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核电厂废物固化体90Sr、137Cs、60Co的浸出行为研究
引用本文:范雯雯,刘铁军,白杨,张志银.核电厂废物固化体90Sr、137Cs、60Co的浸出行为研究[J].原子能科学技术,2016,50(6):973-976.
作者姓名:范雯雯  刘铁军  白杨  张志银
作者单位:1.中国核电工程有限公司,北京100840;2.中国原子能科学研究院,北京102413
摘    要:以去离子水为释放环境,研究核电厂废树脂和浓缩液水泥固化体被完全浸泡情景下核素90Sr、137Cs、60Co的浸出行为。分析中以有效扩散系数表征浸出行为。试验结果表明:固化体中的核素累积浸出份额不超过4%,137Cs浸出最快,90Sr其次,60Co最慢;同类废物体的抗压强度越大,核素浸出速率越慢。

关 键 词:废物固化体    放射性核素    浸出    扩散系数

Study on Release Behavior of 90Sr, 137Cs and 60Co in NPP Solidified Waste Form
FAN Wen-wen,LIU Tie-jun,BAI Yang,ZHANG Zhi-yin.Study on Release Behavior of 90Sr, 137Cs and 60Co in NPP Solidified Waste Form[J].Atomic Energy Science and Technology,2016,50(6):973-976.
Authors:FAN Wen-wen  LIU Tie-jun  BAI Yang  ZHANG Zhi-yin
Affiliation:1.China Nuclear Power Engineering Co., Ltd., Beijing 100840, China; 2.China Institute of Atomic Energy, Beijing 102413, China
Abstract:The release behavior of radioactive nuclides 90Sr,137Cs and 60Co in NPP resin and concentrate cement-solidified waste form was studied.The release surrounding is that the waste is totally immersed by deionized water.The effective diffusivity was taken as release behavior.The results show that cumulative leaching fraction of nuclides in test solidified waste is under 4%,the release of 137Cs is the fastest,90Sr is the second and 60Co is the slowest.Nuclides releasing in the same waste sample becomes going down with compressive strength enlarging.
Keywords:solidified waste form  radioactive nuclide  release  diffusivity
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