Studies on LLFP transmutation in a pressurized water reactor

A systematic study on the long-lived fission product (LLFP) transmutation in a pressurized water reactor (PWR) is performed, aiming at an optimal transmutation strategy for present nuclear energy development. The LLFPs selected in the analysis include ⁹⁹Tc and ¹²⁹I discharged from light water reactors (LWRs). The isotope ¹²⁷I is also considered to avoid the difficulties in isotopes separation. To minimize the negative impacts of LLFPs on the core performance and safety parameters, metallic technetium or MgI₂ target pins mixed with ZrH₂ are designed and investigated. Through the numerical analysis on equilibrium cycles, the transmuted amounts of ⁹⁹Tc and ¹²⁹I equal to the yields from 1.94 and 4.22 PWRs with a power of 1000 MWe, respectively. Numerical results indicate that both ⁹⁹Tc and ¹²⁹I can be transmuted conveniently in present PWRs in the form of target pins.