Sick building syndrome—A case study in a multistory centrally air-conditioned building in the Delhi City

Recently, airtight envelope system has become popular in the design of office buildings to reduce heating and cooling loads. Maintaining allowable indoor air quality (IAQ) for such airtight buildings totally depends on mechanical ventilation systems. Subsequently, poor operation of the ventilation system in such office buildings causes ineffective removal of polluted indoor air, and displays a sign of “sick building syndrome” (SBS). User's perception is an important parameter for evaluating IAQ. A questionnaire study was carried out to investigate the prevalence of the SBS at a multistory centrally air-conditioned Airport Authority of India (AAI) building in the New Delhi city. Quantification of the perceptions of the users regarding IAQ was done by converting their responses to a SBS score. The quantified answers were then subjected to statistical analysis. Qualitative analysis of the questionnaire was carried out to evaluate relationships between SBS score and carbon dioxide (CO₂) and other parameters related to building and work environment. Quantitative analysis of IAQ was also conducted by monitoring indoor concentrations of four pollutants, namely, nitrogen dioxide (NO₂), sulphur dioxide (SO₂), suspended particulate matter (SPM) and carbon monoxide (CO). Concentrations of pollutants were complying with IAQ standards as given by ASHRAE and WHO. The SBS was higher on the third floor as compared to other floors and the control tower. The main symptoms prevailing were headache (51%), lethargy (50%), and dryness in body mucous (33%). The third floor and the control tower were affected by infiltration, mainly from entrance doors. A direct relation between the average SBS score and CO₂ concentration was found, i.e., the average SBS score increased with CO₂ concentration and vice versa, clearly signifying the usefulness of SBS score in IAQ.     

Indoor emissions of total and fluorescent supermicron particles during HOMEChem

Inhalation of particulate matter is associated with adverse health outcomes. The fluorescent portion of supermicron particulate matter has been used as a proxy for bioaerosols. The sources and emission rates of fluorescent particles in residential environments are not well-understood. Using an ultraviolet aerodynamic particle sizer (UVAPS), emissions of total and fluorescent supermicron particles from common human activities were investigated during the HOMEChem campaign, a test-house investigation of the chemistry of indoor environments. Human occupancy and activities, including cooking and mopping, were found to be considerable sources of indoor supermicron fluorescent particles, which enhanced the indoor particle concentrations by two orders of magnitude above baseline levels. The estimated total (fluorescent) mass emission rates for the activities tested were in the range of 4-30 (1-11) mg per person meal for cooking and 0.1-4.9 (0.05-4.7) mg/h for occupancy and mopping. Model calculations indicate that, once released, the dominant fate of coarse particles (2.5-10 micrometer in diameter) was deposition onto indoor surfaces, allowing for the possibility of subsequent resuspension and consequent exposures over durations much longer than the ventilation time scale. Indoor coarse particle deposition would also contribute to soiling of indoor surfaces.     

Measurements of biological contaminants and particulate matter inside a dwelling in Japan

To investigate the biological contaminant levels inside dwellings in Japan, the authors measured fungal indices, airborne mite allergens (Der 1 and Der 2), and suspended particulate matter (SPM). Measurements were continuously conducted at one dwelling located in Yokosuka-city, Kanagawa. The biosensors for fungal index were set at 12 points inside and 2 points outside the dwelling. An SPM sampler was placed in the living room, and samplers for collecting allergens were placed in the living room and in the washroom. The peak level of the fungal index was recorded during July, which is the rainy season in Japan. The highest value in the dwelling was 6.9 in the toilet, and the second highest was 6.6 near a window in the living room that faces southeast, and behind the sofa. The highest monthly SPM level was 21.5 micrograms/m3 during October, and the highest monthly allergen level (Der 1) in the living room was 25.7 pg/m3 during November. A positive relationship between the fungal index and mite allergens was not observed, and the levels of contaminants were not as those found in other studies. However, further study to investigate the distribution of biological contaminants is needed because indoor temperature and relative humidity are comparatively high.     

