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In2Se3纳米片改性的GO/WS2/Mg-ZnO复合材料光催化性能的研究
引用本文:龙慧,魏子乔,罗思瑶,董华锋,陈传盛.In2Se3纳米片改性的GO/WS2/Mg-ZnO复合材料光催化性能的研究[J].广东工业大学学报,2022,39(4):107-112.
作者姓名:龙慧  魏子乔  罗思瑶  董华锋  陈传盛
作者单位:1. 广东工业大学 物理与光电工程学院, 广东 广州 510006;2. 长沙理工大学 材料科学与工程学院, 湖南 长沙 410114
基金项目:国家自然科学基金资助项目(62005053);广东省基础与应用研究基金资助项目(2020A1515011178);广东工业大学青年百人计划资助项目(批准号:220413293)
摘    要:二维纳米材料由于其结构和性能的独特性受到广泛的关注,各类二维纳米材料合成方法和表面改性的研究也得到了快速发展,在光催化性能提升和能源环境领域等方面发挥着重要作用。本文通过在复合物GO/WS2/Mg-ZnO(rGOWMZ)中添加直接带隙半导体In2Se3纳米片,合成rGOWMZ+In2Se3复合材料。并研究其光催化性能,发现性能得到了明显的改善,其中In2Se3纳米片质量分数为0.5%经过600℃热处理的复合物,在自然光照射下对罗丹明B的降解率为99.6%。本报道中In2Se3纳米片是通过液相超声剥离法制备的,大小为100 nm,厚度约为5层。并采用透射电子显微镜、原子力显微镜、X射线衍射仪、扫描电子显微镜对复合材料进行了物相分析。发现rGOWMZ+In2Se3复合材料对有机颜料罗丹明B具有优异的光催化性能,此复合材料将在光催化领域中具有巨大的应用潜力。

关 键 词:In2Se3纳米片  二维材料  自然光  光催化降解  
收稿时间:2021-08-04

In2Se3 Sheets as Photosensitizers to Enhance the Photocatalytic Performance of Graphene Oxide/WS2/Mg-doped ZnO Composite under Natural Sunlight
Long Hui,Wei Zi-qiao,Luo Si-yao,Dong Hua-feng,Chen Chuan-sheng.In2Se3 Sheets as Photosensitizers to Enhance the Photocatalytic Performance of Graphene Oxide/WS2/Mg-doped ZnO Composite under Natural Sunlight[J].Journal of Guangdong University of Technology,2022,39(4):107-112.
Authors:Long Hui  Wei Zi-qiao  Luo Si-yao  Dong Hua-feng  Chen Chuan-sheng
Affiliation:1. School of Physics and Optoelectronic Engineering, Guangdong University of technology, Guangzhou 510006, China;2. College of Materials Science and Engineering, Changsha University of Science and Technology, Changsha 410114, China
Abstract:With the development of photocatalytic technology, the research and exploration of photocatalytic properties of 2D materials have also attracted much attention. The photocatalytic performance of graphene oxide/WS2/Mg-doped ZnO (rGOWMZ) composites under 600 ℃ annealing is excellent because the degradation rate of Rhodamine B (RhB) is 99.6% under natural light, with the added 0.5% amount of In2Se3 sheets which is a direct bandgap semiconductor. The In2Se3 sheets prepared through liquid exfoliation are about 100 nm and ~5 atomic layers thickness. The composites are carried out with Transmission electron microscope (TEM), Atomic force microscope (AFM), X-ray diffraction (XRD), and Scanning electron microscope (SEM). And the rGOWMZ+In2Se3 composites exhibit excellent photocatalytic property, showing great potential in photocatalyst application.
Keywords:In2Se3 sheets  2D materials  natural sunlight  photocatalytic enhancement  
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