Time-of-flight photoelectron spectroscopy of gases using synchrotron radiation

A gas-phase time-of-flight (TOF) photoelectron spectrometer has been developed for use with synchrotron radiation. The excellent time structure of the synchrotron radiation at the Stanford Positron Electron Accelerator Ring (SPEAR) has been used as the time base for the TOF measurements. The TOF analyzer employs two multichannel plates (MCPs) in tandem as a fast electron multiplier with a matched 50-Omega anode to form an electron detector with a timing resolution of 相似文献   

A photoelectron velocity map imaging spectrometer for experiments combining synchrotron and laser radiations

A velocity map imaging/ion time-of-flight spectrometer designed specifically for pump-probe experiments combining synchrotron and laser radiations is described. The in-house built delay line detector can be used in two modes: the high spatial resolution mode and the coincidence mode. In the high spatial resolution mode a kinetic energy resolution of 6% has been achieved. The coincidence mode can be used to improve signal-to-noise ratio for the pump-probe experiments either by using a gate to count electrons only when the laser is present or by recording coincidences with the ion formed in the ionization process.     

A reversible time-of-flight detector for use in pseudocontinuous resonance enhanced multiphoton (pc-REMPI) detection

A time-of-flight coincidence detector is demonstrated. This detector is optimized for use in a pseudocontinuous resonance enhanced multiphoton ionization scheme that requires photoelectrons and photoions to be detected in coincidence. The detector utilizes two simultaneously operating charged particle detectors, one for the detection of electrons and the other for the detection of ions. In order to allow for field reversal, the detectors are physically identical, differing only by the value of applied voltages. Particular attention is given to the implementation of a charge-to-voltage transducer that allows for subnanosecond detection of both electrons and ions.     

10 ps resolution, 160 ns full scale range and less than 1.5% differential non-linearity time-to-digital converter module for high performance timing measurements

We present a compact high performance time-to-digital converter (TDC) module that provides 10 ps timing resolution, 160 ns dynamic range and a differential non-linearity better than 1.5% LSB(rms). The TDC can be operated either as a general-purpose time-interval measurement device, when receiving external START and STOP pulses, or in photon-timing mode, when employing the on-chip SPAD (single photon avalanche diode) detector for detecting photons and time-tagging them. The instrument precision is 15 ps(rms) (i.e., 36 ps(FWHM)) and in photon timing mode it is still better than 70 ps(FWHM). The USB link to the remote PC allows the easy setting of measurement parameters, the fast download of acquired data, and their visualization and storing via an user-friendly software interface. The module proves to be the best candidate for a wide variety of applications such as: fluorescence lifetime imaging, time-of-flight ranging measurements, time-resolved positron emission tomography, single-molecule spectroscopy, fluorescence correlation spectroscopy, diffuse optical tomography, optical time-domain reflectometry, quantum optics, etc.     

Combining high mass resolution and velocity imaging in a time-of-flight ion spectrometer using pulsed fields and an electrostatic lens

We describe a momentum resolving time-of-flight ion mass spectrometer that combines a high mass resolution, a velocity focusing condition for improved momentum resolution, and field-free conditions in the source region for high resolution electron detection. It is used in electron-ion coincidence experiments to record multiple ionic fragments produced in breakup reactions of small to medium sized molecules, such as F(3)SiCH(2)CH(2)Si(CH(3))(3). These breakup reactions are caused by soft x rays or intense laser fields. The ion spectrometer uses pulsed extraction fields, an electrostatic lens, and a delay line detector to resolve the position. Additionally, we describe a simple analytical method for calculating the momentum from the measured hit position and the time of flight of the ions.     

32 bin near-infrared time-multiplexing detector with attojoule single-shot energy resolution

We present two implementations of photon counting time-multiplexing detectors for near-infrared wavelengths, based on Peltier cooled InGaAs/InP avalanche photodiodes. A first implementation is motivated by practical considerations using only commercially available components. It features 16 bins, pulse repetition rates of up to 22 kHz, and a large range of applicable pulse widths of up to 100 ns. A second implementation is based on rapid gating detectors, permitting dead times below 10 ns. This allows one to realize a high dynamic-range 32 bin detector, able to process pulse repetition rates of up to 6 MHz for pulse widths of up to 200 ps. Analysis of the detector response at 16.5% detection efficiency reveals a single-shot energy resolution on the attojoule level.     

