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1.
Dr. Dae-Shik Kim Dr. Atsushi Endo Dr. Francis G. Fang Dr. Kuan-Chun Huang Dr. Xingfeng Bao Dr. Hyeong-wook Choi Dr. Utpal Majumder Dr. Young Y. Shen Steven Mathieu Xiaojie Zhu Kristen Sanders Dr. Thomas Noland Dr. Ming-Hong Hao Dr. Yu Chen Dr. John Y. Wang So Yasui Karen TenDyke Jiayi Wu Christy Ingersoll Kara A. Loiacono Dr. Janna E. Hutz Dr. Nadeem Sarwar 《ChemMedChem》2021,16(11):1741-1744
A strategy for creating potent and pan-genotypic stimulator of interferon genes (STING) agonists is described. Locking a bioactive U-shaped conformation of cyclic dinucleotides by introducing a transannular macrocyclic bridge between the nucleic acid bases leads to a topologically novel macrocycle-bridged STING agonist (MBSA). In addition to substantially enhanced potency, the newly designed MBSAs, exemplified by clinical candidate E7766 , exhibit broad pan-genotypic activity in all major human STING variants. E7766 is shown to have potent antitumor activity with long lasting immune memory response in a mouse liver metastatic tumor model. Two complementary stereoselective synthetic routes to E7766 are also described. 相似文献
2.
Wen Ma Yuanming Gao Jingxin Zhang Yu Bai Ruiling Jia Hongying Dong Ruijun Wang Manyu Bao 《Journal of the European Ceramic Society》2021,41(4):2734-2745
Srx(Zr0.9Y0.05Yb0.05)O1.95+x (x=1.0, 0.9, 0.8, 0.7) ceramics were prepared by solid state reaction sintering. The sintered Sr1.0(Zr0.9Y0.05Yb0.05)O2.95 is a single-phase solid solution while the sintered Srx(Zr0.9Y0.05Yb0.05)O1.95+x (x=0.9?0.7) are composites, and a significant grain growth inhibition is observed in the sintered Srx(Zr0.9Y0.05Yb0.05)O1.95+x (x=1.0, 0.9). Rare-earth elements distribution in the bulk materials indicates that Yb and Y preferentially substitute Zr-sites in SrZrO3, and the highest solubility of RE2O3 in pure SrZrO3 is ~0.8 mol%. The sintered Srx(Zr0.9Y0.05Yb0.05)O1.95+x have high thermal expansion coefficients up to ~11.0×10?6 K-1 (1200°C). Sr0.8(Zr0.9Y0.05Yb0.05)O2.75 has the lowest thermal conductivity of 1.38 W·m-1·K-1 at 800°C. Srx(Zr0.9Y0.05Yb0.05)O1.95+x (x=1.0, 0.9, 0.8) show no phase transition from 600 to 1400°C, whereas Srx(Zr0.9Y0.05Yb0.05)O1.95+x (x=0.9, 0.8) have excellent high-temperature phase stability over the whole investigated temperature range. Therefore, Srx(Zr0.9Y0.05Yb0.05)O1.95+x (x=1.0, 0.9, 0.8) are considered as promising TBCs materials that might be operated at higher temperatures compared to YSZ. 相似文献
3.
N. Clament Sagaya Selvam Lijie Du Bao Yu Xia Pil J. Yoo Bo You 《Advanced functional materials》2021,31(12):2008190
Electroreduction of small molecules such as H2O, CO2, and N2 for producing clean fuels or valuable chemicals provides a sustainable approach to meet the increasing global energy demands and to alleviate the concern on climate change resulting from fossil fuel consumption. On the path to implement this purpose, however, several scientific hurdles remain, one of which is the low energy efficiency due to the sluggish kinetics of the paired oxygen evolution reaction (OER). In response, it is highly desirable to synthesize high-performance and cost-effective OER electrocatalysts. Recent advances have witnessed surface reconstruction engineering as a salient tool to significantly improve the catalytic performance of OER electrocatalysts. In this review, recent progress on the reconstructed OER electrocatalysts and future opportunities are discussed. A brief introduction of the fundamentals of OER and the experimental approaches for generating and characterizing the reconstructed active sites in OER nanocatalysts are given first, followed by an expanded discussion of recent advances on the reconstructed OER electrocatalysts with improved activities, with a particular emphasis on understanding the correlation between surface dynamics and activities. Finally, a prospect for clean future energy communities harnessing surface reconstruction-promoted electrochemical water oxidation will be provided. 相似文献
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计算机技术、控制技术及信息技术的发展,电力系统自动化面临着空前的变革,多媒体技术、智能控制技术将迅速进入电力系统自动化领域。 相似文献
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Thermal management and catalytic combustion stability characteristics of premixed methane/air in heat recirculation meso‐combustors 下载免费PDF全文
Yunfei Yan Shuai Feng Zizhen Huang Li Zhang Wenli Pan Lixian Li Zhongqing Yang 《国际能源研究杂志》2018,42(3):999-1012
In order to illuminate heat recirculation effect on catalytic combustion stability and further improve energy conversion efficiency in meso‐combustor, the catalytic combustion characteristics of the combustor with/without preheating channels are numerically studied at steady conditions. It is found that methane conversion rate and combustion efficiency increases by 2% to 3% and approximately 9% in the heat recirculation meso‐combustor, indicating that heat recirculation effect facilitates more complete combustion of methane and medium components. Preheating channels show positive effects on improving combustion stability in the heat recirculation meso‐combustor. On one hand, preheating channels facilitate heat recirculation effect, and heat recirculation rate exceeds 10% for all cases and reaches 31.8% with an inlet velocity of 0.5 m/s, leading to significant increment of methane‐specific enthalpy at the preheating channel outlet. On the other hand, Rh(s)/O(s) ratios of catalytic surface and catalytic surface temperature in main reaction zone are enlarged by the preheating channels, facilitating methane adsorption at catalytic surface. Specially, most of fuels are consumed in a shorter distance with higher methane conversion speed, which brings benefits to promote combustion efficiency and may be helpful to inhibit the combustion instability in heat recirculation meso‐combustors. 相似文献
8.
