金属原子二维平面蒸发动力学过程研究

从由Ｂｏｌｔｚｍｍａｎ方程来的ＢＧＫ方程发出,数值模拟长槽型坩埚二维平面蒸发动学过程,着重对分离器中加入精料收集板,贫料收集板和热离子收集板时蒸气原子的空间物理特征进行数值模拟和分析,并对收集板的吸收率和温度以及Ｋｎ变化时,蒸气原子的空间物理特性进行了分析。     

考虑共振电荷转移的二维等离子体离子收集过程

对考虑了共振电荷转移碰撞过程的二维ＡＶＬＩＳ离子引出收集问题进行了数值模拟，分析结果表明：碰撞主要发生在鞘层中；影响碰撞损失率的主要因素是极板间距，应选择小于３ｃｍ的收集板间距；离子引出时间不是判断碰撞损失率的标准。     

Numerical Simulation for Metastable States' Deexcitation in Electron Beam Evaporation Process

A direct simulation Monte Carlo (DSMC) method was modified in order to analyze the evaporation process in atomic vapor laser isotope separation (AVLIS), whereby energy transfer between discrete energy levels of metastable states and continuous energy level of translation took place. The atomic excitation temperatures of gadolinium atom were calculated for the model in five low-lying states. Calculation results were compared with those of the experiments obtained by laser absorption spectroscopy. Two types of DSMC simulations which were different in inelastic collision procedures were carried out. It was concluded that the energy transfer was forbidden unless the total energy of the colliding atoms exceeded a threshold value. It was also found that the DSMC method is suitable for treating deexcitation of metastable states accompanied by rapid expansion in the AVLIS evaporation process.     

Calculation of Electron Swarm Parameters of SF6/N2 in a Uniform Field Using an Improved Monte Carlo Collision Simulation Method

The electron swarm parameters of SF6/N2 are calculated in the present study using an improved Monte Carlo collision simulation method （MCS）. And some improved sampling techniques are also adopted. The simulation results show that the improved simulation method can provide more accurate results.     

Velocity Distributions in High Density Gadolinium Atomic Beam Produced with Axial Electron Beam Gun

The parallel and perpendicular velocity distributions of a gadolinium atomic beam produced with an axial electron beam gun have been measured by a Doppler-shift technique and a Doppler limited absorption spectroscopy, respectively. The atomic density of 10¹⁸~10¹⁹atoms/m³ at a laser irradiated zone was sufficient for the process, such as an atomic vapor laser isotope separation. The atomic beam velocity of 800 m/s was obtained by a free expansion near an evaporation surface. This velocity, however, was 100 m/s slower than that we had measured with a magnetic transverse electron beam gun in a previous experiment. The reasons for the slower velocity in this experiment than that in the previous one are discussed. In keeping with the deposition rate, the parallel translational temperature rapidly decreased to 200 K, while the perpendicular translational temperature gradually increased and approached to the parallel translational temperature. This result suggested that the collisional region where both translational temperatures are equal extended to the laser irradiated zone in high-rate evaporations.     

Numerical analysis of highly efficient laser-based method of radioactive Cs isotope separation utilizing light-induced drift in D1 and D2 transitions in rare gases

We investigated the feasibility of separating radioactive Cs isotopes using the effects of light-induced drift (LID). LID is the massive flow of particles caused by the difference between the collision frequencies of the buffer particles in the optically connected ground and excited states. We numerically evaluated the LID velocities of Cs-133, Cs-135, and Cs-137 in rare gases based on the currently available experimental technologies. The calculations were performed utilizing the steady-state analytical model and assuming that all of the collisions were strong. The velocity-dependent collision cross-sections were estimated using the WKB approximation with the recently developed ab initio atom–atom interaction potentials. A maximum velocity of more than 10 m/s was obtained when He was utilized as the buffer gas, and the expected maximum annual throughput was approximately 600 g, which is sufficient for practical purposes. We also examined the negative effects that were neglected in the employed model.     

Angular Distribution of Gadolinium Vapor Produced by Electron Beam Heating

Static corrosion tests were performed for the glass phase of a simulated waste form of non-combustible radioactive low-level waste to study a basic aqueous corrosion behavior. The waste form, which was fabricated from simulated waste sample by use of in-can type induction-heated melting, consists of two separated phases; a glass phase and a metal phase. Tests were performed for the glass phase from two types of the waste form with different chemical composition at 35°C and S/V ratio of 2,600 m^?1. The glass phase with both types showed an incongruent dissolution similar to conventional high-level radioactive waste (HLW) glasses, i.e., the normalized elemental mass loss (NL_i) for soluble elements such as B and Na continued to increase after the saturation of insoluble elements such as Si, A1 and Ca. The NL_i for B increased in proportion to the square root of time except for early stage, which suggests that the rate of the long-term dissolution or alteration may be controlled by a diffusion process. Potential secondary phases forming as the results of incongruent dissolution were estimated to be kaolinite and calcite by comparison of the measured solution data with the thermodynamically calculated phase stability relationships. These results suggest that the glass phase has a potential chemical durability not so different from conventional HLW glasses.     

Ion Extraction Characteristics from Photoionized Plasma by Radio-Frequency Resonance Method

In order to raise ion extraction efficiency in laser isotope separation, we have developed a radio-frequency (rf) resonance method. Then, to confirm feasibility of this method to a photoionized plasma, we experimentally studied the ion extraction characteristics.

When the rf frequency was swept under a weak magnetic field (5mT), the plasma-sheath resonance was found to occur at about 12MHz which was almost the same value as the theoretical one. Moreover, it was confirmed that the ion extraction time at the resonance frequency became the minimum.

When the magnetic field strength decreased from 5mT to zero, the ion extraction time became long. From the simulation results, this was because the plasma potential decreased with the magnetic field strength. Therefore, a magnetic field strength of more than 1mT was required to obtain a sufficient ion extraction efficiency.

To obtain the same extraction time as when applying a ?3kV dc voltage in the electrostatic method, the rf resonance method needed a voltage more than 70V_rms, in which the dc bias was ?1kV. Therefore, we confirmed that this method is feasible for the ion extraction from the photoionized plasma.     

New Sampling Method in Continuous Energy Monte Carlo Calculation for Pebble Bed Reactors

A pebble bed reactor generally has double heterogeneity consisting of two kinds of spherical fuel element. In the core, there exist many fuel balls piled up randomly in a high packing fraction. And each fuel ball contains a lot of small fuel particles which are also distributed randomly. In this study, to realize precise neutron transport calculation of such reactors with the continuous energy Monte Carlo method, a new sampling method has been developed. The new method has been implemented in the general purpose Monte Carlo code MCNP to develop a modified version MCNP-BALL. This method was validated by calculating inventory of spherical fuel elements arranged successively by sampling during transport calculation and also by performing criticality calculations in ordered packing models. From the results, it was confirmed that the inventory of spherical fuel elements could be reproduced using MCNP-BALL within a sufficient accuracy of 0.2%. And the comparison of criticality calculations in ordered packing models between MCNP-BALL and the reference method shows excellent agreement in neutron spectrum as well as multiplication factor.

MCNP-BALL enables us to analyze pebble bed type cores such as PROTEUS precisely with the continuous energy Monte Carlo method.