| 铁基催化剂光催化还原CO2研究进展 |
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| 引用本文： | 党永强,李博妮,李可可,张建兰,冯香钰,张亚婷. 铁基催化剂光催化还原CO2研究进展[J]. 化工学报, 2021, 72(10): 5016-5027. DOI: 10.11949/0438-1157.20210617 |
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| 作者姓名： | 党永强 李博妮 李可可 张建兰 冯香钰 张亚婷 |
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| 作者单位： | 西安科技大学化学与化工学院,陕西西安710054;西安科技大学化学与化工学院,陕西西安710054;自然资源部煤炭资源勘查与综合利用重点实验室,陕西西安710021 |
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| 基金项目： | 国家自然科学基金青年项目(21503164);NSFC-山西煤基低碳联合基金项目(U1810113) |
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| 摘 要： | 利用可再生清洁能源——太阳能，将CO2转化为一氧化碳、甲烷、甲醇等，因同时具有提供可持续燃料和解决全球变暖问题的潜力而受到越来越多的关注。铁基材料因具有金属/半导体的特性和独特的电子结构，在光催化还原CO2领域具有广阔的应用潜力。基于此，各种具有高催化活性的铁基催化剂已经被设计来提高光催化还原CO2的效率。概述了近年来铁基催化剂在光催化还原二氧化碳中的研究进展，对它们的结构特征和催化活性进行了阐述和比较，最后总结了铁基催化剂在光催化还原CO2领域中待解决的问题，并展望了未来发展的方向。
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| 关 键 词： | 二氧化碳 还原 光催化 铁基催化剂 |
| 收稿时间： | 2021-05-06 |
Research progress in photocatalytic reduction of CO2 with iron-based catalysts |
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| Yongqiang DANG,Boni LI,Keke LI,Jianlan ZHANG,Xiangyu FENG,Yating ZHANG. Research progress in photocatalytic reduction of CO2 with iron-based catalysts[J]. Journal of Chemical Industry and Engineering(China), 2021, 72(10): 5016-5027. DOI: 10.11949/0438-1157.20210617 |
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| Authors: | Yongqiang DANG Boni LI Keke LI Jianlan ZHANG Xiangyu FENG Yating ZHANG |
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| Affiliation: | 1.College of Chemistry and Chemical Engineering, Xi’an University of Science and Technology, Xi’an 710054, Shaanxi, China;2.Key Laboratory of Coal Resources Exploration and Comprehensive Utilization, Ministry of Natural Resources, Xi’an 710021, Shaanxi, China |
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| Abstract: | Using renewable clean energy-solar energy to convert CO2 into carbon monoxide, methane, methanol, etc., has attracted more and more attention because of its potential to provide sustainable fuels and solve global warming problems. Iron-based materials have broad application potential in the field of photocatalytic reduction of CO2 due to their metal/semiconductor properties and unique electronic structure. According to this, various iron-based catalysts with high catalytic activity have been designed to enhance the efficiency of photocatalytic reduction of CO2. This article reviews recent advances in the field of photocatalytic reduction of carbon dioxide based on iron-based catalysts. The structural characteristics and catalytic activity of iron-based catalysts are described and compared. Finally, the problems to be solved and the future development direction of iron-based catalysts in the field of photocatalytic reduction of CO2 are summarized and prospected. |
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| Keywords: | carbon dioxide reduction photocatalysis iron-based catalyst |
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