Multifilter rotating shadowband radiometer calibration for spectral aerosol optical depth retrievals over S?o Paulo City, Brazil

Multifilter rotating shadowband radiometer (MFRSR) calibration values for aerosol optical depth (AOD) retrievals were determined by means of the general method formulated by Forgan [Appl. Opt.33, 4841 (1994)] at a polluted urban site. The obtained precision is comparable with the classical method, the Langley plot, applied on clean mountaintops distant of pollution sources. The AOD retrieved over S?o Paulo City with both calibration procedures is compared with the Aerosol Robotic Network data. The observed results are similar, and, except for the shortest wavelength (415 nm), the MFRSR's AOD is systematically overestimated by approximately 0.03.     

Retrieval of the ultraviolet aerosol optical depth during a spring campaign in the Bavarian Alps

A measurement campaign was organized in March 1999 in the Bavarian Alps as part of the European project, Characteristics of the UV Radiation Field in the Alps (CUVRA), to analyze the effect of altitude, aerosols, and snow cover on ground-level UV spectral irradiance. We present the results of simultaneous measurements of aerosol optical depth (AOD) made at various sites on two cloudless days in March 1999. The two days exhibited different aerosol conditions. Results derived from spectral measurements of UV irradiance are compared with data from filter radiometer measurements made at discrete wavelengths extending from the UV to the near IR. The different methods generated values for the AOD that were in good agreement. This result confirms that one can use either method to retrieve the AOD with an uncertainty of approximately 0.03-0.05. On 18 March, high turbidity was observed at low altitude (400-nm AOD approximately 0.5 at 700 m above sea level), and the AOD decreased regularly with altitude; on 24 March, the turbidity was much less (0.11 at 700 m above sea level). On both days very low AODs (0.05-0.09) were measured at 3000 m above sea level. The spectral dependence of the AOD is often parameterized by the angstrom relationship; the alpha parameter is generally difficult or impossible to retrieve from spectral measurements because of the relatively narrow wavelength range (320-400 nm), and only one of the spectro-radiometers used during the campaign permits this retrieval. In most cases, during this field campaign, alpha was found by filter sunphotometers to be 1.1-1.5.     

Wavelength Dependence of Backscatter by use of Aerosol Microphysics and Lidar Data Sets: Application to 2.1- mum Wavelength for Space-Based and Airborne Lidars

An aerosol microphysics dataset was used to model backscatter in the 0.35-11-mum wavelength range, with the results validated by comparison with measured cw and pulsed lidar backscatter obtained during two NASA-sponsored airborne field experiments. Different atmospheric features were encountered, with aerosol backscatter ranging over 4 orders of magnitude. Modeled conversion functions were used to convert existing lidar backscatter datasets to 2.1 mum. Resulting statistical distribution shows the midtropospheric aerosol backscatter background mode of beta(2.1) to be between ~3.0 x 10(-10) and ~1.3 x 10(-9) m(-1) sr(-1), ~10-20 times higher than that for beta(9.1); and a beta(2.1) boundary layer mode of ~1.0 x 10(-7) to ~1.3 x 10(-6) m(-1) sr(-1), ~3-5 times higher than beta(9.1).     

合肥地区气溶胶光学特性的地基观测研究

利用自主研制的DTF-5型太阳辐射计观测合肥地区2008年10月—2010年5月的太阳直接辐射消光,反演合肥地区气溶胶光学厚度、Angstrom参数和沙尘天气过程中的粒子谱分布,并对结果进行分析。结果表明:合肥地区气溶胶光学厚度季节变化除气候因素外,受人为因素影响明显,季节变化规律复杂。总体上秋季较小,冬春季节持续增大,夏季较平稳。而Angstrom参数与气溶胶光学厚度大致呈反相关,秋冬上升,春季骤降,夏季平稳值较大。气溶胶光学厚度日变化大致可分为4种类型:日变化相对稳定;整体呈上升趋势;整体呈下降趋势;一日内出现一到多个峰值。其中第四种类型出现几率最大。沙尘天气过程中,气溶胶光学厚度和Angstrom参数分别呈现出"谷-峰-谷"、"峰-谷-峰"的变化规律,其中Angstrom参数在沙尘影响严重时甚至出现负值。半径为0.2~1.0μm的大粒子和大于1.0μm的巨粒子浓度在沙尘天气过程中大幅增加。     

Vertical variability of aerosol backscatter from an airborne-focused continuous-wave CO2 lidar at 9.1-microm wavelength

Atmospheric aerosol backscatter measurements taken with a continuous-wave focused Doppler lidar at 9.1-mum wavelength were obtained over western North America and the Pacific Ocean from 13 to 26 September 1995 as part of a NASA airborne mission. Backscatter variability was measured for ~52 flight hours, covering an equivalent horizontal distance of ~30,000 km in the troposphere. Some quasi-vertical backscatter profiles were also obtained during various ascents and descents at altitudes that ranged from ~0.1 to 12 km. Similarities and differences for aerosol loading over land and ocean were observed. A midtropospheric aerosol backscatter background mode near 3 x 10(-11) to 1 x 10(-10) m(-1) sr(-1) was obtained, which is consistent with those of previous airborne and ground-based data sets.     

