of nuclear waste disposal is achieved through the formation of a porous aluminosilicate gel layer that provides passivity and limits the transport of water to the reaction front. Detailed understanding of the porous silicate gel layer is thus critical in elucidating the corrosion mechanism of these glasses and to design of new glass composition for waste immobilization and other applications. In this paper, we use the diffuse charge reactive potential to generate porous aluminosilicate glass structures with compositions equivalent to the gel layers formed at the glass-water interface with an aim to understand the processing condition on the microstructure and atomic structure of these systems. We demonstrate the use of the charge scaling techniques is an effective approach to generate these porous structures with controllable pore mophologies. After initial validation of the potentials and calcium aluminosilicate glass structures using neutron diffraction, we created gel structures with compositions similar to well-known model nuclear waste borosilicate glasses. The porosities and the pore size distribution bear a strong correlation to the processing temperature, as well as to the local atomic structure. Thus, by controlling the processing parameters, the generated porous structures can be customized to closely resemble gel structures due to borosilicate glass corrosion. These results provide insights of the micro- and atomic structure features of the porous aluminosilicate glasses and on the optimal procedure to generate porous structures that can be comparable to experimentally observed gel layer structures thus to elaborate on the correlations between the structure and phenomena in glass-water interactions.  相似文献   
2.

In recent days, wireless sensor networks (WSN) plays a major role in the real time applications like military battlefield surveillance, industrial process monitoring, machine health monitoring and so on. In WSN, selecting the cluster head (CH) is the challenging task. CH selection is done by considering parameters of single layer only. In cross layer protocol more than one layers are considered for inter related parameters such as integration of MAC/physical layer and integration routing/MAC/physical layers. The main drawback of layer-based approach is not considering the effect on improvement of particular layer parameter to other layer parameters. In this paper, new cross layer technique for energy efficient module is designed to address the energy efficiency issues, which is common to all layers and used to optimize the energy from one layer parameter by others. Nowadays everything is possible with the help of Internet, so sharing the information between WSN and TCP through the energy efficient cross layer can be done. It is done with transport layer to enhance the application filed to be reliably connected to the web. In this paper, dynamically adapted sleep scheduling mechanism is used with residual energy of each node. Virtual end-to-end packet rate selection and congestion control feedback mechanism are considered for end to end delay. This reduces the packet loss with the support of data-rate adaptation technique.

  相似文献   
3.
During manufacturing of a component, cutting, turning, grinding, and milling operations are inevitable and these operations induce surface residual stresses. In this study, it is shown that, depending on the process employed for cutting, residual stresses generated at the cut surfaces can vary widely and they can, in turn, make the cut surfaces of austenitic stainless steel (SS) prone to stress corrosion cracking (SCC). An austenitic SS 304L plate was cut using three different procesess: bandsaw cutting, cutting using the cut-off wheel, and shearing. Surface residual stress measurement using the X-ray diffraction (XRD) technique is carried out close to the cutting edges and on the cross-section. SCC susceptibility studies were carried out as per ASTM G36 in 45% boiling magnesium chloride solution. Optical microscopic examination showed the presence of cracks, and confocal microscopy was used to measure the depth of cracks. The study confirmed that high tensile residual stresses present in the cut surfaces produced by cut-off wheel and shear cutting make the surfaces susceptible to SCC while the surfaces produced by bandsaw cutting are resistant to SCC. Hence, it is shown that there is a definite risk of SCC for product forms of austenitic SS with cut surfaces produced using cutting processes that generate high tensile residual stresses stored for a long period of time in a susceptible environment.  相似文献   
4.
Itaconate (ITA) is an emerging powerhouse of innate immunity with therapeutic potential that is limited in its ability to be administered in a soluble form. A library of polyester materials that incorporate ITA into polymer backbones resulting in materials with inherent immunoregulatory behavior is developed. Harnessing hydrolytic degradation release from polyester backbones, ITA polymers result in the mechanism specific immunoregulatory properties on macrophage polarization in vitro. In a functional assay, the polymer-released ITA inhibits bacterial growth on acetate. Translation to an in vivo model of biomaterial associated inflammation, intraperitoneal injection of ITA polymers demonstrate a rapid resolution of inflammation in comparison to a control polymer silicone, demonstrating the value of sustained biomimetic presentation of ITA.  相似文献   
5.