Indoor aerosols: from personal exposure to risk assessment

Motivated by growing considerations of the scale, severity, and risks associated with human exposure to indoor particulate matter, this work reviewed existing literature to: (i) identify state‐of‐the‐art experimental techniques used for personal exposure assessment; (ii) compare exposure levels reported for domestic/school settings in different countries (excluding exposure to environmental tobacco smoke and particulate matter from biomass cooking in developing countries); (iii) assess the contribution of outdoor background vs indoor sources to personal exposure; and (iv) examine scientific understanding of the risks posed by personal exposure to indoor aerosols. Limited studies assessing integrated daily residential exposure to just one particle size fraction, ultrafine particles, show that the contribution of indoor sources ranged from 19% to 76%. This indicates a strong dependence on resident activities, source events and site specificity, and highlights the importance of indoor sources for total personal exposure. Further, it was assessed that 10–30% of the total burden of disease from particulate matter exposure was due to indoor‐generated particles, signifying that indoor environments are likely to be a dominant environmental factor affecting human health. However, due to challenges associated with conducting epidemiological assessments, the role of indoor‐generated particles has not been fully acknowledged, and improved exposure/risk assessment methods are still needed, together with a serious focus on exposure control.     

Study of mutagenic pollution in Bombay

Airborne suspended particulate matter (SPM) from seven areas in and around Bombay city were collected over glass fibre filters (0.8 μm porosity). The chemicals from the SPM were extracted in dimethylsulfoxide and distilled water and were further tested for mutagenicity by Ames' test using five mutants of Salmonella typhimurium. Of the seven areas studied, only four exhibited mutagenicity, which was confirmed by dose—response assays using the mutant strain TA 100. The very high mutagenicity observed in central Bombay correlates with the higher incidence of respiratory tract diseases in the resident population.     

Retrieval of suspended particulate matter concentrations in the Danube River from Landsat ETM data

Alternations in river channel morphology result in a disturbed natural transport of suspended particulate matter (SPM). Suspended particulate matter serves as a transport medium for various pollutants, e.g. heavy metals. It is therefore important to understand how artificial obstructions alter the natural transport of suspended matter. Measurements of SPM in rivers are traditionally carried out during in situ sampling campaigns, which can provide only a limited view of the actual spatial distribution of suspended matter over large distances. Several authors have studied how space-borne remote sensing could be used for mapping of water quality in standing waters, but with only little attention paid to rivers. This paper describes the methodology how a Landsat ETM image was used to map the spatial patterns of SPM in the Slovak portion of the Danube River. Results of our investigation reveal that the Danube River in Slovakia exhibits gradual longitudinal decrease in concentrations of SPM. Based on a strong relationship between the Landsat near-infrared band (TM4) and field measurements, we developed a map of suspended particulate matter in the Danube River with a standard error (SE) of 2.92 mg/L. This study aims to show how archived satellite data and historical water quality data can be used for monitoring of SPM in large rivers. A methodology describing the minimum samples required for sufficiently accurate results is discussed in this paper also.     

住宅室内细颗粒物质量浓度及预测研究

选取哈尔滨某住宅,监测室内(以客厅为主要研究对象)细颗粒物质量浓度与人员活动情况,分析外窗渗透、外窗渗透+厨房炊事条件下客厅细颗粒物质量浓度的变化.建立室内细颗粒物质量浓度预测模型,结合实测数据对预测效果进行验证.实测结果表明:总体上客厅细颗粒物质量浓度均低于室外,且客厅细颗粒物质量浓度与室外细颗粒物质量浓度的变化趋势...     

