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Nature and characteristics of gas–liquid flow regimes in a micro-packed bed reactor |
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| Authors: | Wei Liu Bingqi Xie Chenghao Zhang Xiaonan Duan Jisong Zhang |
| Affiliation: | 1. State Key Laboratory of Chemical Engineering, Department of Chemical Engineering, Tsinghua University, Beijing, China
Contribution: Investigation (lead), Visualization (lead), Writing - original draft (lead);2. State Key Laboratory of Chemical Engineering, Department of Chemical Engineering, Tsinghua University, Beijing, China Contribution: Software (equal);3. State Key Laboratory of Chemical Engineering, Department of Chemical Engineering, Tsinghua University, Beijing, China Contribution: Data curation (equal);4. State Key Laboratory of Chemical Engineering, Department of Chemical Engineering, Tsinghua University, Beijing, China Contribution: Formal analysis (equal);5. State Key Laboratory of Chemical Engineering, Department of Chemical Engineering, Tsinghua University, Beijing, China |
| Abstract: | Micro-packed bed reactors (μPBRs) have the advantages of high heat and mass transfer efficiency and excellent safety, and they have been successfully applied to hydrogenation and oxidation reactions. However, the study of gas–liquid flow regimes in the μPBR, which is essential for the mass transfer modeling and reactor scale-up, is still insufficient due to the limitation of micro-scale and complexity of capillary force. In this work, the flow regimes in the two-dimensional μPBR were systematically studied by visual method utilizing a high-performance camera. Four typical flow regimes and characteristics were captured, and flow regime transition was revealed. Effects of gas and liquid superficial velocities, liquid physical properties, and particle sizes on liquid spreading areal fraction and pressure drop were investigated. Flow regime transition correlation of churn flow and pseudo-static flow in the μPBR was provided for the first time based on the summary of the current and previous published results. |
| Keywords: | flow regime transition gas–liquid flow behavior micro-packed bed reactor pressure drop visualization |