Versatile mobile lidar system for environmental monitoring

A mobile lidar (light detection and ranging) system for environmental monitoring is described. The optical and electronic systems are housed in a truck with a retractable rooftop transmission and receiving mirror, connected to a 40-cm-diameter vertically looking telescope. Two injection-seeded Nd:YAG lasers are employed in connection with an optical parametric oscillator-optical parametric amplification transmitter, allowing deep-UV to mid-IR wavelengths to be generated. Fast switching that employs piezoelectric drivers allows multiwavelength differential absorption lidar for simultaneous measurements of several spectrally overlapping atmospheric species. The system can also be used in an imaging multispectral laser-induced fluorescence mode on solid targets. Advanced LabVIEW computer control and multivariate data processing render the system versatile for a multitude of measuring tasks. We illustrate the monitoring of industrial atmospheric mercury and hydrocarbon emissions, volcanic sulfur dioxide plume mapping, fluorescence lidar probing of seawater, and multispectral fluorescence imaging of the facades of a historical monument.     

Development of a differential-absorption lidar system for measurement of atmospheric atomic mercury by use of the third harmonic of an LDS-dye laser

A differential-absorption lidar system that uses a long-life transmitter for monitoring of atomic-mercury concentrations in the atmosphere has been developed. The third harmonic of a tunable dye laser with LDS 765 dye pumped by the second harmonic of a Nd:YAG laser was used as the emitted beam from the transmitter. By use of this system, atmospheric concentrations of atomic mercury of less than 0.4 part in 10(12) were measured. The time trend of the measured concentration agreed with that obtained by a conventional gold amalgamation method combined with atomic absorption spectroscopy on the ground.     

探测低空大气温度分布的转动拉曼激光雷达

提出了一种新的探测对流层低层大气温度的转动拉曼激光雷达方法,通过测量N2和O2的后向散射的纯转动拉曼谱的强度,计算它们的比值来确定大气温度的垂直分布,并对其性能进行了数值模拟。转动拉曼激光雷达的光源是一个调Q的Nd:YAG激光器,经扩束器后输出能量200mJ;采用双光栅单色仪提取所需要的氮气和氧气的转动拉曼谱;接收机采用光电倍增管和双通道光子计数器,量子效率是10%(48000个脉冲累加)。夜晚它对近地面10.2km高度内的探测信噪比在10:1以上,白天它对近地面3.6km高度内的探测信噪比在10:1以上,计算的温度与模拟用的温度真值阔线相差约0.3K。     

Lidar measurements taken with a large-aperture liquid mirror. 2. Sodium resonance-fluorescence system

Sodium resonance-fluorescence lidar is an established technique for measuring atmospheric composition and dynamics in the mesopause region. A large-power-aperture product (6.6-W m(2)) sodium resonance-fluorescence lidar has been built as a part of the Purple Crow Lidar (PCL) at The University of Western Ontario. This sodium resonance-fluorescence lidar measures, with high optical efficiency, both sodium density and temperature profiles in the 83-100-km region. The sodium lidar operates simultaneously with a powerful Rayleigh- and Raman-scatter lidar (66 W m(2)). The PCL is thus capable of simultaneous measurement of temperature from the tropopause to the lower thermosphere. The sodium resonance-fluorescence lidar is shown to be able to measure temperature to an absolute precision of 1.5 K and a statistical accuracy of 1 K with a spatial-temporal resolution of 72 (km s) at an altitude of 92 km. We present results from three nights of measurements taken with the sodium lidar and compare these with coincident Rayleigh-scatter lidar measurements. These measurements show significant differences between the temperature profiles derived by the two techniques, which we attribute to variations in the ratio of molecular nitrogen to molecular oxygen that are not accounted for in the standard Rayleigh-scatter temperature analysis.     

Heterodyne lidar returns in the turbulent atmosphere: performance evaluation of simulated systems

Simulations of beam propagation in three-dimensional random media were used to study the effects of atmospheric refractive turbulence on coherent lidar performance. By use of the two-beam model, the lidar return is expressed in terms of the overlap integral of the transmitter and the virtual (backpropagated) local oscillator beams at the target, reducing the problem to one of computing irradiance along the two propagation paths. This approach provides the tools for analyzing laser radar with general refractive turbulence conditions, beam truncation at the antenna aperture, beam-angle misalignment, and arbitrary transmitter and receiver configurations. Simplifying assumptions used in analytical studies, were tested and treated as benchmarks for determining the accuracy of the simulations. The simulation permitted characterization of the effect on lidar performance of the analytically intractable return variance that results from turbulent fluctuations as well as of the heterodyne optical power and system-antenna efficiency.     

