Femtosecond Traveling-Wave Optical Parametric Amplification in MgO:LiNbO(3)

A mid-infrared femtosecond optical parametric amplifier tunable in the chemically important spectral region between 3.1 and 3.9 mum (at >10-muJ idler pulse energy) has been constructed on the basis of MgO:LiNbO(3) with 7% doping. With femtosecond pumping near 800 nm (Ti:sapphire regenerative amplifier) and narrow-band (long-pulse) seeding, this simple single-stage device provides maximum conversion efficiencies of 40% and exhibits extremely low seed threshold (<10-mW peak seed power for >1-muJ idler output). The generated idler pulses are almost transform limited with <200-fs pulse duration. The pulse-to-pulse fluctuations reproduce the stability of the pump source at 1-kHz repetition rate.     

High-power,high-repetition-rate picosecond optical parametric oscillators for the near-to mid-infrared

Abstract

We report high-repetition-rate, singly-resonant, picosecond optical parametric oscillators based on the nonlinear crystals LiB₃O₅ and KTiOAsO₄ which are synchronously pumped by a self-mode-locked Ti:sapphire laser operating at 81 MHz. These devices allow tunable pulse generation from 1·116-3·160 μm to be achieved. The LiB₃O₅ system produces average nearinfrared output powers of 325 mW and is continuous tuning over the wavelength range 1·16-2·26 μm. For 1·8 ps input pump pulses, transform-limited signal pulses with durations of 1-1·2 ps and idler pulses with durations of 2-2·2 ps have been generated over 1·2-2·2 μm, without requirement for dispersion compensation. The KTiOAsO₄ system produces average near-infrared output powers of 403 mW, with the signal tuning over 1·116-1·281 μm and idler tuning over 2·260-3·160 μm. Without dispersion compensation, signal (idler) pulses with durations between 1·01-1·03 (1·61-2·91) ps have been obtained for 1·2 ps input pump pulses.     

Timing jitter reduction and single-frequency operation in an acousto-optic Q-switched Cr,Nd:YAG laser

A laser-diode-pumped watt-level single-frequency combined actively and passively Q-switched (CAPQ) laser with a wavelength of 1064 nm that simultaneously uses a codoped Cr(4+),Nd(3+):YAG crystal as the gain medium and mode selector is presented. The optimum repetition period of the CAPQ laser is approximately 1.5 times the natural repetition period of the passively Q-switched laser. The averaged timing jitter is approximately 400 ns in the CAPQ laser and the repetition rate of the CAPQ laser is experimentally shown to reach a time instability of 0.2% over 10(6) pulses. The output is a stable single frequency with a linewidth of 400 MHz at 20 W pump power.     

Highly efficient, widely tunable, 10-Hz parametric amplifier pumped by frequency-doubled femtosecond Ti:sapphire laser pulses

We report a 10-Hz, highly efficient, widely tunable (from the visible to the IR), broadband femtosecond optical parametric generator and optical parametric amplifier (OPA) in BBO, LBO, and CBO crystals pumped by the frequency-doubled output of a regeneratively amplified Ti:sapphire laser at 400 nm. The output of the system is continuously tunable from 440 nm to 2.5 mum with a maximum overall efficiency of ~25% at 670 nm and an optical conversion efficiency of more than 36% in the OPA stage. The effects of the seed beam energy, the type of the crystal and the crystal length, and the pumping energy of the output of the OPA, such as the optical efficiency, the bandwidth, the pulse duration, and the group velocity mismatch between the signal and the idler and between the seeder and the pump, are investigated. The results provide useful information for optimization of the design of the system.     

