Real-time inversion of polarization gate frequency-resolved optical gating spectrograms

Frequency-resolved optical gating (FROG) is a technique used to measure the intensity and phase of ultrashort laser pulses through the optical construction of a spectrogram of the pulse. To obtain quantitative information about the pulse from its spectrogram, an iterative two-dimensional phase retrieval algorithm must be used. Current algorithms are quite robust but retrieval of all the pulse information can be slow. Previous real-time FROG trace inversion work focused on second-harmonic-generation FROG, which has an ambiguity in the direction of time, and required digital signal processors (DSPs). We develop a simplified real-time FROG device based on a single-shot geometry that no longer requires DSPs. We use it and apply the principal component generalized projections algorithm to invert polarization gate FROG traces at rates as high as 20 Hz.     

Cross-correlation frequency-resolved optical gating for studying ultrashort-pulse nonlinear dynamics in arbitrary fibers

We describe a cross-correlation frequency-resolved optical-gating system specifically designed for studying nonlinear pulse-propagation dynamics in fibers of arbitrary length at telecommunication wavelengths. The formation of optical solitons and the appearance of temporal phase slips are observed in 100 m of fiber. The wide phase-matching bandwidth and high sensitivity of this system allow us to visualize femtosecond-pulse evolution in a range of linear and nonlinear propagation regimes.     

Measurement for optical arbitrary waveforms using cross-phase modulation cross-correlation frequency-resolved optical gating in a single-mode fibre

A novel scheme of cross-correlation frequency-resolved optical gating (X-FROG) measurement for optical arbitrary waveforms based on the photo-elastic effect and cross-phase modulation (XPM) effect in a single-mode fibre is proposed. In this scheme, a variable delay is generated in the former part of the single-mode fibre by a uniform lateral pressure, and the XPM effect is achieved in the latter part of the fibre. The proposed scheme is very simple and easy to be realized. The amplitude and phase of optical arbitrary waveform to be measured is retrieved from the X-FROG trace using principal component generalized projects algorithm based on matrix. The impacts of the shape of gate pulse, fibre length, relative intensity between gate pulse and optical arbitrary waveform and the complexity of the optical arbitrary waveform on the accuracy of retrieved amplitude and phase are investigated. Simulation results show that, rectangular pulse is a better gate pulse due to lower errors. The accuracy of measurement is improved with the increase in fibre length, and relative intensity between gate pulse and optical arbitrary waveform. Moreover, this scheme also can be used to measure extremely complex optical arbitrary waveforms.     

2R optical regenerator in As2Se3 chalcogenide fiber characterized by a frequency-resolved optical gating analysis

We present a detailed analysis of a 2R optical regenerator based on self-phase modulation in As(2)Se(3) chalcogenide glass fiber using frequency-resolved optical gating (FROG). We obtain good agreement between the FROG measurements and theory, and confirm that the output pulses are near-transform limited. We show that two-photon absorption improves the profile of the power transfer function while not degrading the temporal performance.     

Complete characterization of a self-mode-locked ti:sapphire laser in the vicinity of zero group-delay dispersion by frequency-resolved optical gating

The intensity and the phase of ultrashort pulses from a self-mode-locked Ti:sapphire laser operating in the vicinity of zero group-delay dispersion (GDD) have been completely characterized by the technique of frequency-resolved optical gating (FROG). For small values of negative GDD, the appearance of a dispersive wave in the pulse spectrum is manifested in the measured FROG trace, and pulse retrieval directly shows its association with a broad leading-edge pedestal. For positive GDD, we confirm previous experimental observations of picosecond pulses with large positive chirp and report a new operating regime in which the output pulses are of picosecond duration but are intensity modulated at 20 THz. The physical origin of this modulation is discussed by analogy with similar effects observed during pulse propagation in optical fibers, and the experimental results are compared with a model of intracavity four-wave mixing about the cavity zero GDD wavelength.     