Compact airborne lidar for tropospheric ozone: description and field measurements

An airborne lidar has been developed for tropospheric ozone monitoring. The transmitter module is based on a solid-state Nd:YAG laser and stimulated Raman scattering in deuterium to generate three wavelengths (266, 289, and 316 nm) that are used for differential ozone measurements. Both analog and photon-counting detection methods are used to produce a measurement range up to 8 km. The system has been flown on the French Fokker 27 aircraft to perform both lower tropospheric (0.5-4-km) and upper tropospheric (4-12-km) measurements, with a 1-min temporal resolution corresponding to a 5-km spatial resolution. The vertical resolution of the ozone profile can vary from 300 to 1000 m to accommodate either a large-altitude range or optimum ozone accuracy. Comparisons with in situ ozone measurements performed by an aircraft UV photometer or ozone sondes and with ozone vertical profiles obtained by a ground-based lidar are presented. The accuracy of the tropospheric ozone measurements is generally better than 10-15%, except when aerosol interferences cannot be corrected. Examples of ozone profiles for different atmospheric conditions demonstrate the utility of the airborne lidar in the study of dynamic or photochemical mesoscale processes that control tropospheric ozone.     

Scanning lidar with a coupled radar safety system

A small scanning three-wavelength lidar system at NASA Langley Research Center in Hampton, Virginia, has been used since 1992 to make atmospheric measurements on stratospheric and upper tropospheric aerosols and on the evolution of aircraft exhaust plumes. Many of these measurements have been made away from the zenith, and, to reduce the hazard to air traffic produced by the laser beam, a radar safety device has been installed. The radar application is original in that the radar beam is made collinear with the laser beam by use of a dichroic mirror that transmits the laser radiation and reflects the microwaves. This mirror is inserted into the outgoing optical path prior to the radiation from both the radar and the laser passing through the independent scanning unit. Tests of the complete system show that the lidar and radar beams remain collocated as they are scanned and that the radar can be used to inhibit the laser prior to an aircraft passing through the beam.     

Side-line tunable laser transmitter for differential absorption lidar measurements of CO2: design and application to atmospheric measurements

A 2 microm wavelength, 90 mJ, 5 Hz pulsed Ho laser is described with wavelength control to precisely tune and lock the wavelength at a desired offset up to 2.9 GHz from the center of a CO(2) absorption line. Once detuned from the line center the laser wavelength is actively locked to keep the wavelength within 1.9 MHz standard deviation about the setpoint. This wavelength control allows optimization of the optical depth for a differential absorption lidar (DIAL) measuring atmospheric CO(2) concentrations. The laser transmitter has been coupled with a coherent heterodyne receiver for measurements of CO(2) concentration using aerosol backscatter; wind and aerosols are also measured with the same lidar and provide useful additional information on atmospheric structure. Range-resolved CO(2) measurements were made with <2.4% standard deviation using 500 m range bins and 6.7 min? (1000 pulse pairs) integration time. Measurement of a horizontal column showed a precision of the CO(2) concentration to <0.7% standard deviation using a 30 min? (4500 pulse pairs) integration time, and comparison with a collocated in situ sensor showed the DIAL to measure the same trend of a diurnal variation and to detect shorter time scale CO(2) perturbations. For vertical column measurements the lidar was setup at the WLEF tall tower site in Wisconsin to provide meteorological profiles and to compare the DIAL measurements with the in situ sensors distributed on the tower up to 396 m height. Assuming the DIAL column measurement extending from 153 m altitude to 1353 m altitude should agree with the tower in situ sensor at 396 m altitude, there was a 7.9 ppm rms difference between the DIAL and the in situ sensor using a 30 min? rolling average on the DIAL measurement.     

Intrapulse temporal and wavelength shifts of a high-power 2.1-µm Ho:YAG laser and their potential influence on atmospheric lidar measurements

A high-power, flash-lamp-pumped, Q-switched Ho:YAG laser has been developed to produce up to 150 mJ in a 100-ns Q-switched pulse. The Ho laser was initially used in a direct detection lidar-differential absorption lidar (DIAL) system to measure vertical density profiles of aerosols and water vapor in the atmosphere. It was found, however, that the Ho laser operated simultaneously on two closely spaced spectral emission wavelengths (2.090 and 2.097 μm) and that the distribution of energy between the two wavelengths could change significantly on time scales of several seconds to minutes. Such intrapulse temporal and wavelength shifts were found to alter the atmospheric lidar return significantly because one of the laser lines coincided with a water vapor absorption line in the atmosphere. This laser spectral output problem was overcome by the use of intracavity étalons that controlled the laser spectral-temporal characteristics but reduced the laser output energy to approximately 75 mJ/pulse in a 100-ns pulse length. These results are important as they serve to point out the difficulties of developing and using a high-power 2.1- μm Ho laser for atmospheric lidar when high-resolution spectral and temporal characteristics can significantly influence the lidar return and be misinterpreted as resulting from atmospheric signals.     