Indoor air quality for chemical and ultrafine particle contaminants from printers

There are various emission sources of chemical contaminants, such as volatile organic compounds (VOCs) and ozone and particulate matter. This report is a study into the indoor air of a room containing either a laser printer/ink-jet printer, and the air contaminations were monitored for VOCs, ozone and ultrafine particle. The result confirmed an increase in the concentration of ozone and ultrafine particle numbers in the printing processes of the printer. The emission of VOCs and ozone were measured by the use of a test chamber. The chamber concentrations of styrene, xylenes and ozone were increased in printing process of the laser printer, and pentanol was detected from the ink-jet printer. The results suggest that an office or residential printer may be a source of indoor air contamination. It is necessary for emission from printers to monitor not only VOCs and particle but also ultrafine particles and other contaminants in indoor air.     

Correlations, partitioning and bioaccumulation of heavy metals between different compartments of Lake Balaton

Correlations between trace metals in dissolved and particulate phases, zooplankton, mussels and sediments in Lake Balaton were investigated. The degree of correlation between the various metals was different in each of the investigated compartments. Particulate metal concentrations (microg g(-1)) were anti-correlated with suspended particulate matter (SPM) (mg l(-1)), indicating a dilution effect, while total metal concentrations in the water column (microg l(-1)) were highly correlated with SPM, implying a major influence of the turbidity on the total metal concentrations. Between compartments, not many significant correlations were recognized. Only Ba, Ca, Sr and Mg are correlated in the sediments and in the particulate phase, suggesting common sources for both compartments. Partitioning coefficients (Kd) of trace metals between dissolved and particulate phases are generally low, typical for natural water and fairly stable over the lake. Most of the trace metals (Zn, Co, Cd and Pb) exist in the particulate phase (for about 70% of the total metal load). Cu and Ni are exceptions, showing a more equal distribution. Bioconcentration factors (BCF) of zooplankton and mussels were comparable to those of other natural waters. A negative biomagnification from suspended particulate matter to zooplankton and from sediment to mussel was recognized for all trace metals, except a small enrichment of Zn in zooplankton and Cd in mussel. Four factors were recognized in SPM and in sediments but they did not contain the same group of metals. Cluster analysis showed that metal accumulations in the sediments were different between northern and southern shores and in SPM between western and eastern areas.     

Characterisation of urban catchment suspended particulate matter (Auckland region, New Zealand); a comparison with non-urban SPM

Suspended particulate matter (SPM) is an important transport agent for metal contaminants in streams, particularly during high flow periods such as storm events. For highly contaminated urban catchments in the greater Auckland (New Zealand) area, trace metal partitioning between the dissolved phase and SPM was determined, and SPM characterised in terms of its Si, Al, Fe, Mn, Zn, Cu, Pb, TOC, TON and PO(4) concentrations, as well as particle size, abundance, type and surface area. This data was compared to similar data from representative non-urban catchments in the Auckland region, the Kaipara River and Waikato River catchments, to identify any significant differences in the SPM and its potential trace metal adsorption capacity. Trace metal partitioning was assessed by way of a distribution coefficient: K(D)=[Me(SPM)]/[Me(DISS)]. Auckland urban SPM comprises quartz, feldspars and clay minerals, with Fe-oxides and minor Mn-oxides. No particles of anthropogenic origin, other than glass shards, were observed. No change in urban SPM particle size or SSA was observed with seasonal change in temperature, but the nature of the SPM was observed to change with flow regime. The abundance of finer particles, SSA and Al content of the SPM increased under moderate flow conditions; however, Si/Al ratios remained constant, confirming the importance of aluminosilicate detrital minerals in surface run-off. The SPM Fe content was observed to decrease with increased flow and was attributed to dilution of SPM Fe-oxide of groundwater origin. The Kaipara River SPM was found to be mineralogically, chemically and biologically similar to the urban SPM. However, major differences between urban catchment SPM and SPM from the much larger (non-urban) Waikato River were observed, and attributed to a higher abundance of diatoms. The Fe content of the Waikato River SPM was consistently lower (<5%), and the Si/Al ratio and Mn content was higher. Such differences observed between urban and non-urban SPM did not appear to affect the partitioning of Zn and Cu; however, Pb in the Kaipara and Waikato Rivers was found to be more associated with the dissolved phase. This is likely to reflect higher particulate Pb inputs to urban systems.     

