Impurity Scattering Effect on Superfluidity of 3He in Aerogel

The impurity scattering effect on superfluid ³ He in aerogel is studied on the basis of the standard impurity theory within the weak coupling limit. We discuss the superfluid transition temperature and the superfluid density in the dirty Fermi liquid. The results are compared with recent experiments on the superfluidity of ³ He in aerogel. The low pressure data of the observed superfluid density are shown to be in better agreement with the results for the A-phase than for the B-phase. The B-phase results show considerable disagreement with the low pressure data.     

Sound Spectroscopy of the Superfluid Phases of 3He in Aerogel in Zero Magnetic Field

Low-frequency sound is used to study phase transitions of ³He confined in 98% open aerogel. Superfluidity is manifested by the onset of the low frequency (slow) mode whose velocity (as a function of pressure and temperature) was used to map out the phase diagram of the B-phase and the metastable A-phase of ³He in aerogel. Analysis of the slow mode's evolution with temperature allows the development of the superfluid fraction in the A and B phases to be determined. The metastable A-phase and the equilibrium B-phase can co-exist in a properly prepared sample. Both the superfluid transition and the A→B transition exhibit a finite width of ～20–25 µK.     

Absolute Ultrasound Attenuation Measurements in Superfluid 3He in 98% Aerogel by Direct Transmission

Systematic investigations on the effect of static disorder on p-wave superfluid ³He have been made possible by utilizing the unique structure of high porosity silica aerogel. For the past 10 years, a burst of experimental efforts revealed that three distinct superfluid phases exists. We have performed longitudinal ultrasound (9.5 MHz) attenuation measurements in the B-phase of the superfluid ³He in 98% aerogel. The absolute attenuation was determined by direct propagation of sound pulses through the medium in a wide range of temperatures, down to 200 μK, for sample pressures of 10 and 29 bars. Our results provide direct information on the zero-energy density of states of the superfluid phase in aerogel originating from impurity scattering.     

Perturbative Study of Strong Coupling Correction in Superfluid 3He in Aerogel

The AB transition curve of superfluid ³He in aerogel often shows a positive slope dT _AB(P)/dP>0 over the measured pressures P, contrary to that of the bulk liquid. Bearing this behavior in mind suggestive of a unexpectedly strong reduction of the strong coupling (SC) correction due to the aerogel, we examine impurity effects on the SC contributions to the quartic term of the Ginzburg-Landau (GL) functional. Our analysis perturbative both in the repulsive interaction and the impurity scattering suggests that, in agreement with experimental data, the impurity scattering weakens the relative stability of the ABM state to the BW state and notably reduces the SC correction for the ABM phase.     

Sound Experiments on Superfluidity of 3He in Highly Porous Aerogels

We have carried out sound experiments on superfluid ³ He in three highly porous aerogels with different porosities. Two of the acoustic cells contain aerogels inside the pores in roughly sintered silver powder to avoid the vibration of the aerogel. In these acoustic cells we have detected fourth sound, and extracted the superfluid density from the fourth sound velocity. The effect of the sintered silver on superfluid ³ He was examined by using another acoustic cell which contains the sintered silver without aerogel. The size of the pores in the sintered silver was large enough not to show the size effect of superfluid ³ He and small enough to observe fourth sound of ³ He. In another cell without sintered silver, we have observed second-sound-like signal. The superfluid transition temperatures of ³ He are suppressed more in higher density aerogel. The aerogel density dependence of the suppression of the superfluid transition temperature of ³ He in aerogel can be explained qualitatively by the simple s-wave scattering approximation. However, the superfluid density shows quite different pressure-dependence in different porous aerogels. The reason of this phenomenon is not understood yet.     

NMR Study of Superfluid Phases of 3He Confined in 97.5% Porous Silica Aerogel

We have studied the scattering effect from aerogel strands on superfluid phases of ³He by a cw NMR method at 920 kHz. Liquid ³He at a pressure of 13 bar was confined in 97.5% porous aerogel from the same batch as that of a recent 4th sound study. The NMR experiment was performed in a magnetic field of 28.4 mT down to 0.3 mK. As temperature decreased, the NMR resonant frequency increased below 0.76 mK. The temperature of 0.76 mK agrees with the superfluid transition temperature T ^aerogel _c observed in the 4th sound study at the same pressure. Below T ^aerogel _c the behavior of thefrequency shift as a function of temperature indicates that there is no phasetransition to the other superfluid phase down to about 0.4 T ^aerogel _c . Owing to a very large surface solid ³He magnetization, we could not determine the superfluid phase of ³He in the aerogel in the magnetization measurement.     