The International Journal of Advanced Manufacturing Technology - This study attempts to incorporate SiC particles in the weld zone during friction stir welding of Al 6351 alloy. SiC particles of...  相似文献   
6.
Starting with Darwin, biologists have asked how populations evolve from a low fitness state that is evolutionarily stable to a high fitness state that is not. Specifically of interest is the emergence of cooperation and multicellularity where the fitness of individuals often appears in conflict with that of the population. Theories of social evolution and evolutionary game theory have produced a number of fruitful results employing two-state two-body frameworks. In this study, we depart from this tradition and instead consider a multi-player, multi-state evolutionary game, in which the fitness of an agent is determined by its relationship to an arbitrary number of other agents. We show that populations organize themselves in one of four distinct phases of interdependence depending on one parameter, selection strength. Some of these phases involve the formation of specialized large-scale structures. We then describe how the evolution of independence can be manipulated through various external perturbations.  相似文献   
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8.
A novel, model-based test case generation approach for validating reactive systems, especially those supporting richly structured data inputs and/or interactions, is presented. Given an executable system model and an extended symbolic grammar specifying plausible system inputs, the approach performs a model-based simulation to (i) ensure the consistency of the model with respect to the specified inputs, and (ii) generate corresponding test cases for validating the system. The model-based simulation produces a state transition diagram (STD) automatically justifying the model runtime behaviors within the test case coverage. The STD can further be transformed to produce an evolved symbolic grammar, which can then be used to incrementally generate a refined set of test cases. As a case study, we present a live sequence chart (LSC) model-based test generator, named LCT in short, for LSC simulation and consistency testing. The evolved symbolic grammar produced by the simulator can either be used to generate practical test cases for software testing, or be further refined by applying our model-based test generation approach again with additional test coverage criteria. We further show that LSCs can also be used to specify and test certain temporal system properties during the model simulation. Their satisfaction, reflected in the STD, can either be served as a directive for selective test generation, or a basis for further temporal property model checking.  相似文献   
9.
Porous conducting carbon fiber‐based composite paper is used as an electrode backing in the fuel cell assembly. It not only acts as a channel through which the reactant and product gases pass to and from the bipolar plate and the catalyst site but also helps in the flow of electrons. In order to perform its role efficiently, it should have sufficient strength, high electrical conductivity, and ideal porous structure. Carbon paper has been fabricated, which builds up the required composite properties. Studies have been conducted to optimize the fiber/matrix ratio in the carbon paper, while ensuring the perfect combination of porosity, mechanical strength, and electrical conductivity for an electrode in a proton electrolyte membrane fuel cells. Detail physico‐mechanical and electrochemical characterizations further ascertain that the fiber/matrix ratio plays an important role in tuning the composite properties. The polarization curve of the unit proton exchange membrane (PEM) fuel cell (with an effective electrode area 4 cm2) shows a peak power density of 916 mW/cm2 for the sample with fiber/matrix ratio of 65:35, which is almost the same as the commercially available sigracet gas diffusion layer (SGL) carbon paper tested under similar conditions. Further, proportionally enlarging the electrode area to 100 cm2 shows that the carbon paper not only shows almost repeatable results in a given set up but also scales up.  相似文献   
10.
On‐demand and long‐term delivery of drugs are common requirements in many therapeutic applications, not easy to be solved with available smart polymers for drug encapsulation. This work presents a fundamentally different concept to address such scenarios using a self‐replenishing and optogenetically controlled living material. It consists of a hydrogel containing an active endotoxin‐free Escherichia coli strain. The bacteria are metabolically and optogenetically engineered to secrete the antimicrobial and antitumoral drug deoxyviolacein in a light‐regulated manner. The permeable hydrogel matrix sustains a viable and functional bacterial population and permits diffusion and delivery of the synthesized drug to the surrounding medium at quantities regulated by light dose. Using a focused light beam, the site for synthesis and delivery of the drug can be freely defined. The living material is shown to maintain considerable levels of drug production and release for at least 42 days. These results prove the potential and flexibility that living materials containing engineered bacteria can offer for advanced therapeutic applications.  相似文献   
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