Dispersion-free, multiple-beam interferometer

A two-mirror Fabry-Perot interferometer is described haivng a dependence of transmission T? (ω) on frequency that is very different from the dependence T? (l) on the distance l between the mirrors. This feature is due to resonant dielectric mirrors in which the reflection phase and amplitude depend sharply on ω. The function T? (ω) can have several extrema ?T? /?ω = 0. At these points the interferometer becomes insensitive to a frequency change, whereas the dependence on l remains. Interferometer parameters are defined and some examples are considered. The dispersion-free interferometer can be used for measuring very small mechanical displacements with a light source with poor frequency stability. The applications to gravitational wave detectors and sensitive seismometers can be suggested if the small distance between the mirrors is acceptable.     

High-resolution optical chirped pulse gating

We describe a system for achieving high-resolution range gating using optically chirped pulses. The technique converts signals from the time domain into signals in the frequency domain through a nonlinear, sum-frequency generation process. The technique is based on similar methods used in microwave radar. We draw analogies between our method and conventional and time-lens imaging processes, and present experimental results demonstrating the method.     

Analysis of transient-grating signals for reacting-flow applications

Single-shot transient-grating measurements for thermometry in pressurized reacting flows are examined in the context of rapid digital signal processing. Simple approaches are discussed for temperature determination and rejection of unwanted signals in real-time measurement applications. Examples of temperature data in pressurized postflame gases are presented in the form of probability-density functions (PDFs). Three contributions to the PDF half-widths are discussed. Analysis of phase-matching requirements indicates that beam steering as a result of density fluctuations affects the signal amplitude but not the grating period. Therefore, such stochastic beam deviations have little effect on the derived temperatures. Mode noise on the cw probe beam as well as linear light scattering are found to be insignificant in the frequency range of the observed transient-grating acoustic signature. Use of a single-mode laser for the pump beams is shown to enhance the signal intensity.     

Fluorescence anisotropy by use of optical kerr gating with incoherent laser light

Incoherent fluorescence optical Kerr gating can in principle be used to measure fluorescence anisotropies and determine molecular reorientational times. A novel method for fluorescence anisotropy by use of optical Kerr gating with incoherent laser light is presented. Incoherent optical Kerr signals have been obtained for parallel and perpendicular fluorescence polarization for a 10(-3)-M solution of Rhodamine 6G in ethanol.     

Design and characterization of a femtosecond fluorescence spectrometer based on optical Kerr gating

Design and characterization of a general-purpose spectrometer for recording time-resolved emission spectra of typical fluorescent species is described. The system is based on a high repetition rate amplified Ti : sapphire system, an optical Kerr shutter for gating the emission, and a polychromator plus charge-coupled device (CCD) detection system. Using 1 mm of liquid benzene as the Kerr medium, and optics designed to provide high polarization quality, emission spectra of dilute solutions of solutes with nanosecond lifetimes can be recorded with good signal-to-noise ratios. The current spectrometer uses excitation wavelengths near 390 nm and provides spectra over the wavelength range 400-650 nm with 4 nm resolution and instrument response times of 450 fs (full width at half-maximum, FWHM). Selected applications are described to demonstrate the utility of this instrument.     

Monte Carlo model of the penetration depth for polarization gating spectroscopy: influence of illumination-collection geometry and sample optical properties

Polarization-gating has been widely used to probe superficial tissue structures, but the penetration depth properties of this method have not been completely elucidated. This study employs a polarization-sensitive Monte Carlo method to characterize the penetration depth statistics of polarization-gating. The analysis demonstrates that the penetration depth depends on both the illumination-collection geometry [illumination-collection area (R) and collection angle (θ(c))] and on the optical properties of the sample, which include the scattering coefficient (μ(s)), absorption coefficient (μ(a)), anisotropy factor (g), and the type of the phase function. We develop a mathematical expression relating the average penetration depth to the illumination-collection beam properties and optical properties of the medium. Finally, we quantify the sensitivity of the average penetration depth to changes in optical properties for different geometries of illumination and collection. The penetration depth model derived in this study can be applied to optimizing application-specific fiber-optic probes to target a sampling depth of interest with minimal sensitivity to the optical properties of the sample.     