Impurity Scattering Effect on Superfluid Phases of 3He in 97.5% Porous Silica Aerogel

No Heading NMR studies of superfluid ³He in 97.5% aerogel have been performed in a magnetic field of 28.4 mT. A small-angle neutron scattering experiment on the structure of the aerogel shows that the average separation distance of silica strands is 54 nm. The aerogel strands were covered with a few layers of solid ³He whose magnetization shows Curie-Weiss behaviour. On cooling process A-like phase appeared at suppressed superfluid transition temperature T_C^aero and B-like phase appeared at lower temperatures although only the B-like phase was observed up to T_C^aero on warming process above 2.1 MPa. The superfluid transitions in aerogel always occur below the AB phase transition temperature of bulk liquid at all pressures. An isotropic inhomogeneous scattering model(IISM) proposed by Thuneberg et al. explained well the observed suppressed T_C^aero in 97.5% with the radius 59 nm of voids in this model. This radius is similar with the average strand separation distance of 54 nm measured in the structural analysis. This similarity of two lengths shows the connection of the suppression of T_C^aero with the actual average separation distance of the silica strands.PACS numbers: 67.57.Pq, 67.80.Jd     

Thermodynamic Potential for Superfluid 3He in?Aerogel

We present a free energy functional for superfluid ³He in the presence of homogeneously distributed impurity disorder which extends the Ginzburg-Landau free energy functional to all temperatures. We use the new free energy functional to calculate the thermodynamic potential, entropy, heat capacity and density of states for the B-phase of superfluid ³He in homogeneous, isotropic aerogel.     

Model Calculation of Orientational Effect of Deformed Aerogel on the Order Parameter of Superfluid 3He

Theory of Rainer and Vuorio of small objects in superfluid ³He is applied for calculation of the average orientational effect of a deformed aerogel on the order parameter of ³He. The minimum deformation which stabilizes the ordered state is evaluated both for specular and diffusive scattering of quasiparticles by the strands of aerogel.      

Capture of Superfluid Helium by Porous Structures

We have studied superfluid helium capture in a sample of silica aerogel of 98.2% porosity in the temperature range from 1.22 K up to 1.89 K. The high retention of He in the aerogel sample corresponds to a similar phenomenon in impurity-helium condensates, in which very high values of the ratio of helium atoms to impurity atoms (up to 60) have been seen. We have observed that removing the aerogel sample from superfluid helium in a cylindrical glass beaker caused a decrease of the helium level corresponding to the geometrical volume of the sample (≈1 cm³). This observation has allowed us to conclude that superfluid helium is completely captured by the porous sample. Superfluid helium filling aerogel and impurity-helium samples (porous structures) serves as a dispersive medium of gel-like samples which interacts strongly with impurity nanoclusters forming the dispersing system.      

Magnetic Susceptibility of the Balian–Werthamer Phase of 3He in Aerogel

The equilibrium superfluid phase of ³He impregnated into high-porosity (98%) silica aerogels appears to be a non-equal-spin-pairing state in zero field at all pressures, which is generally assumed to be the Balian–Werthamer (BW) phase modified by the depairing effects of the aerogel structure. The nuclear magnetic susceptibility played a key role in identifying the B-phase of pure ³He with the BW state. We report theoretical calculations of the nuclear magnetic susceptibility for the BW model of superfluid ³He in aerogel within the framework of the Fermi-liquid theory of superfluid ³He. Scattering of quasiparticles by the aerogel, in addition to Fermi-liquid exchange corrections, leads to substantial changes in the susceptibility of the BW phase. The increase in the magnetic susceptibility of ³He-aerogel compared to pure³He-B is related to the polarizability of the gapless excitations and the impurity-induced local field. The limited data that is available is in rough agreement with theoretical predictions. Future measurements could prove important for a more definitive identification of the ordered phase, as well as for refining the theoretical model for the effects of disorder and scattering on the properties of superfluid ³He.     

Superfluid helium three in aerogel

We report measurements of the superfluid density and transition temperature of³He confined within 98.2% open aerogel. Both the superfluid fraction and the temperature at which the superfluid is manifested are suppressed strongly from their bulk values. The results suggest that the aerogel reduces the order parameter by a mechanism other than as a diffusely scattering surface.     

Packed Powder as Superleak for Spin Pump Experiments in Superfluid 3He A1

Experimental exploration of highly spin-polarized states of liquid ³He by applying external magnetic field is limited by the availability of static magnetic field. In the “ferromagnetic” superfluid A₁ phase of liquid ³He there is an alternate method for boosting spin-polarization by the process of spin pumping without requiring such high magnetic field. The spin pumping in the A₁ phase takes advantage of a superleak (SL) acting simultaneously as a filter for both entropy and spin. The spin pump technique that uses the SL-spin filter and a mechanical actuator enables us to directly boost polarization of ³He. The amount of enhancement of spin polarization has been limited so far. We are now developing a new type of SL filter made of packed aluminum oxide powder (referred as PAP-SL), in order to achieve greater enhancement of spin polarization. Several kinds of the PAP-SL filter were constructed by pressing aluminum oxide powders into a cylinder holder. The packed structures were carefully characterized by a flow-rate-measurement, X-ray tomography, and mercury intrusion porosimetry. The preliminary result shows that the PAP-SL works as SL filter for the superfluid ³He.     