Seeded femtosecond optical parametric amplification in the mid-infrared spectral region above 3 mum

Femtosecond optical parametric amplification that results in microjoule mid-infrared pulses at wavelengths exceeding 3 mum is demonstrated. Narrow-band quasi-cw seeding at the signal wavelength is applied to ensure the generation of nearly transform-limited femtosecond pulses at the idler wavelength. The broad bandwidth of the parametric amplification provided by pumping with femtosecond pulses from a Ti:sapphire regenerative amplifier at high intensity results in idler pulse durations shorter than the pump pulse length. The potentials of three nonlinear optical crystals that belong to the potassium titanyl phosphate family are comparatively studied. At 1-kHz repetition rate our all-solid-state system produces highly synchronized ~100-fs pulses in the spectral range between 3 and 4 mum.     

Tunable ultrafast infrared/visible laser to probe vibrational dynamics

A tunable, ultrafast (approximately 100 fs-approximately 1 ps) laser system generating mid-IR (3-10 microm) and UV/visible (392-417 nm, 785-835 nm) radiation is described and its output characterized. The system is designed to explore vibrational dynamics in the condensed phase in a direct, two-pulse, time-resolved manner, using Raman spectroscopy as the probe. To produce vibrational resolution, probe pulses are spectrally narrowed by use of a long doubling crystal. Frequency-resolved optical gating is used to evaluate beam characteristics. An effective method for determining the temporal overlap of the pump and probe pulses for a one-color, 400 nm configuration is illustrated. Representative results from studies of heme and paranitroaniline vibrational dynamics illustrate the effectiveness of the visible pump-visible probe portion of the system in illuminating fast structure and energy dynamics.     

Tunable continuous-wave doubly resonant optical parametric oscillator by use of a semimonolithic KTP crystal

A temperature-tuned continuous-wave doubly resonant optical parametric oscillator (OPO) consisting of a semimonolithic KTP crystal and a concave mirror has been designed and built. Under single-axial-mode-pair operation, we obtained a combined output power of the signal and idler light fields up to 365 mW at a pump power of 680 mW. The output wavelength of the OPO can be temperature tuned by as much as 9 nm. We achieved 2.8-GHz continuous frequency tuning of the OPO by tuning the pump laser frequency.     

Experimental investigation of high-energy wave-breaking-free-pulse generation in bidirectional-pumping all-fiber laser

We report a passively mode-locked all-fiber laser with bidirectional pumping, emitting high-energy wave-breaking-free pulses. Experimental investigations show that forward and backward pump powers mainly contribute on the chirp and the nonlinear phase shift of pulses, respectively. Nonlinear chirp pulses with 50 nJ pulse energy, 340 ps duration at a 8.2 MHz repetition rate are directly emitted from the all-fiber laser pumped by two 550 mW, 977 nm laser diodes. The pulses cannot be compressed to near the transform limit, showing that the chirp of pulses is nonlinear.     

Compact Dye Laser with High Peak Power

A low energy, unconfined spark provides an inexpensive and reliable source of pump radiation for a small dye laser. Kilowatt peak laser output is obtained, using sub-joule spark input energy. Pulse durations of order 10 ^-7 sec and repetition rates up to at least several hundred pulses per second are typical. Maintenance-free operation exceeds 10⁶ pulses, and a modular design facilitates replacement of expendable components when required.     

Synchronously pumped optical parametric oscillation in periodically poled lithium niobate with 1-w average output power

We report on a rugged all-solid-state laser source of near-IR radiation in the range of 1461-1601 nm based on a high-power Nd:YVO(4) laser that is mode locked by a semiconductor saturable Bragg reflector as the pump source of a synchronously pumped optical parametric oscillator with a periodically poled lithium niobate crystal. The system produces 34-ps pulses with a high repetition rate of 235 MHz and an average output power of 1 W. The relatively long pulses lead to wide cavity detuning tolerances. The comparatively narrow spectral bandwidth of <15 GHz is suitable for applications such as pollutant detection.     