为研究铝合金三角形波纹夹芯板对平头弹体的抗冲击性能及损伤特性,利用有限元软件ABAQUS/Explicit建立弹体冲击靶板的数值模拟模型,并结合实验验证了模型及其参数的有效性。基于数值计算结果,分析了三角形波纹夹芯板几何结构对其防护性能、失效模式和能量吸收的影响规律及机理,并与等面密度单层板进行对比分析,研究结果表明,靶体几何结构对其抗冲击性能存在影响,三角形波纹夹芯板抗冲击性能低于单层板抗冲击性能。此外,增加芯体拓扑结构夹角能显著提高三角形波纹夹芯板的抗冲击性能,并且靶板几何形状会对其失效模式及耗能特性存在影响。 相似文献
9.
目的 在视觉引导的工业机器人自动拾取研究中,关键技术难点之一是机器人抓取目标区域的识别问题。特别是金属零件,其表面的反光、随意摆放时相互遮挡等非结构化因素都给抓取区域的识别带来巨大的挑战。因此,本文提出一种结合深度学习和支持向量机的抓取区域识别方法。方法 分别提取抓取区域的方向梯度直方图(HOG)和局部二进制模式(LBP)特征,利用主成分分析法(PCA)对融合后的特征进行降维,以此来训练支持向量机(SVM)分类器。通过训练Mask R-CNN(regions with convolutional neural network)神经网络完成抓取区域的初步分割。然后利用SVM对Mask R-CNN识别的抓取区域进行二次分类,完成对干扰区域的剔除。最后计算掩码完成实例分割,以此达到对抓取区域的精确识别。结果 对于随机摆放的铜质金属零件,本文算法与单一的Mask R-CNN及多特征融合的SVM算法就识别准确率、错检率、漏检率3个指标进行了比较,结果表明本文算法在识别准确率上较Mask R-CNN和SVM算法分别提高了7%和25%,同时有效降低了错检率与漏检率。结论 本文算法结合了Mask R-CNN与SVM两种方法,对于反光和遮挡情况具有一定的鲁棒性,同时有效地提升了目标识别的准确率。 相似文献
10.
Yin Bao Lie Tang Matthew W. Breitzman Maria G. Salas Fernandez Patrick S. Schnable 《野外机器人技术杂志》2019,36(2):397-415
Sorghum (Sorghum bicolor) is known as a major feedstock for biofuel production. To improve its biomass yield through genetic research, manually measuring yield component traits (e.g. plant height, stem diameter, leaf angle, leaf area, leaf number, and panicle size) in the field is the current best practice. However, such laborious and time‐consuming tasks have become a bottleneck limiting experiment scale and data acquisition frequency. This paper presents a high‐throughput field‐based robotic phenotyping system which performed side‐view stereo imaging for dense sorghum plants with a wide range of plant heights throughout the growing season. Our study demonstrated the suitability of stereo vision for field‐based three‐dimensional plant phenotyping when recent advances in stereo matching algorithms were incorporated. A robust data processing pipeline was developed to quantify the variations or morphological traits in plant architecture, which included plot‐based plant height, plot‐based plant width, convex hull volume, plant surface area, and stem diameter (semiautomated). These image‐derived measurements were highly repeatable and showed high correlations with the in‐field manual measurements. Meanwhile, manually collecting the same traits required a large amount of manpower and time compared to the robotic system. The results demonstrated that the proposed system could be a promising tool for large‐scale field‐based high‐throughput plant phenotyping of bioenergy crops. 相似文献