The Influence of Human Activity on the Vertical Distribution of Airborne Particle Concentration in Confined Environments: Preliminary Results

Abstract Vertical concentration profiles for various size fractions of airborne particulate matter have been measured in a nonsmoking indoor environment used mainly as a meeting point during coffee break (11.00 a.m.) and tea time (4.00 p.m.). This monitoring exercise was carried out using a novel sampling system specifically designed for measuring concentration gradients of airborne particles (but which can be easily modified for gaseous pollutants) over the first three metres from ground. The results show substantial gradients in concentration, with the highest occurring at around 1.3 m height. A plausible explanation for the measured time series of concentration at different levels from ground, and the vertical distribution of concentration, is thought to be human movement and activity in the confined environment. The implications that the results of this experiment have for indoor air quality standards for airborne particulate matter are discussed.     

Would removing indoor air particulates in children's environments reduce rate of absenteeism--a hypothesis.

To conduct a controlled trial to test the ability of a newly developed electrostatic air cleaning technology (EAC) to improve Indoor Air Quality (IAQ) as defined by levels of airborne particles and to investigate the potential to reduce non-attendance rates due to illness among children in two Swedish day care centres. The EAC technology was shown to significantly reduce the indoor particulate load for very fine particles caused by outdoor air pollution by 78% and to reduce the number of fine particles produced indoors by 45%. To test the hypothesis, non-attendance was followed in two centres during 3 years. The EAC technology was in operation during year 2. Non-attendance rates among children in the larger day-care centre decreased by 55%, equalling those levels noted in family-based day care. It is speculated that the air cleaning effect may be due to alterations in electrostatic forces operating within the room enabling fine particulate matter to more easily become and stay airborne. The EAC technology is cost-efficient and might be a way forward to improve IAQ.     

Airborne particulate matter and gaseous air pollutants in residential structures in Lodi province, Italy

The province of Lodi is located in northern Italy on the Po River plain, where high background levels of air pollutants are prevalent. Lodi province is characterized by intensive agriculture, notably animal husbandry. This paper assesses indoor levels of selected airborne pollutants in 60 homes in the province, with special attention to size-fractionated particulate matter (PM). Indoor PM?.? concentrations are frequently higher than current guidelines. PM?? and nitrogen dioxide also exceed the respective guideline recommendations in some cases, noting that 24-h nitrogen dioxide levels were compared with an annual limit value. All other studied pollutant levels are below current international guidelines. Among indoor PM size fractions, PM?.? is predominant in terms of mass concentrations corresponding to 57% of PM?? in summer and 71% in winter. A strong seasonal trend is observed for all studied pollutants, with higher levels in winter corresponding to changes in ambient concentrations. The seasonal variation in PM?? is largely due to PM?.? increase from summer to winter. Summer indoor PM levels are mainly from indoor-generated particles, while particles of outdoor origin represent the main contribution to winter indoor PM levels. On average, indoor concentrations of coarse PM are mostly constituted by indoor-generated particles. PRACTICAL IMPLICATIONS: This study presents a comparison between measured indoor concentrations in the study area and indoor air quality guideline criteria. Accordingly, particulate matter (PM) and NO? are identified as key pollutants that may pose health concerns. It is also found that indoor PM in residential units is mainly constituted by particles with aerodynamic diameters <0.5 μm, especially in winter. Risk mitigation strategies should be focused on the reduction in indoor levels of NO? and ultrafine and fine particles, both infiltrated from outdoors and generated by indoor sources.     