Precise wavelength control of a single-frequency pulsed Ho:Tm:YLF laser

We demonstrate wavelength control of a single-frequency diode-pumped Ho:Tm:YLF laser by referencing its wavelength to an absorption line of carbon dioxide. We accomplish this wavelength control by injection seeding with a cw Ho:Tm:YLF laser that can be tuned over or stabilized to carbon dioxide or water vapor lines. We show that the pulsed laser can be scanned precisely over an absorption line of carbon dioxide by scanning the injection seed laser wavelength. We locked the pulsed laser to within 18.5 MHz of the absorption line center by stabilizing the injection seed on the line center. The single-frequency pulsed output, intended for use as a transmitter for differential absorption lidar detection of atmospheric carbon dioxide and water vapor and for coherent detection of wind, is 100 mJ per pulse at a 5-Hz repetition rate.     

An a posteriori method based on photo-acoustic cell information to correct for lidar transmitter spectral shift: application to atmospheric CO(2) differential absorption lidar measurements

An a posteriori corrective method based on photo-acoustic cell (PAC) information is proposed to correct for laser transmitter spectral shift during atmospheric CO(2) measurements by 2 microm heterodyne differential absorption lidar (HDIAL) technique. The method for using the PAC signal to retrieve the actual atmospheric CO(2) absorption is presented in detail. This issue is tackled using a weighting function. The performance of the proposed corrective method is discussed and the various sources of error associated with the PAC signal are investigated. For 300 shots averaged and a frequency shift (from the CO(2) absorption line center) lower than the CO(2) absorption line half-width, the relative error on HDIAL CO(2) mixing ratio measurements is lower than 1.3%. The corrective method is validated in absolute value by comparison between HDIAL and in situ sensor measurements of CO(2).     

Compact high-pulse-energy ultraviolet laser source for ozone lidar measurements

An all solid-state Ti:sapphire laser differential absorption lidar transmitter was developed. This all-solid-state laser provides a compact, robust, and highly reliable laser transmitter for potential application in differential absorption lidar measurements of atmospheric ozone. Two compact, high-energy-pulsed, and injection-seeded Ti:sapphire lasers operating at a pulse repetition frequency of 30 Hz and wavelengths of 867 and 900 nm, with M2 of 1.3, have been experimentally demonstrated and their properties compared with model results. The output pulse energy was 115 mJ at 867 nm and 105 mJ at 900 nm, with a slope efficiency of 40% and 32%, respectively. At these energies, the beam quality was good enough so that we were able to achieve 30 mJ of ultraviolet laser output at 289 and 300 nm after frequency tripling with two lithium triborate nonlinear crystals.     

High-spectral-resolution lidar with iodine-vapor filters: measurement of atmospheric-state and aerosol profiles

A high-spectral-resolution lidar can measure vertical profiles of atmospheric temperature, pressure, the aerosol backscatter ratio, and the aerosol extinction coefficient simultaneously. We describe a system with these characteristics. The transmitter is a narrow-band (FWHM of the order of 74 MHz), injection-seeded, pulsed, double YAG laser at 532 nm. Iodine-vapor filters in the detection system spectrally separate the molecular and aerosol scattering and greatly reduce the latter (-41 dB). Operating at a selected frequency to take advantage of two neighboring lines in vapor filters, one can obtain a sensitivity of the measured signal-to-air temperature ratio equal to 0.42%/K. Using a relatively modest size transmitter and receiver system (laser power times telescope aperture equals 0.19 Wm(2)), our measured temperature profiles (0.5-15 km) over 11 nights are in agreement with balloon soundings to within 2.0 K over an altitude range of 2-5 km. There is good agreement in the lapse rates, tropopause altitudes, and inversions. In principle, to invert the signal requires a known density at one altitude, but in practice it is convenient to also use a known temperature at that altitude. This is a scalable system for high spatial resolution of vertical temperature profiles in the troposphere and lower stratosphere, even in the presence of aerosols.     

Remote Raman spectra of benzene obtained from 217 meters using a single 532 nm laser pulse

This report describes a mobile Raman lidar system that has been developed for spectral measurements of samples located remotely at ranges of hundreds of meters. The performance of this system has been quantitatively verified in a lidar calibration experiment using a hard target of standardized reflectance. A new record in detection range was achieved for remote Raman systems using 532 nm laser excitation. Specifically, Raman spectra of liquid benzene were measured with an integration time corresponding to a single 532 nm laser pulse at a distance of 217 meters. The single-shot Raman spectra at 217 meters demonstrated high signal-to-noise ratio and good resolution sufficient for the unambiguous identification of the samples of interest. The transmitter consists of a 20 Hz Nd:YAG laser emitting at 532 nm and 1064 nm and a 178 mm telescope through the use of which allows the system to produce a focused beam at the target location. The receiver consists of a large custom telescope (609 mm aperture) and a Czerny-Turner monochromator equipped with two fast photomultiplier tubes.     