Seeded femtosecond optical parametric amplification in the mid-infrared spectral region above 3 mum

Femtosecond optical parametric amplification that results in microjoule mid-infrared pulses at wavelengths exceeding 3 mum is demonstrated. Narrow-band quasi-cw seeding at the signal wavelength is applied to ensure the generation of nearly transform-limited femtosecond pulses at the idler wavelength. The broad bandwidth of the parametric amplification provided by pumping with femtosecond pulses from a Ti:sapphire regenerative amplifier at high intensity results in idler pulse durations shorter than the pump pulse length. The potentials of three nonlinear optical crystals that belong to the potassium titanyl phosphate family are comparatively studied. At 1-kHz repetition rate our all-solid-state system produces highly synchronized ~100-fs pulses in the spectral range between 3 and 4 mum.     

Multiply scattered aerosol lidar returns: inversion method and comparison with in situ measurements

A novel aerosol lidar inversion method based on the use of multiple-scattering contributions measured by a multiple-field-of-view receiver is proposed. The method requires assumptions that restrict applications to aerosol particles large enough to give rise to measurable multiple scattering and depends on parameters that must be specified empirically but that have an uncertainty range of much less than the boundary value and the backscatter-to-extinction ratio of the conventional single-scattering inversion methods. The proposed method is applied to cloud measurements. The solutions obtained are the profiles of the scattering coefficient and the effective diameter of the cloud droplets. With mild assumptions on the form of the function, the full-size distribution is estimated at each range position from which the extinction coefficient at any visible and infrared wavelength and the liquid water content can be determined. Typical results on slant-path-integrated optical depth, vertical extinction profiles, and fluctuation statistics are compared with in situ data obtained in two field experiments. The inversion works well in all cases reported here, i.e., for water clouds at optical depths between ~0.1 and ~4.     

Computationally efficient method for retrieving aerosol optical depth from ATSR-2 and AATSR data

We present a robust and computationally efficient method for retrieving aerosol optical depth (AOD) from top-of-atmosphere ATSR-2 (Along-Track Scanning Radiometer) and AATSR (Advanced ATSR) reflectance data that is formulated to allow retrieval of the AOD from the 11 year archive of (A)ATSR data on the global scale. The approach uses a physical model of light scattering that requires no a priori information on the land surface. Computational efficiency is achieved by using precalculated lookup tables (LUTs) for the numerical inversion of a radiative-transfer model of the atmosphere. Estimates of AOD retrieved by the LUT approach are tested on AATSR data for a range of global land surfaces and are shown to be highly correlated with sunphotometer measurements of the AOD at 550 nm. (Pearson's correlation coefficient r(2) is 0.71.).     

Solar corona caused by juniper pollen in Texas

Coronas are colorful, concentric rings centered on a bright light such as the Sun, the Moon, or even a streetlamp. Coronas are most commonly caused by water droplets or ice particles of relatively uniform size. Observers in Finland have reported spectacular clear-sky coronas caused by pollen grains. A clear-sky corona in central Texas occurred during the peak of the juniper pollinating season. The aerosol optical thickness at each of three wavelengths was highest when the corona was most prominent. Photographic measurements of the corona infer a particle diameter of ~32.4 mum. Because juniper pollen grains have a diameter of from 22 to 30 mum, they are the aerosol most likely to have caused the corona.     

Microphysical particle parameters from extinction and backscatter lidar data by inversion with regularization: experiment

We present effective radius, volume, surface-area, and number concentrations as well as mean complex refractive index of tropospheric particle size distributions based on lidar measurements at six wavelengths. The parameters are derived by means of an inversion algorithm that has been specifically designed for the inversion of available optical data sets. The data were taken on 20 June and on 20 July 1997 during the Aerosol Characterization Experiment ACE 2 (North Atlantic/Portugal) and on 9 August 1998 during the Lindenberg Aerosol Characterization Experiment LACE 98 (Lindenberg/Germany). Measurements on 20 June 1997 were taken in a clean-marine boundary layer, and a large value of 0.64 mum for the effective radius, a low value of 1.45 for the real part, and a negligible imaginary part of the complex refractive index were found. The single-scatter albedo was 0.98 at 532 nm. It was derived from the particle parameters with Mie-scattering calculations. In contrast, the particles were less than 0.2 mum in effective radius in a continental-polluted aerosol layer on 20 July 1997. The real part of the complex refractive index was ~1.6; the imaginary part showed values near 0.03i. The single-scatter albedo was 0.84. On 9 August 1998 an elevated particle layer located from 3000 to 6000 m was observed, which had originated from an area of biomass burning in northwestern Canada. Here the effective radius was ~0.24 mum, the real part of the complex refractive index was above 1.6, the imaginary part was ~0.04i, and the single-scatter albedo was 0.81. Excellent agreement has been found with results based on sunphotometer and in situ measurements that were performed during the field campaigns.     