A magnetic-bottle multi-electron-ion coincidence spectrometer

A novel multi-electron-ion coincidence spectrometer developed on the basis of a 1.5 m-long magnetic-bottle electron spectrometer is presented. Electrons are guided by an inhomogeneous magnetic field to a detector at the end of the flight tube, while a set of optics is used to extract counterpart ions to the same detector, by a pulsed inhomogeneous electric field. This setup allows ion detection with high mass resolution, without impairing the high collection efficiency for electrons. The performance of the coincidence spectrometer was tested with double ionization of carbon disulfide, CS(2) → CS(2)(2+) + e(-) + e(-), in ultrashort intense laser fields (2.8 × 10(13) W/cm(2), 280 fs, 1030 nm) to clarify the electron correlation below the rescattering threshold.     

Optimisation of a scanning atom probe with improved mass resolution using post deceleration

In this paper, we present calculations and experimental results obtained using post deceleration of ions in a scanning atom probe (SAP) geometry to improve the mass resolution. Various electrode geometries, tip to electrode distances in the range 50-170 microm and three different pulse shapes have been evaluated. Experimental mass resolutions of 750 FWHM and 200 FWTM have been achieved reproducibly for the 184W3+ peak without the use of a reflectron lens. 3D finite element electrostatics software has been used to simulate the ion trajectories through the instrument and thus to calculate the variations in velocities for the different electrode configurations. The observed trends are found to agree well with experimental results.     

Transmissive x-ray beam position monitors with submicron position- and submillisecond time resolution

We present the development of fast transmissive center-of-mass x-ray beam position monitors with a large active area, based on a thinned position sensitive detector in both a duo- and a tetra-lateral variant. The detectors were tested at BESSY beamlines BL14.1, KMC-1, and KMC-2 and yielded signal currents of up to 3 microA/100 mA ring current at 10 keV photon energy using the monochromatic focused beam of BL14.1. The active area sizes were 1 x 1 and 3 x 3 mm(2) for the duo-lateral and 5 x 5 mm(2) for the tetra-lateral devices, with the duo-lateral detectors currently being available in sizes from 1 x 1 to 10 x 10 mm(2) and thicknesses between 5 and 10 microm. The presented detectors' thicknesses were measured to be 5 and 8 microm with a corresponding transmission of up to 93% at 10 keV and 15% at 2.5 keV. Up to a detection bandwidth of 10 kHz, the monitors provide submicron position resolution. For lower detection bandwidths, the signal-to-noise reaches values of up to 6 x 10(4) at 10 Hz, corresponding to a position resolution of better than 50 nm for both detector sizes. As it stands, this monitor design approach promises to be a generic solution for automation of state-of-the-art crystal monochromator beamlines.     

Improving the timing resolution of an electromagnetic calorimeter based on lead tungstate crystals

Results of the beam tests of the prototype photon spectrometer PHOS for the ALICE experiment at the Large Hadron Collider (CERN) are presented. The spectrometer is based on detector elements composed of lead tungstate (PbWO₄) crystals with dimensions of 22 × 22 × 180 mm and Hamamatsu S8664-55 (S8148) avalanche photodiodes. The beam tests have been performed on the secondary T10 beamline of the PS proton synchrotron. The main emphasis has been placed on the possibility of improving the PHOS timing resolution. Introduction of an additional timing channel with a silicon photomultiplier (SiPM) used as a photodetector is shown to improve the timing resolution for 1-GeV deposited energy from current value σ _t = 3 to 0.3 ns. Silicon photomultipliers of the Hamamatsu MPPC S10362-33 family with an active area of 3 × 3 mm² are used in these measurements. Using fast photomultiplier tubes with an 8-mm-diameter photocathode, the timing resolution attainable in electromagnetic shower development in a lead tungstate crystal has been measured for a large-area photodetector. The timing resolution for a deposited energy of 1 GeV is 150 ps. The effect of the detector channel temperature on the timing resolution is investigated. Cooling the crystal results in an increase both in the scintillation intensity and in the decay time of the scintillator and fails to substantially improve the timing resolution.     

