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Strong localization effect and carrier relaxation dynamics in self-assembled InGaN quantum dots emitting in the green
Authors:Guo-En?Weng  Wan-Ru?Zhao  Shao-Qiang?Chen  Hidefumi?Akiyama  Zeng-Cheng?Li  Jian-Ping?Liu  Bao-Ping?ZhangEmail author
Affiliation:1.Department of Physics and Semiconductor Photonics Research Center,Xiamen University,Xiamen,P. R. China;2.Department of Electronic Engineering,Optoelectronics Engineering Research Center, Xiamen University,Xiamen,P. R. China;3.Institute for Solid State Physics, The University of Tokyo,Kashiwa,Japan;4.Department of Electronic Engineering,East China Normal University,Shanghai,P. R. China;5.Suzhou Institute of Nano-Tech and Nano-Bionics,Chinese Academy of Sciences,Suzhou,P. R. China
Abstract:Strong localization effect in self-assembled InGaN quantum dots (QDs) grown by metalorganic chemical vapor deposition has been evidenced by temperature-dependent photoluminescence (PL) at different excitation power. The integrated emission intensity increases gradually in the range from 30 to 160 K and then decreases with a further increase in temperature at high excitation intensity, while this phenomenon disappeared at low excitation intensity. Under high excitation, about 40% emission enhancement at 160 K compared to that at low temperature, as well as a higher internal quantum efficiency (IQE) of 41.1%, was observed. A strong localization model is proposed to describe the possible processes of carrier transport, relaxation, and recombination. Using this model, the evolution of excitation-power-dependent emission intensity, shift of peak energy, and linewidth variation with elevating temperature is well explained. Finally, two-component decays of time-resolved PL (TRPL) with various excitation intensities are observed and analyzed with the biexponential model, which enables us to further understand the carrier relaxation dynamics in the InGaN QDs.
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