Flash-lamp-pumped Ho:Tm:Cr:YAG and Ho:Tm:Er:YLF lasers: modeling of a single, long pulse length comparison

Two methods of producing the long pulse lengths that promote efficient extraction of energy from low-gain, quasi-four-level lasers are analyzed. A long pulse length output can mitigate laser-induced damage effects and can be generated in quasi-four-level lasers by two disparate methods. One method utilizes Q-switching techniques in resonators designed to extend the pulse length and another utilizes the first pulse in a relaxation oscillation pulse train. Models for quasi-four-level lasers are derived here taking into account the nonnegligible thermal population of the lower laser level. Closed-form expressions are derived for both modes of operation of quasi-four-level laser systems so the parametric dependencies of both forms of operation become obvious, allowing facile comparison. In addition, a combined absorption and quantum efficiency, germane for flash-lamp pumping, is calculated for both Cr and Er sensitizers. Although the former has the advantage of broad absorption bands, the latter has the advantage of a quantum efficiency approaching 3.     

Flash-lamp-pumped Ho:Tm:Cr:YAG and Ho:Tm:Er:YLF lasers: experimental results of a single, long pulse length comparison

Flash-lamp-pumped, room-temperature Ho:Tm:Cr:YAG and Ho:Tm:Er:YLF are compared for single but long pulse operation, with pulse lengths of approximately 1.0 mus. Under similar operating conditions in normal-mode operation, a slope efficiency of 0.0331 was observed for Ho:Tm:Er:YLF compared with 0.0047 for Ho:Tm:Cr:YAG. For Q-switched operation, Ho:Tm:Er:YLF yielded a slope efficiency of 0.0075. In comparison, a slope efficiency of 0.0012 was obtained for Ho:Tm:Cr:YAG. Two methods of producing long pulse lengths are compared: pulse selection of normal-mode relaxation oscillations and Q-switching in a long resonator. Theoretical models developed in a companion paper for normal-mode relaxation oscillations and Q-switching in quasi-four-level solid-state lasers are in agreement with the experimental results.     

Tm：YAG和Ho：YAG单晶光纤的光谱及Cr~（3＋）的敏化作用

测量了Ｔｍ３＋和Ｈｏ３＋离子的吸收谱以及Ｃｒ３＋离子在ＹＡＧ单晶光纤中的Ｒ荧光线的寿命．用Ｄｅｘｔｅｒ理论讨论了Ｃｒ３＋离子的能量转移效率。结果表明Ｃｒ３＋→Ｔｍ３＋的能量转移效率比Ｃｒ３＋→Ｈｏ３＋的大．     

Modeling of Tm, Ho:YAG and Tm, Ho:YLF 2- mum Lasers and Calculation of Extractable Energies

The development of a model for 2-mum laser operation in Tm, Ho:YAG and YLF crystals pumped in the near infrared is reported. This model, based on a simplified spectroscopic scheme, is fitted to a set of characterization experiments by means of three adjustable parameters. Results show that the excited-state populations are predicted with a relative accuracy of approximately 10% for a large range of pump levels. Using this model, we calculate the extractable energy on short-laser-pulse interactions for the two materials under different operation conditions. We study the sensitivity to pump duration and the optimization of dopant concentrations. We investigate the improvement of the extractable-energy efficiency with multiple-pulse operation. For double-pulse operation the improvement is approximately a factor of 1.5 and leads to overall extractable-energy efficiencies of 16% in YAG and 15% in YLF for an absorbed pump energy of 10 J cm(-3).     

(Cr,Tm,Ho):YAG晶体中Tm~(3+)离子的中介能量转移作用

测定了晶体的吸收谱，荧光谱和荧光寿命，用Taylor和Dexter理论计算了Cr3+－Ho3+,Cr3+－Tm3+和Tm3_－Ho3+离子间能量转移效率和转移几率．讨论了（Cr，Tm．Ho）：YAG晶体中Tm3+的能量转移中介作用．     

Theoretical modeling and design of a Tm, Ho:YLiF4 microchip laser

We present theoretical modeling that makes it possible to compute the output characteristics of a laser-pumped codoped Tm, Ho microchip laser and the experimental results already obtained with a Tm, Ho:YLiF(4) crystal. By taking into account the match of the pump beam to the self-induced eigenmode of the cavity, we find good agreement between theory and experiment when the pump beam size is properly adjusted relative to the absorbed pump power and the crystal characteristics.     

Numerical study of passive Q switching of a Tm:YAG laser with a Ho:YLF solid-state saturable absorber

In a previous work [Appl. Phys. Lett. 65, 3060 (1994)] we experimentally demonstrated that passive Q switching of a 2,017-nm, flashlamp-pumped Tm,Cr:YAG laser with a Ho:YLF saturable absorber could be obtained with an internal focusing lens. We numerically investigate the optical performance of the Ho:YLF Q-switched Tm:YAG laser system by solving the coupled rate equations. The simulation results indicate that the results obtained numerically are in good agreement with those obtained experimentally. With typical laser configuration, a Q-switched laser pulse of 35 mJ in 30 ns is obtained.     