A study of the possibility of improving the time resolution of the PHOS spectrometer

Experimental investigations have shown that a timing device based on a constant-fraction discriminator is capable of providing a time resolution of approximately 0.5 ns and a timing error of approximately ±0.25 ns in the energy range of 0.8?1.8 GeV. In the region of “low” energies (<0.6 GeV), the time resolution is decreased by the influence of detector noise, whose level is ~3–5 mV for most scintillation detectors under investigation.     

Monoenergetic proton emission from nuclear reaction induced by high intensity laser-generated plasma

A 10(16) W∕cm(2) Asterix laser pulse intensity, 1315 nm at the fundamental frequency, 300 ps pulse duration, was employed at PALS laboratory of Prague, to irradiate thick and thin primary CD(2) targets placed inside a high vacuum chamber. The laser irradiation produces non-equilibrium plasma with deutons and carbon ions emission with energy of up to about 4 MeV per charge state, as measured by time-of-flight (TOF) techniques by using ion collectors and silicon carbide detectors. Accelerated deutons may induce high D-D cross section for fusion processes generating 3 MeV protons and 2.5?MeV neutrons, as measured by TOF analyses. In order to increase the mono-energetic proton yield, secondary CD(2) targets can be employed to be irradiated by the plasma-accelerated deutons. Experiments demonstrated that high intensity laser pulses can be employed to promote nuclear reactions from which characteristic ion streams may be developed. Results open new scenario for applications of laser-generated plasma to the fields of ion sources and ion accelerators.     

The CORSET time-of-flight spectrometer for measuring binary products of nuclear reactions

The CORSET time-of-flight spectrometer has been developed at the Flerov Laboratory of Nuclear Reactions of the Joint Institute for Nuclear Research (Dubna, Russia) for investigating binary products of nuclear reactions. The spectrometer has been used to study the dynamics of fusion-fission and quasi-fission of superheavy elements. The design and the main characteristics of the spectrometer, as well as the algorithms for deducing the mass-energy distributions of fragments and the cross sections of nuclear reactions, are presented. The spectrometer contains two time-of-flight arms based on microchannel-plate detectors and three telescopes, each of which is composed of two microchannel-plate detectors and one semiconductor detector. A system of four semiconductor detectors is used to obtain the absolute value of a cross section. The time resolution of the time-of-flight arms is 150 ps, which allows the time-of-flight distances to be set at 10–20 cm, thus providing a mass resolution of 3 amu and an angular resolution of 0.3°. Owing to these characteristics, the spectrometer can be used as a trigger in multidetector setups for measuring light charged particles, neutrons, and γ rays in coincidence with reaction fragments.     

A large aperture magnification lens for velocity map imaging

We have designed and implemented a large aperture electrostatic Einzel lens that magnifies the images of low energy ions or electrons in a standard velocity map imaging apparatus by up to a factor of 5 while allowing the normal use of the apparatus (without blocking any part of the detector). The field strength in the interaction region remains reasonably constant with or without magnification, and the lens can be used in the normal "crush" mode or with any of the different variants of the "slicing" mode. We have characterized the performance of the lens by imaging ion recoil due to two-photon resonant three-photon ionization [(2+1) REMPI] of O((3)P(2)) atoms and by imaging slow NO molecules from the near-threshold photodissociation of the NO-Ar van der Waals complex.     

Monte Carlo simulations of microchannel plate detectors. I. Steady-state voltage bias results

X-ray detectors based on straight-channel microchannel plates (MCPs) are a powerful diagnostic tool for two-dimensional, time-resolved imaging and time-resolved x-ray spectroscopy in the fields of laser-driven inertial confinement fusion and fast Z-pinch experiments. Understanding the behavior of microchannel plates as used in such detectors is critical to understanding the data obtained. The subject of this paper is a Monte Carlo computer code we have developed to simulate the electron cascade in a MCP under a static applied voltage. Also included in the simulation is elastic reflection of low-energy electrons from the channel wall, which is important at lower voltages. When model results were compared to measured MCP sensitivities, good agreement was found. Spatial resolution simulations of MCP-based detectors were also presented and found to agree with experimental measurements.     

