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Ultrafast carrier dynamics of near-band-edge emission in single-crystal ZnO nanorods
Authors:Dandan Wang  Guozhong Xing  Xinying Wang  Mi Zhou  Jinghai Yang  Jian Cao
Affiliation:a School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang 212013, People's Republic of China
b Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore 637371, Singapore
c Department of Civil Engineering, Northeast Dianli University, Jilin 132012, People's Republic of China
d Department of Physics, Northeast Normal University, Changchun 130024, People's Republic of China
e State Key Laboratory of Supramolecular Structure and Materials, and Department of Physics, Jilin University, Changchun 130012, People's Republic of China
f Department of Physics, Jilin Normal University, Siping 136000, People's Republic of China
g Department of Science and Technology, Linköping University, Campus Norrköping, SE-601 74 Norrköping, Sweden
Abstract:We report on rational synthesis and optical characteristics of highly crystallined ZnO nanorods which were grown by a facile chemical vapor transport method. Temperature-dependent photoluminescence spectra of as-fabricated ZnO nanorods are dominated by near-band-edge emission with a characteristic fine structure due to high crystallinity. Furthermore, the recombination emission involving carrier dynamics of near-band-edge emission in ZnO nanorods was systematically investigated by temperature-dependent time-resolved photoluminescence spectroscopy. Recombination peaks pertaining to the exciton emissions are monitored and resolved in both temporal and spatial regimes.
Keywords:A. Semiconductors   B. Vapor deposition   D. Optical properties
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