Negative Ion Mobility in Superfluid 3He Under High Magnetic Field

The negative ion mobility has been measured in superfluid ³He at pressures above 20 bar under high magnetic field up to 14 Tesla. It does not depend on the temperature in the normal phase, followed by a rapid increase below the superfluid transition in both A ₁ and A ₂ phase. The isothermal mobility is found to be independent of the magnetic field in the normal and A ₂ phase, while it decreases with increasing magnetic field in the A ₁ phase. This field dependence is explained by taking account of the field dependence of the transition temperature (T _{A 1}) between the normal and the A ₁ phase. Therefore the scattering cross section between, the negative ion and the ³He quasiparticles has no magnetic field dependence both in the superfluid and the normal phase.     

A Preliminary Heat Capacity Measurement of 3He in Aerogel near its Superfluid Transition

We report simultaneous heat capacity and torsional oscillator measurement of ³ He in aerogel near the superfluid transition. The heat capacity has a peak at the temperature T_c where the torsional oscillator shows the onset of superfluid decoupling. The coincidence of these signatures suggests that ³ He in aerogel does undergo a true thermodynamic transition.     

Novel Oscillating Aerogel Experiments in Superfluid 3He at Ultralow Temperatures

We present novel experiments on a disk of 98% aerogel oscillating in superfluid ³ He at ultralow temperatures. The aerogel dik is attached to a goal post shaped vibrating wire resonator and immersed in liquid ³ He cooled by a Lancaster style nuclear cooling stage. At low pressures we see no evidence for superfluidity within the aerogel down to our base temperature of below <0.11T_c. At higher pressures we observe large temperature dependent frequency shifts, reminiscent of torsional oscillator experiments. We find the transition temperature at 5 bar to be around 600K. The response of the resonator is highly non linear when the helium in the aerogel is superfluid. The resonant frequency decreases strongly with increasing wire amplitude. This offers an exciting new technique for measuring the superfluid properties of ³ He in aerogel in the ultralow temperature regime.     

Recent Spin Pump Experiments on Superfluid 3He–A1

The superfluid ³He A₁ phase, containing a spin-polarized condensate allows us to explore the dynamics of superfluid spin current. In the mechano-spin effect (MSE), a mechanically applied pressure gradient and a superleak-spin filter enable one to directly boost spin polarization of ³He in a small chamber. We are developing new apparatus for achieving greater enhancement of spin density. A development of a new-type ³He-hydraulic actuator has been already reported. We present here the construction of new-type of superleak-spin-filter made of packed powder aluminum oxide (referred as PAP-SL). The PAP-SL is popular in the study of superfluid ⁴He, but has not been established for that of the superfluid ³He. The attempt to construct the PAP-SL for the spin pump experiment was made by using aluminum oxide powder with nominal 1 μm powder diameter and with packing fraction of 40 %. Before executing the experiment, the nuclear demagnetization cryostat of ISSP, Univ. Tokyo which has been used for this experimental activity, was heavily damaged by the 2011 Great East Japan (Higashi Nihon) Earthquake. The repair work and earthquake damage protection strengthening has just been accomplished.     

Possible Existence of Dense Superfluid 3He-4He Mixture in Aerogel

While studying superfluid ³He of 2.4 MPa in 97.5 %-porosity aerogel with NMR/MRI techniques, we find that the T _C is reduced when more than adequate amount of ⁴He, which covers the surface of silica strands, is introduced. For a sample, whose T _C is reduced to as low as 0.9 mK, we find that the spin diffusion coefficient in the normal phase is increased by a factor of 1.56 both in high temperature region, where ³He-³He scattering dominates, and in low temperature region, where ³He-aerogel scattering dominates. This enhancement is attributed to a modification of Landau parameter $F_{0}^{a}$ from ?0.757 to ?0.62, which is a change towards less ferromagnetic direction. The modification of microscopic quantity could be explained if small amount of ⁴He has homogeneously mixed into liquid ³He in the aerogel.     

Effect of Strong Magnetic Fields on Superfluid 3He in 98% Porosity Aerogel

No Heading We report our results of shear acoustic impedance measurements performed on superfluid ³He in 98% porosity silica aerogel. Experiments in high porosity aerogel provide unique opportunity to study the influence of disorder on a p-wave superfluid and compare the behavior with that of the well understood pure bulk. Our experiment is designed to detect acoustic signatures from both bulk liquid and liquid in aerogel. In the past, experiments on ³He in aerogel have been conducted in zero or low magnetic fields (< 1 tesla). We made measurements in magnetic fields as high as 15 tesla at 28.4 and 33.5 bars and observed a new phase in aerogel induced by magnetic fields splitting the superfluid transition into two.PACS numbers: 67.57Pq, 67.80Mg     

Robust Superfluid Phases of 3He in Aerogel

Within a phenomenological approach possible forms of the order parameter of the superfluid phases of ³He in the vicinity of the transition temperature are discussed. The effect of aerogel is described by a random tensor field interacting with the orbital part of the order parameter. With respect to their interaction with the random tensor field a group of “robust” order parameters which can maintain long-range order in the presence of the random field is specified. Robust order parameters, corresponding to Equal Spin Pairing (ESP) states are found and proposed as candidates for the observed A-like superfluid phase of liquid ³He in aerogel.