Sum-frequency-generation system for differential absorption lidar measurement of atmospheric nitrogen dioxide

A sum-frequency-generation system for differential absorption lidar measurement of atmospheric nitrogen dioxide in the lower troposphere was developed. The system uses a combination of a pair of KD*P crystals and a tunable dye laser with LDS 765 dye pumped by the second harmonic of a Nd:YAG laser to generate lambdaon and lambdaoff alternatively. Compared with the conventional system that uses Coumarin 445 dye pumped by the third harmonic, the output energy and long-term stability were improved. By use of this system, atmospheric NO2 concentrations of approximately 10-50 ppb were measured, with an instrumental error of approximately 7 ppb.     

Rocketborne Rayleigh lidar for in situ measurements of neutral atmospheric density

We describe the design of a small Rayleigh scattering lidar for launch on a sounding rocket as well as the first, to our knowledge, in situ measurements of neutral number density performed with a rocketborne lidar in the mesosphere. The aim of the experiment is to study the dynamics of the neutral atmosphere with emphasis on turbulent structures and gravity waves. The altitude resolution of the density profile is better than 10 m. The uncertainty is 0.3% below 55 km and better than 1% to an altitude of 65 km. The lidar technique meets the requirement of measurement of total molecular density outside the shock front surrounding the supersonic payload, which is necessary for precision measurements of neutral atmospheric density. We have compared different component technologies and design approaches and show performance calculations for two electro-optical systems. The first system has laser and detector components that were available in 1993, the second has new solutions that became available in 1995. The second system has a signal-to-noise ratio that is five times higher than the first and employs a pulsed high-power laser diode array as the transmitter and a large-area avalanche photodiode as the receiver.     

Injection-seeded pulsed Ti:sapphire laser with novel stabilization scheme and capability of dual-wavelength operation

A gain-switched, single-frequency titanium-sapphire laser for atmospheric humidity measurements using the differential absorption lidar technique operating in the 820 nm wavelength region is described. The laser is pumped by a frequency-doubled, flashlamp-pumped Nd:YAG laser at a repetition rate of 50 Hz and injection seeded by two external-cavity-diode lasers. The system yields pulses with an energy of 15 mJ and high spectral purity. We describe a novel active injection-locking technique that avoids the problems of established methods like dither-lock or ramp-and-fire. Furthermore, our method opens the possibility to switch between two wavelengths for alternating shots, in contrast to most established techniques that only allow operation at one wavelength.     

Improved speckle statistics in coherent differential absorption lidar with in-fiber wavelength multiplexing

Remote detection of gaseous pollutants and other atmospheric constituents can be achieved with differential absorption lidar (DIAL) methods. The technique relies on the transmission of two or more laser wavelengths and exploits absorption features in the target gas by measuring the ratio of their detected powers to determine gas concentration. A common mode of operation is when the transmitter and receiver are collocated, and the absorption is measured over a return trip by a randomly scattering topographic target. Hence, in coherent DIAL, speckle fluctuation leads to a large uncertainty in the detected powers unless the signal is averaged over multiple correlation times, i.e., over many independent speckles. We examine a continuous-wave coherent DIAL system in which the laser wavelengths are transmitted and received by the same single-mode optical fibers. This ensures that the two wavelengths share a common spatial mode, which, for certain transmitter and target parameters, enables highly correlated speckle fluctuations to be readily achieved in practice. For a DIAL system, this gives the potential for improved accuracy in a given observation time. A theoretical analysis quantifies this benefit as a function of the degree of correlation between the two time series (which depends on wavelength separation and target depth). The results are compared with both a numerical simulation and a laboratory-based experiment.     

Cloud-droplet-size distribution from lidar multiple-scattering measurements

A method for calculating droplet-size distribution in atmospheric clouds is presented, based on measurement of laser backscattering and multiple scattering from water clouds. The lidar uses a Nd:YAG laser that emits short pulses at a moderate repetition rate. The backscattering, which is composed mainly of single scattering, is measured with a detector pointing along the laser beam. The multiple scattering, which is mainly double scattering, is measured with a second detector, pointing at a specified angle to the laser beam. The domain of scattering angles that contribute to the doublescattering signal increases monotonically as the pulse penetrates the cloud. The water droplets within the probed volume are assumed to have a constant size distribution. Hence, from the double-scatteringmeasured signal as a function of penetration depth within the cloud, the double-scattering phase function of the scattering volume is derived. Inverting the phase function results in a cloud-droplet-size distribution in the form of a log-normal function.