Investigation of Cr:Tm:Er:YAG laser crystals in a resonator with various degrees of spectral selectivity

It has been established that Tm(3+) ions do not prevent multiple-wavelength oscillation in Cr:Tm:Er:YAG laser crystals inserted inside of the completely nonselective mirror resonator. The output mirror spectral selectivity needed for single-wavelength oscillation at 2.697 mum for a considerable excess of pumping energy over the threshold has been determined experimentally. It has been shown that Tm(3+) optimum concentration in the crystals could be determined correctly in the described resonator scheme.     

Diode-pumped efficient laser operation and spectroscopy of Tm,Ho:YVO4

Spectroscopic characterization of co-doped Tm,Ho:YVO₄ crystal grown by the Czochralski method has been performed including absorption spectrum, emitting spectrum and luminescence decay lifetime. The polarization emitting spectrum around 2 μm is accomplished by exciting a singly Ho³⁺ doped YVO₄ crystal to exclude the influence of Tm³⁺³F₄-³H₆ transition and the emission cross section is deduced from both Fuchtbauer-Ladenburg (F-L) equation and reciprocity method (RM). In addition, we report up to 10.4 W continuous wave (CW) output with a conversion efficiency of 40% and 10.3 W Q-Switch output with 12.5 kHz pulse repetition rate of diode-pumped cryogenic Tm,Ho:YVO₄ laser. For Q-Switch operation, the minimum pulse width of 28.2 ns is obtained, all of which demonstrate that the Tm,Ho:YVO₄ is excellent laser material for 2 μm radiation.     

Theoretical and experimental investigations of injection-locked signal extraction of Tm:YAG laser

Injection-seeded is an effective method to obtain high-power pulsed laser with pure spectrum, which is useful to be the laser source of a coherent Doppler LIDAR or a differential absorption LIDAR. In order to achieve the useful injection-locked signal, mode matching between master laser and slave laser is necessary. In this paper, various factors influencing on the extraction of injection-locked signal are analyzed theoretically. Then, experiments on an injection-seeded Tm:YAG laser are carried on, and injection-locked signal is extracted successfully. Moreover, an injection-seeded Tm:YAG laser is achieved, with pulsed single-frequency at 2013 nm, output energy of 3.16 mJ, and pulse width of 238.7 ns, at a repetition rate of 100 Hz.     

Optical properties, fluorescence mechanisms and energy transfer in Tm, Ho and Tm -Ho doped near-infrared laser glasses, sensitized by Yb

The optical properties of the rare elements Tm³⁺, Ho³⁺ and Yb³⁺ were systematically investigated in various glasses. The Tm³⁺ doped aluminozircofluoride glass shows higher quantum efficiency, longer lifetime and stronger fluorescence intensity than Tm³⁺ doped YSGG crystal and other Tm³⁺ doped glasses for the ³H₄ → ³H₆ transition. Similar quantum efficiency, longer lifetime and stronger fluorescence intensity were also found in Ho³⁺ doped aluminozircofluoride glass for the ⁵I₇ → ⁵I₈ transition. The higher quantum efficiencies of Tm³⁺ and Ho³⁺ in aluminozircofluoride glass are due to the longer lifetime and the lower phonon energy. The fluorescence mechanisms and energy transfer in the Yb³⁺ -Tm³⁺ system, Yb³⁺ -Ho³⁺ system and Yb³⁺ - Tm³⁺ -Ho³⁺ system were studied. The very strong fluorescence intensities in the Yb³⁺ -Tm³⁺ system for Tm³⁺ and the Yb³⁺ -Tm³⁺ -Ho³⁺ system for Ho³⁺ which are 1.68 times that of Tm³⁺ doped YSGG crystal and 2.25 times that of Tm³⁺---Ho³⁺ codoped YSGG crystal are attributed to the efficient Yb³⁺ → Tm³⁺, Yb³⁺ → Ho³⁺ and Tm³⁺ → Ho³⁺ energy transfer processes. The fluorescence processes are described by cross relaxations of ²F_5/2 → ³H₅ → ³H₄ → ³H₆ → ²F_7/2 and²F_5/2 → ³H₅ (or ²F_5/2 → ⁵I₆ → ³H₅) → ³H₄ → ⁵I₇ → ⁵I₈ → ³H₆ → ²F_7/2.     

