Heavy metal pollution of coal mine-affected agricultural soils in the northern part of Bangladesh |
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Authors: | Mohammad A.H. Bhuiyan Lutfar Parvez M.A. Islam Samuel B. Dampare Shigeyuki Suzuki |
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Affiliation: | 1. Environment and Information Sciences, Yokohama National University, 79-7 Tokiwadai, Hodogaya-ku, Yokohama, Kanagawa 240-8501, Japan;2. Department of Soil Science, Patuakhali Science and Technology University, Dumki, Patuakhali-8602, Bangladesh;3. Department of Oceanography, University of Dhaka, Dhaka-1000, Bangladesh;4. Department of Fisheries, University of Dhaka, Dhaka-1000, Bangladesh;1. Department of Analytical Chemistry, Faculty of Science and Technology, University of the Basque Country, UPV/EHU, P.O. Box 644, 48080 Bilbao, Basque Country, Spain;2. Laboratory of Environmental Researches and Nanotechnology Development, Centro Universitário La Salle, Mestrado em Avaliação de Impactos Ambientais em Mineração, Victor Barreto, 2288 Centro, 92010-000 Canoas, RS, Brazil |
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Abstract: | Total concentrations of heavy metals in the soils of mine drainage and surrounding agricultural fields in the northern part of Bangladesh were determined to evaluate the level of contamination. The average concentrations of Ti, Mn, Zn, Pb, As, Fe, Rb, Sr, Nb and Zr exceeded the world normal averages and, in some cases, Mn, Zn, As and Pb exceeded the toxic limit of the respective metals. Soil pollution assessment was carried out using enrichment factor (EF), geoaccumulation index (Igeo) and pollution load index (PLI). The soils show significant enrichment with Ti, Mn, Zn, Pb, As, Fe, Sr and Nb, indicating inputs from mining activities. The Igeo values have revealed that Mn (1.24 ± 0.38), Zn (1.49 ± 0.58) and Pb (1.63 ± 0.38) are significantly accumulated in the study area. The PLIs derived from contamination factors indicate that the distal part of the coal mine-affected area is the most polluted (PLI of 4.02). Multivariate statistical analyses, principal component and cluster analyses, suggest that Mn, Zn, Pb and Ti are derived from anthropogenic sources, particularly coal mining activities, and the extreme proximal and distal parts are heavily contaminated with maximum heavy metals. |
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