Self-suppression of reset induced triggering in picosecond SPAD timing circuits

We present a new photon timing circuit that achieves a time resolution of 35 ps full width at half maximum with single photon avalanche diodes having active area diameters up to 200 microm. The timing circuit is based on a double avalanche current sensing network that makes it particularly suited to operation at high photon counting rates. Thanks to its self-adjusting capabilities, no trimming is needed even when changing the photodetector operating conditions over a wide range.     

A time-of-flight detector of low-energy ions for an accelerating mass-spectrometer

The results of experiments with a time-of-flight detector for detecting rare ions at the output of the accelerating mass spectrometer of the Institute of Nuclear Physics (Siberian Branch, Russian Academy of Sciences) are described. The operation of this detector is based on detection of electron emission from thin films by means of microchannel plates. Owing to the small thickness of films, ions can sequentially pass through several films—this is the basis of the time-of-flight system for identifying isotopes. The high time resolution of detectors allows a significant decrease in the external-radiation background compared to one semiconductor complete-absorption detector that measures the ion energy.     

高能量离子束诊断质谱仪的研制及性能表征

本研究开发了一台应用于高能量离子束诊断的直线式飞行时间质谱仪,实现了其与高能真空弧放电离子源的联用。该仪器加速电压30 kV,飞行腔有效飞行距离1.5 m,通过短脉冲离子门精确截取,ICCD高速相机优化聚焦,仪器分辨率优于90 FWHM,对放电过程中产生的等离子体可实现不同时间的离子成分分析。将该方法用于真空弧放电离子源放电过程中离子成分的检测,放电2 μs时,电离成分以气态离子C⁺、O⁺、C²⁺、O²⁺为主;放电6 μs后,除气体成分外,还可以检测到Fe⁺、Cu⁺及其同位素金属离子峰。该仪器能够给出离子源放电产生离子的种类、价态以及相对含量等信息,可实现整个放电过程产生离子成分信息的准确诊断。     

High sensitivity microchannel plate detectors for space extreme ultraviolet missions

Microchannel plate (MCP) detectors have been widely used as two-dimensional photon counting devices on numerous space EUV (extreme ultraviolet) missions. Although there are other choices for EUV photon detectors, the characteristic features of MCP detectors such as their light weight, low dark current, and high spatial resolution make them more desirable for space applications than any other detector. In addition, it is known that the photocathode can be tailored to increase the quantum detection efficiency (QDE) especially for longer UV wavelengths (100-150 nm). There are many types of photocathode materials available, typically alkali halides. In this study, we report on the EUV (50-150 nm) QDE evaluations for MCPs that were coated with Au, MgF(2), CsI, and KBr. We confirmed that CsI and KBr show 2-100 times higher QDEs than the bare photocathode MCPs, while Au and MgF(2) show reduced QDEs. In addition, the optimal geometrical parameters for the CsI deposition were also studied experimentally. The best CsI thickness was found to be 150 nm, and it should be deposited on the inner wall of the channels only where the EUV photons initially impinge. We will also discuss the techniques and procedures for reducing the degradation of the photocathode while it is being prepared on the ground before being deployed in space, as adopted by JAXA's EXCEED mission which will be launched in 2013.     

Collection of secondary electrons in scanning electron microscopes

Collection of the secondary electrons in the scanning electron microscope was simulated and the results have been experimentally verified for two types of the objective lens and three detection systems. The aberration coefficients of both objective lenses as well as maximum axial magnetic fields in the specimen region are presented. Compared are a standard side‐attached secondary electron detector, in which only weak electrostatic and nearly no magnetic field influence the signal trajectories in the specimen vicinity, and the side‐attached (lower) and upper detectors in an immersion system with weak electrostatic but strong magnetic field penetrating towards the specimen. The collection efficiency was calculated for all three detection systems and several working distances. The ability of detectors to attract secondary electron trajectories for various initial azimuthal and polar angles was calculated, too. According to expectations, the lower detector of an immersion system collects no secondary electrons I and II emitted from the specimen and only backscattered electrons and secondary electrons III form the final image. The upper detector of the immersion system exhibits nearly 100% collection efficiency decreasing, however, with the working distance, but the topographical contrast is regrettably suppressed in its image. The collection efficiency of the standard detector is low for short working distances but increases with the same, preserving strong topographical contrast.