连续Nd:YAG激光器输出功率稳定性研究

本文介绍一种用两套LiNbO3晶体作电光调制器,高稳定硅光电二极管作光反馈控制信号的激光稳功率仪串联使用来稳定Nd:YAG激光器输出功率的方法。对于输出功率为5瓦左右,本身输出功率稳定度为10%/小时的Nd:YAG激光器,其输出光束经稳功率系统后,其稳定度为0.2/小时。     

Performance of diode-end-pumped Cr, Nd:YAG self-Q-switched and Nd:YAG/Cr:YAG diffusion bonded lasers

Self-passively Q-switching of a diode-pumped Cr,Nd:YAG, where the Cr⁴⁺ is used as a saturable absorber for the 1064 nm laser emission is reported. The maximum average output power was obtained using an output coupler of R=86%. The self-Q-switched diode pumped laser yielded 1.86-W average output power with low threshold pumping power (≈1.7-W), average slope efficiency of ≈34%, pulse duration of about 14–16 ns, and modulation frequency ranging from 2.4 to 73 kHz, depending on the input pumping power. These results are the highest reported for self-Q-switched lasers. Higher slope efficiency (42%) and shorter Q-switched pulses were obtained for a Q-switched Nd:YAG/Cr⁴⁺:YAG diffusion bonded laser. A comparison of the codoped Cr,Nd:YAG laser performance, with that of a diffusion bonded laser is reported and analyzed.     

Timing jitter reduction and single-frequency operation in an acousto-optic Q-switched Cr,Nd:YAG laser

A laser-diode-pumped watt-level single-frequency combined actively and passively Q-switched (CAPQ) laser with a wavelength of 1064 nm that simultaneously uses a codoped Cr(4+),Nd(3+):YAG crystal as the gain medium and mode selector is presented. The optimum repetition period of the CAPQ laser is approximately 1.5 times the natural repetition period of the passively Q-switched laser. The averaged timing jitter is approximately 400 ns in the CAPQ laser and the repetition rate of the CAPQ laser is experimentally shown to reach a time instability of 0.2% over 10(6) pulses. The output is a stable single frequency with a linewidth of 400 MHz at 20 W pump power.     

Diode-pumped 214.8-nm Nd:YAG /Cr4+:YAG microchip laser system for the detection of NO

A passively Q-switched 214.8-nm Nd:YAG/Cr(4+):YAG microchip laser system for the detection of NO was designed, constructed, and tested. The system uses the fifth harmonic of the 1.074-microm transition in Nd:YAG to detect NO by laser-induced fluorescence. A significant challenge was the development of an environmentally stable coating to provide the necessary discrimination between the 1.074-microm laser line and the stronger transition at 1.064 microm. The exact position of the fifth-harmonic frequency was determined by use of NO fluorescence excitation spectra to be 46556 +/- 1.5 cm(-1). With a pulse energy of approximately 50 nJ of fifth-harmonic light, we observed a detection sensitivity for NO of approximately 15 parts per billion by volume in a simple, compact optical system.     

Stability analysis of a diode-pumped,thermal birefringence-compensated two-rod Nd:YAG laser with 770-W output power

Using a ray matrix method, we analyze theoretically how the r and theta polarizations affect the resonator stability condition of two laser heads with or without thermal birefringence compensation. The resonator stability condition is analyzed graphically for a plane-parallel and a concave-concave resonator. The maximum range of stable region is found for both the short and the long cavity. The characteristics of the laser output power are confirmed experimentally in association with the resonator stability condition. The laser output power of 776 W is obtained with the optical-to-optical efficiency of 45% for a plane-parallel resonator with a short crystal separation.     

Spectroscopic evaluation of CaYA1O4 doped with trivalent Er, Tm, Yb and Ho for eyesafe laser applications

Spectroscopic properties of relevance for laser applications have been studied for rare earths in CaYA1O₄. Fitting of a theoretical model to observed energy levels yields crystal field parameters and unobserved levels. Structural disorder leads to broad linewidths,but cross sections are larger than in many common hosts. Tm-Tm cross relaxation rates are comparable to those in Tm: YAG, and Yb-Er transfer rates are comparable to those in Yb, Er:phosphate glass. Room temperature Yb-Er upconversion is stronger than in YAG, but modeling shows that neither unconversion nor population of Er⁴I_13/2 is very efficient upon pumping Yb. The host's yellow color intensifies upon annealing in air, a potential problem for visible laser operation. Tm or Ho 2 μm laser operation, or Er 1.5 μ operation upon direct excitation of Er⁴I_13/2, are more promising.     

Comparison of Lasing Performance of Tm, Ho:YLF Lasers by use of Single and Double Cavities

The lasing performance of single-cavity and double-cavity Tm, Ho:YLF lasers was measured experimentally. The maximum, single-longitudinal mode output power for the double-cavity laser was 30 mW, whereas for the single-cavity laser it was 7 mW. We determined the frequency stabilities to be 600 Hz for a single-cavity laser and 300 Hz for a double-cavity laser, by measuring the fluctuation of a self-heterodyne beat signal for a 1.5-micros delay time over a 10-min integrated period. In addition, we obtained a 15-GHz frequency tuning range for the double-cavity laser by changing its cavity length under maximum stable conditions at room temperature.