室内颗粒物的来源和特点研究

分析了国内外在室内颗粒物的来源和室内外颗粒源对室内颗粒物浓度的影响方面的研究进展。指出了目前研究中存在的问题,并对未来的研究方向进行了展望。     

Relation between Indoor and Outdoor Exposure to Fine Particles near a Busy Arterial Road

Abstract Various studies on indoor and outdoor particulate matter in the urban environment in the vicinity of busy arterial roads in the centre of the subtropical city of Brisbane have indicated that the revised United States Environmental Protection Agency National Ambient Air Quality Standards (US EPA NAAQS) for Particulate matter PM_2.5 could be exceeded not only outdoors but also indoors. The aim of this work was to investigate outdoor exposure to submicrometer particles and their relationship with indoor exposure in a hypothetical office building located in the vicinity of a busy arterial road. The outdoor exposure values and trends were measured in terms of particle number in the submicrometer size range and were then recalculated to represent mass concentration trends. The results of this study indicate that exposure to PM_0.7 particles in ambient air close to a busy road often exceeds the levels of the annual and 24-hour US EPA NAAQS PM_2.5 standards. It is likely that exposure to PM_2.5 is even higher, and may significantly exceed these standards.     

Particle size distribution and composition in a mechanically ventilated school building during air pollution episodes

Particle count-based size distribution and PM(2.5) mass were monitored inside and outside an elementary school in Salt Lake City (UT, USA) during the winter atmospheric inversion season. The site is influenced by urban traffic and the airshed is subject to periods of high PM(2.5) concentration that is mainly submicron ammonium and nitrate. The school building has mechanical ventilation with filtration and variable-volume makeup air. Comparison of the indoor and outdoor particle size distribution on the five cleanest and five most polluted school days during the study showed that the ambient submicron particulate matter (PM) penetrated the building, but indoor concentrations were about one-eighth of outdoor levels. The indoor:outdoor PM(2.5) mass ratio averaged 0.12 and particle number ratio for sizes smaller than 1 microm averaged 0.13. The indoor submicron particle count and indoor PM(2.5) mass increased slightly during pollution episodes but remained well below outdoor levels. When the building was occupied the indoor coarse particle count was much higher than ambient levels. These results contribute to understanding the relationship between ambient monitoring station data and the actual human exposure inside institutional buildings. The study confirms that staying inside a mechanically ventilated building reduces exposure to outdoor submicron particles. PRACTICAL IMPLICATIONS: This study supports the premise that remaining inside buildings during particulate matter (PM) pollution episodes reduces exposure to submicron PM. New data on a mechanically ventilated institutional building supplements similar studies made in residences.     

Organic compound characterization and source apportionment of indoor and outdoor quasi-ultrafine particulate matter in retirement homes of the Los Angeles Basin

Abstract Quasi‐ultrafine (quasi‐UF) particulate matter (PM_0.25) and its components were measured in indoor and outdoor environments at four retirement communities in Los Angeles Basin, California, as part of the Cardiovascular Health and Air Pollution Study (CHAPS). The present paper focuses on the characterization of the sources, organic constituents and indoor and outdoor relationships of quasi‐UF PM. The average indoor/outdoor ratios of most of the measured polycyclic aromatic hydrocarbons (PAHs), hopanes, and steranes were close to or slightly lower than 1, and the corresponding indoor–outdoor correlation coefficients (R) were always positive and, for the most part, moderately strong (median R was 0.60 for PAHs and 0.74 for hopanes and steranes). This may reflect the possible impact of outdoor sources on indoor PAHs, hopanes, and steranes. Conversely, indoor n‐alkanes and n‐alkanoic acids were likely to be influenced by indoor sources. A chemical mass balance model was applied to both indoor and outdoor speciated chemical measurements of quasi‐UF PM. Among all apportioned sources of both indoor and outdoor particles, vehicular emissions was the one contributing the most to the PM_0.25 mass concentration measured at all sites (24–47% on average).