Subwavelength-resolvable focused non-gaussian beam shaped with a binary diffractive optical element.

The diffraction-limited spot size limits the optical disk storage capacity and microscopic resolution. We describe a technique to shape a focused Gaussian beam into a superresolving beam by using a diffractive optical element fabricated by laser-assisted chemical etching. The focused shaped beam has a smaller width and a longer depth of focus than a similarly focused Gaussian beam. Using the diffraction-limited shaped beam along with threshold writing, we achieved a written pit size of less than 0.33 mum at a 695-nm laser wavelength, compared with a 0.7-mum focused Gaussian spot size (full width at e(-2) of the peak) with the same focusing lens. The energy conversion efficiency for the beam shaping was ~81%.     

X-ray imaging by angular raster scanning

The technology of x-ray W-Al multilayer mirrors with an angular reflection width of more than 0.4 degrees at a 1.54-A wavelength is developed. On this basis an x-ray scanner is constructed. We show experimentally the possibility of object-transfer imaging with a resolution of ~20 mum.     

Long-wavelength vertical-cavity surface-emitting lasers for high-speed applications and gas sensing

Long-wavelength InGaAlAs-InP vertical-cavity surface-emitting lasers (LW-VCSELs) covering the wavelength range from 1.3 to 2.3 mum are presented. Furthermore, these lasers can be fabricated in a novel high-speed design-reducing parasitics to enable bandwidths in excess of 11 GHz at 1.55 mum. To the best of the authors' knowledge, this is the fastest 1.55 mum VCSEL ever presented. As a proof-of-concept one- and two-dimensional arrays have been fabricated with high yield. All devices use a buried tunnel junction for current confinement and a dielectric backside reflector with integrated electroplated gold-heatsink. This concept enables CW operation at room temperature with typical single-mode output powers above 1 mW. Both, wavelength range and modulation performance, together with VCSEL features such as operation voltage around IV and power consumption as low as 10-20 mW enable applications in tunable diode laser spectroscopy (TDLS) and optical data transmission. Error-free data transmission at 10 Gbit/s over 22 km which can be readily applied in uncooled coarse wavelength division multiplex passive optical networks is presented. A laser hygrometer using a 1.84 mum VCSEL demonstrates the functionality of TDLS systems with VCSELs.     

Degree of linear polarization in spectral radiances from water-viewing infrared radiometers

Infrared radiances from water become partially polarized at oblique viewing angles through both emission and reflection. I describe computer simulations that show how the state of polarization for water varies with environmental conditions over a wavelength range of 3-15 mum with 0.05-mum resolution. Polarization at wavelengths longer than approximately 4 mum generally is negative (p, or vertical) and increases with incidence angle up to approximately 75 degrees , beyond which the horizontally polarized reflected atmospheric radiance begins to dominate the surface emission. The highest p polarization (~4-10%) is found in the atmospheric window regions of approximately 4-5 and 8-14 mum. In the 3-5-mum spectral band, especially between 3 and 4 mum, reflected atmospheric radiance usually is greater than surface emission, resulting in a net s polarization (horizontal). The results of these simulations agree well with broadband measurements of the degree of polarization for a water surface viewed at nadir angles of 0-75 degrees .     

Aerosol and cloud backscatter at 1.06, 1.54, and 0.53 mum by airborne hard-target-calibrated Nd:YAG /methane Raman lidar

A lidar instrument was developed to make simultaneous measurements at three distinct wavelengths in the visible and near infrared at 0.532, 1.064, and 1.54 mum with high cross-sectional calibration accuracy. Aerosol and cloud backscatter cross sections were acquired during November and December 1989 and May and June 1990 by the NASA DC-8 aircraft as part of the Global Backscatter Experiment. The instrument, methodology, and measurement results are described. A Nd:YAG laser produced 1.064- and 0.532-mum energy. The 1.54-mum transmitted pulse was generated by Raman-shifted downconversion of the 1.064-mum pulse through a Raman cell pressured with methane gas. The lidar could be pointed in the nadir or zenith direction from the aircraft. A hard-target-based calibration procedure was used to obtain the ratio of the system calibration between the three wavelengths, and the absolute calibration was referenced to the 0.532-mum lidar molecular backscatter cross section for the clearest scattering regions. From the relative wavelength calibration, the aerosol backscatter cross sections at the longer wavelengths are resolved for values as small as 1% of the molecular cross section. Backscatter measurement accuracies are better than 10(-9) (m sr)(-1) at 1.064 and 1.54 mum. Results from the Pacific Ocean region of the multiwavelength backscatter dependence are presented. Results show extensive structure and variation for the aerosol cross sections. The range of observed aerosol cross section is over 4 orders of magnitude, from less than 10(-9) (m sr)(-1) to greater than 10(-5) (m sr)(-1).     