All-solid-state tunable DCM dye laser pumped by a diode-pumped Nd:YAG laser

Lasing is observed near 620 nm in a DCM dye doped TiO(2)-content organically modified silicate (ORMOSIL) pumped by frequency-doubled radiation from a diode-pumped Q-switched Nd:YAG laser. The laser wavelength is tunable over 60 nm. A conversion efficiency of 18% is obtained at its central wavelength of 621 nm. The laser output energy has only a 10% reduction after 27,000 pulses at a pump repetition rate of 30 Hz and a pump intensity of 1 J/cm(2). An all-solid-state, compact, long-lifetime, and tunable dye laser has been demonstrated.     

Experimental and theoretical investigation of a multipass, plane mirror, femtosecond dye laser amplifier

Femtosecond pulses of a passive mode-locked Rhodamine-6G dye laser are amplified in a double-stage, three-pass, plane mirror, Sulforhodamine-101 amplifier system. Saturable filters (Schott glass RG645 and Malachite Green) are used to suppress amplified spontaneous emission. Input pulses of 110-fs duration are broadened to 240 fs in the amplifier system and recompressed to 75 fs in a prism-pair compressor. Using a 20-Hz Q-switched Nd:YAG pump laser of 50-mJ second-harmonic output energy, we obtained amplified and recompressed pulses of 180-μJ energy at 625 nm starting with 40-pJ input pulses. The small-signal amplification dynamics is studied numerically. Relevant gain dye and saturable filter parameters are derived. The influence of amplified spontaneous emission is analyzed.     

Mid-Infrared-Wavelength Generation in 2-mum Pumped Periodically Poled Lithium Niobate

A periodically poled lithium niobate optical parametric oscillator pumped by a Tm:YAG laser at 2.0124-mum wavelength has been demonstrated. A pump pulse energy of 5.1 mJ generated 0.65 mJ of signal and idler pulse energy at a 50-Hz repetition frequency with a 27.8-mum domain-period-length grating. The lithium niobate crystal at a temperature of 180 degrees C yielded 3.61- and 4.55-mum signal and idler wavelengths, respectively. Wavelength tuning over a wide range was achieved with domain-period lengths from 25.5 to 28.2 mum and crystal temperature tuning from 50 to 180 degrees C. Signal wavelengths of 3.26-3.76 mum and idler wavelengths of 4.33-5.34 mum were generated.     

Tunable single-mode operation of a pulsed optical parametric oscillator pumped by a multimode laser

High-quality single-longitudinal-mode (SLM) tunable signal radiation is generated by a pulsed optical parametric oscillator (OPO) pumped by a compact, inexpensive multimode laser. The OPO is based on periodically poled lithium niobate (PPLN) in a ring cavity that is injection seeded at its resonated signal wavelength by a single-mode tunable diode laser. Accurate control of the OPO cavity length and crystal temperature ensures a continuously tunable SLM signal output frequency range of >7.5 THz (>250 cm(-1)); the corresponding idler output remains multimode. High-resolution molecular spectra are recorded to verify OPO performance at wavelengths of ~1.55 mum. The observed signal optical bandwidth of 相似文献   

Extra-cavity, widely tunable, continuous wave MgO-doped PPLN optical parametric oscillator pumped with a Nd:YVO4 laser

An extra-cavity, widely tunable, and continuous wave (CW) singly resonant optical parametric oscillator (SRO) based on MgO-doped periodically poled lithium niobate (PPMgLN) has been developed. A Nd:YVO₄ laser pumped by 808 nm laser diode array (LDA) is used as the pump source. The threshold value of the SRO system is only 1.86 W at 1064 nm. 1101.1 mW of idler output at 3.217 μm and 2004.3 mW of signal output at 1.590 μm have been achieved when the pump power is 8.76 W, and this corresponds to a total (idler + signal) optic–optic conversion efficiency of 35.5%. The periods of the domain structure on the PPMgLN wafer can be changed by shifting the PPMgLN crystal, thus enabling a widely tunable mid-infrared spectrum of 3.026–4.485 μm, and signal wavelengths widely tunable in range of 1.395–1.641 μm. Along with the signal and idler light, the visible and near-infrared spectrum (697.5–820.5 nm, 603.6–645.5 nm, 532 nm, 421.3–463.3 nm) is observed. This OPO system is compact, simple and operated at room temperature.     

