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S22合金钢的氘扩散渗透行为
引用本文:李映婵,夏体锐,朱欣欣.S22合金钢的氘扩散渗透行为[J].原子能科学技术,2017,51(10):1853-1858.
作者姓名:李映婵  夏体锐  朱欣欣
作者单位:1.南华大学 环境与安全工程学院, 湖南 衡阳421001;2.中国原子能科学研究院 反应堆工程技术研究部,北京102413
基金项目:国家磁约束聚变能专项资助(2015GB109002)
摘    要:在分别采用光学显微镜和辉光放电光谱仪获得S22合金钢的金相显微组织和元素成分的基础上,利用已经过氘渗透速率定量标定的渗透实验装置,研究了S22合金钢在400~600℃下的氘扩散渗透行为,得到了氘在S22合金钢中的渗透率和扩散系数。对比分析了500℃时纯D2和He+1%D2下S22合金钢的氘渗透数据,结果表明,随氘分压的降低,氘在S22合金钢中的扩散渗透孕育期增加,氘渗透速率降低,但即使在较低氘分压下依然有氘渗透现象。该结果可为高温气冷堆、快堆等先进反应堆在使用S22合金钢时进行必要的氚渗透防护及其安全分析提供理论与数据支持。

关 键 词:高温气冷堆    S22合金钢    氘渗透    氚渗透防护

Behavior of Deuterium Diffusion and Permeation in S22 Alloy Steel
LI Ying-chan,XIA Ti-rui,ZHU Xin-xin.Behavior of Deuterium Diffusion and Permeation in S22 Alloy Steel[J].Atomic Energy Science and Technology,2017,51(10):1853-1858.
Authors:LI Ying-chan  XIA Ti-rui  ZHU Xin-xin
Affiliation:1.Institute of Environment and Safety Engineering, University of South China, Hengyang 421001, China; 2.Division of Reactor Engineering Technology Research, China Institute of Atomic Energy, Beijing 102413, China
Abstract:The microstructure and chemical composition of S22 alloy steel (S22 )were measured by using a optical microscope and a glow discharge spectrometer,respectively. The behavior of deuterium diffusion and permeation in S22 was investigated by using a gas permeation apparatus which was calibrated by a standard leak.The permeability and diffusion coefficient of deuterium at the range of 400-600 ℃ in S22 were measured and calculated.Deuterium permeation in S22 was compared between pure D2 and 1% D2 bal-anced with He.The results show that the diffusion and permeation incubation period of deuterium in S22 increases and the rate of deuterium permeation decreases with the decrease of deuterium pressure.But even at lower deuterium pressure,deuterium pene-tration in S22 remains.The results can provide theoretical and data support for the necessary tritium permeation protection and safety analysis in the use of S22 in advanced reactors such as high-temperature gas-cooled reactors and fast reactors.
Keywords:high-temperature gas-cooled reactor  S22 alloy steel  deuterium perme-ation  tritium permeation protection
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