Practical Implications

Although people (particularly the elderly retirees of our study) generally spend most of their time indoors, a major portion of the PM_0.25 particles they are exposed to comes from outdoor mobile sources. This is important because, an earlier investigation, also conducted within the Cardiovascular Health and Air Pollution Study (CHAPS), showed that indoor‐infiltrated particles from mobile sources are more strongly correlated with adverse health effects observed in the elderly subjects living in the studied retirement communities compared with other particles found indoors ( Delfino et al., 2008 ).     

室内颗粒物分布运动研究及进展

针对室内的颗粒物质与室内空气品质（IAQ）有着密切关系的现状,概述了目前室内颗粒物运动分布的研究方法,分析了室内颗粒物特殊行为研究现状,在评述各方法的优缺点和分析目前存在问题的基础上,提出了今后的发展方向。     

Human exposure to air contaminants in sports environments

The aim of this review was to investigate human exposure to relevant indoor air contaminants, predictors affecting the levels, and the means to reduce the harmful exposure in indoor sports facilities. Our study revealed that the contaminants of primary concern are the following: particulate matter in indoor climbing, golf, and horse riding facilities; carbon dioxide and particulate matter in fitness centers, gymnasiums, and sports halls; Staphylococci on gymnasium surfaces; nitrogen dioxide and carbon monoxide in ice hockey arenas; carbon monoxide, nitrogen oxide(s), and particulate matter in motor sports arenas; and disinfection by-products in indoor chlorinated swimming pools. Means to reduce human exposure to indoor contaminants include the following: adequate mechanical ventilation with filters, suitable cleaning practices, a limited number of occupants in fitness centers and gymnasiums, the use of electric resurfacers instead of the engine powered resurfacers in ice hockey arenas, carefully regulated chlorine and temperature levels in indoor swimming pools, properly ventilated pools, and good personal hygiene. Because of the large number of susceptible people in these facilities, as well as all active people having an increased respiratory rate and airflow velocity, strict air quality requirements in indoor sports facilities should be maintained.     

Numerical investigation of airflow pattern and particulate matter transport in naturally ventilated multi-room buildings

This study reports on a numerical investigation of transport behavior of indoor airflow and size-dependent particulate matter (PM) in multi-room buildings. An indoor size-dependent PM transport approach, combining the Eulerian large-eddy simulation of turbulent flow with the Lagrangian particle trajectory tracking, was developed to investigate indoor airflow pattern and PM1/PM2.5/PM10 removal efficiency in naturally ventilated multi-room buildings. A displacement ventilation with a measured indoor PM10 profile in Taipei Metropolis as the initial condition was carried out to characterize spatial and temporal variations of indoor PM1/PM2.5/PM10 removal behavior. The effects of indoor airflow pattern on particle transport mechanisms, e.g., deposition, suspension, migration and escape, were analyzed. Two comparison scenarios, which considered the effects of no indoor partition and different air change rate, respectively, were also conducted. In comparison with the effectiveness of PM1/PM2.5/PM10 removal, the simulated results showed that coarse particles were easier to be removed out of the building than fine particles. Natural ventilation was not an effective way to remove fine particles such as PM1 and PM2.5 in a multi-room building. Indoor partitions can impede 12% of the mean streamwise velocities and significantly increase 30-50% turbulence intensities. However, indoor partitions increased particle deposition and decreased particle escape. As a result of the two opposite particle removal mechanisms, i.e., deposition and escape, the impact of indoor partitions on PM1/PM2.5/PM10 removal behavior was not as significant as the results of airflow velocities. PRACTICAL IMPLICATIONS: This work developed a computational fluid dynamics technique to investigate indoor airflow patterns and PM1/PM2.5/PM10 removal ability in ventilated multi-room buildings. The results of this paper can help to identify adequate PM1/PM2.5/PM10 cleaning procedure and provide useful size-dependent PM control strategy in multi-room buildings.