Single-frequency pulsed laser source with hybrid MOPA configuration

A unique approach with a hybrid master oscillator power amplifier configuration to obtain single-frequency, high-energy laser pulses at 1064 nm is presented. The setup consists of a single-frequency seed laser, a multistage fiber amplifier, and a four-pass crystal rod amplifier. Pulse energy of 10 mJ is obtained at the repetition rate of 100 Hz. The pulse width is about 110 ns with a transform-limited linewidth of 3.2 MHz. The M(2) factor of the output beam is about 1.5. To our knowledge, this is the first report of using a hybrid amplifier to obtain 10 mJ pulses with long pulse width and transform-limited linewidth.     

Generation and optical parametric amplification of picosecond supercontinuum

We have demonstrated the output characteristics of optical parametric amplification (OPA) seeded by a supercontinuum (SC) generated in deionized water excited by 1064 nm. The SC spectrum (from 426 to 943 nm) overlaps well with the tuning range of a 355 nm pumped OPA for both the signal and idler. The tunable range covers from 430 to 2035 nm, with a maximum overall energy conversion efficiency of 32% in the OPA stage. A FWHM bandwidth of 54 nm near the degeneracy point from 658 to 760 nm can be generated by using a collinear OPA. Chirping of the SC pulses is also investigated with the OPA technique. The time delay between the 430 nm component and the 567 nm component of the generated SC due to chirp is measured to be -10.72 ps, increasing almost linearly with the wavelength.     

Compact KTA-based intracavity optical parametric oscillator driven by a passively Q-switched Nd:GdVO4 laser

We present a compact and efficient KTA-based intracavity optical parametric oscillator (IOPO) driven by a diode-end-pumped Nd:GdVO(4)/Cr:YAG passively Q-switched laser. At the incident diode pump power of 9.2 W, signal (1.53 microm) and idler (3.47 microm) average output powers of up to 744 and 356 mW, respectively, have been obtained. The total (signal+idler) optical-to-optical conversion efficiency is as high as 12%. By using the knife-edge method, near-diffraction-limited signal and idler beams have been detected, and the M(2) factors are well within 1.2. In addition, based on the ABCD matrix theory, the impact of mode matching and the thermal lens effect on the OPO output have been analyzed.     

High power 2 MHz passively Q-switched nanosecond Nd:YVO4/Cr4+:YAG 914 nm laser

We report a high-power, high-repetition-rate end-pumped passively Q-switched Nd:YVO4/Cr4+: yttrium aluminum garnet 914 nm laser. The maximum output power of 3.8 W at 914 nm is achieved at 2 MHz with the absorbed pump power of 25.2 W. The highest single pulse energy of a pulsed 914 nm laser reaches 2.3 μJ with a pulse width of 27.1 ns.     

Passive mode-locking in erbium-doped fibre laser based on BN-GO saturable absorber

A C-band mode-locked fibre laser incorporating a boron nitride-doped graphene oxide (BN-GO)-based saturable absorber (SA) is proposed and demonstrated. The SA is fabricated by depositing multiple layers of synthesized BN-GO nanoparticles onto the polished surface of a side-polished fibre, which is then inserted into an erbium-doped fibre laser cavity to generate the desired pulsed output. The strong nonlinear optical response and light absorption of the BN-GO nanoparticles induces the generation of a highly stable mode-locked pulse at 1567.32?nm with visible Kelly’s sidebands. The pulses have a measured repetition rate of 13.56?MHz and a pulse width of 1.18?ps at the maximum pump power of 280.5?mW. The pulses have a frequency signal-to-noise ratio of ～53?dB, indicating a highly stable output. The proposed laser would find significant telecommunications applications, particularly for dense wavelength division multiplexing systems.