Fabrication of thin-film micropolarizer arrays for visible imaging polarimetry

We describe a microfabrication process for fabricating micropolarizer devices with polarization thin film. The polarization film is less than a 0.5 mum thick and can have a polarization extinction ratio of ~330 in the visible wavelength range. A single-state micropolarizer array with polarizing pixels as small as 5 mum x 5 mum has been fabricated. A multilayer spatially multiplexed three-state micropolarizer line array with a 14.4-mum resolution has also been fabricated for visible imaging polarimetry application.     

Multiple-wavelength digital holographic interferometry using tunable laser diodes

Here we present multiple-wavelength digital holographic interferometry with a wide measurement range using laser diodes. Small wavelength differences can be easily realized by the wavelength tuning of laser diodes with injection current controls. A contour map of an object with a wide measurement range and a high sensitivity is demonstrated by combining a few contour maps with several measurement sensitivities. Synthetic wavelengths are calibrated using a known height difference. This alleviates the need to have high precise knowledge of the recording wavelengths. The synthetic wavelengths ranged from ~3 mm for high measurement sensitivity to ~4 cm for wide measurement range. An rms error of ~35 mum for a ~1 cm height measurement is shown. The measured profile of holographic interferometry agrees with a standard stylus instrument.     

Aerosol observations by lidar in the nocturnal boundary layer

Aerosol observations by lidar in the nocturnal boundary layer (NBL) were performed in Potenza, Southern Italy, from 20 January to 20 February 1997. Measurements during nine winter nights were considered, covering a variety of boundary-layer conditions. The vertical profiles of the aerosol backscattering coefficient at 355 and 723.37 nm were determined through a Klett-modified iterative procedure, assuming the extinction-to-backscattering ratio within the NBL has a constant value. Aerosol average size characteristics were retrieved from almost simultaneous profiles of the aerosol backscattering coefficient at 355 and 723.37 nm, the measurements being consistent with an accumulation mode radius not exceeding 0.4 mum. Similar results in terms of aerosol sizes were obtained from measurements of the extinction-to-backscattering ratio profile at 355 nm performed on six nights during the measurement campaign. Backscattering profiles at 723.37 nm were also converted into profiles of aerosol liquid water content.     

Side-line tunable laser transmitter for differential absorption lidar measurements of CO2: design and application to atmospheric measurements

A 2 microm wavelength, 90 mJ, 5 Hz pulsed Ho laser is described with wavelength control to precisely tune and lock the wavelength at a desired offset up to 2.9 GHz from the center of a CO(2) absorption line. Once detuned from the line center the laser wavelength is actively locked to keep the wavelength within 1.9 MHz standard deviation about the setpoint. This wavelength control allows optimization of the optical depth for a differential absorption lidar (DIAL) measuring atmospheric CO(2) concentrations. The laser transmitter has been coupled with a coherent heterodyne receiver for measurements of CO(2) concentration using aerosol backscatter; wind and aerosols are also measured with the same lidar and provide useful additional information on atmospheric structure. Range-resolved CO(2) measurements were made with <2.4% standard deviation using 500 m range bins and 6.7 min? (1000 pulse pairs) integration time. Measurement of a horizontal column showed a precision of the CO(2) concentration to <0.7% standard deviation using a 30 min? (4500 pulse pairs) integration time, and comparison with a collocated in situ sensor showed the DIAL to measure the same trend of a diurnal variation and to detect shorter time scale CO(2) perturbations. For vertical column measurements the lidar was setup at the WLEF tall tower site in Wisconsin to provide meteorological profiles and to compare the DIAL measurements with the in situ sensors distributed on the tower up to 396 m height. Assuming the DIAL column measurement extending from 153 m altitude to 1353 m altitude should agree with the tower in situ sensor at 396 m altitude, there was a 7.9 ppm rms difference between the DIAL and the in situ sensor using a 30 min? rolling average on the DIAL measurement.     

Single-mode optical waveguides fabricated from fluorinated polyimides

Buried channel optical waveguides were fabricated from fluorinated polyimides. They operated in single mode and showed an optical loss of less than 0.3 and 0.7 dB/cm for TE and TM polarizations, respectively, at a wavelength of 1.3 mum. Moreover, these waveguides had high heat and moisture resistance; the optical loss did not significantly change after heating at 380 degrees C for 1 h or after exposure to 85% relative humidity at 85 degrees C for over 200 h.