Calcium-induced voltage gating in single conical nanopores

We examine time signals of ion current through single conically shaped nanopores in the presence of sub-millimolar concentrations of calcium ions. We show that calcium induces voltage-dependent ion current fluctuations in time in addition to the previously reported negative incremental resistance (Nano Lett. 2006, 6, 473-477). These current fluctuations occur on the millisecond time scale at voltages at which the effect of negative incremental resistance was observed. We explain the fluctuations as results of transient binding of calcium ions to carboxyl groups on the pore walls that cause transient changes in electric potential inside a conical nanopore. We support this explanation by recordings of ion current in the presence of manganese ions that bind to carboxyl groups 3 orders of magnitude more tightly than calcium ions. The system of a single conical nanopore with calcium ions is compared to a semiconductor device of a unijunction transistor in electronic circuits. A unijunction transistor also exhibits negative incremental resistance and current instabilities.     

环境响应型智能开关膜的研究进展

综述环境响应型智能开关膜的制备方法和分类,并分别介绍温度响应型、光响应型、电场响应型、pH响应型以及分子识别响应型等智能开关膜的研究现状.     

On carrier-frequency gating systems for static switching circuits

Carrier-frequency gating systems for exciting static electronic switches such as thyristors are examined. The effect of the commutation in the output rectifiers during transmission of the carrier wave is to cause an instantaneous drop in the output voltage during commutation. A compensation for the commutation drop by an overlap technique is proposed, and comparative experimental observations presented on two types of systems.     

Polyelectrolyte multilayer electrostatic gating of graphene field-effect transistors

We apply polyelectrolyte multilayer films by consecutive alternate adsorption of positively charged polyallylamine hydrochloride and negatively charged sodium polystyrene sulfonate to the surface of graphene field effect transistors. Oscillations in the Dirac voltage shift with alternating positive and negative layers clearly demonstrate the electrostatic gating effect in this simple model system. A simple electrostatic model accounts well for the sign and magnitude of the Dirac voltage shift. Using this system, we are able to create p-type or n-type graphene at will. This model serves as the basis for understanding the mechanism of charged polymer sensing using graphene devices, a potentially technologically important application of graphene in areas such as DNA sequencing, biomarker assays for cancer detection, and other protein sensing applications.     

Controlled electrostatic gating of carbon nanotube FET devices

Carbon nanotube transistors are a promising platform for the next generation of nonoptical biosensors. However, the exact nature of the biomolecule interactions with nanotubes in these devices remains unknown, creating one of the major obstacles to their practical use. We assembled alternating layers of oppositely charged polyelectrolytes on the carbon nanotube transistors to mimic gating of these devices by charged molecules. The devices showed reproducible oscillations of the transistor threshold voltage depending on the polarity of the outer polymer layer in the multilayer film. This behavior shows excellent agreement with the predictions of a simple electrostatic model. Finally, we demonstrate that complex interactions of adsorbed species with the device substrate and the surrounding electrolyte can produce significant and sometimes unexpected effects on the device characteristics.     

On-column sample gating for high-speed capillary zone electrophoresis

High-speed zone electrophoresis in a fused-silica capillary is described. Elevated electric fields and short capillary lengths allow a mixture of fluorescein isothiocyanate (FITC) labeled amino acids to be separated in times as short as 1.5 s. Formation of the analyte zone at the head of the capillary is controlled by laser-induced photolysis of a tagging reagent. This gating procedure allows rapid and automated introduction of sample into the capillary. Ultimately, Joule heating of the buffer limits the speed and efficiency of the separation.     

Investigation of ultrafast time gating by spatial filtering

With a spatial-filtering method of gating, we explore image formation through scattering media using first-arriving light. Gating times of a few femtoseconds and less are produced, and the resolution at these extremely short gating times is investigated.