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A process of simultaneous desulfurization and denitrification of flue gas was conducted in this study. The flue gas containing 200 mg·m−3 NO, 1000–4000 mg·m−3 SO2, 3%–9% O2, and 10%–20% CO2 was first oxidized by O3 and then absorbed by ammonia in a bubbling reactor. Increasing the ammonia concentration or the SO2 content in flue gas can promote the absorption of NOX and extend the effective absorption time. On the contrary, both increasing the absorbent temperature or the O2 content shorten the effective absorption time of NOX. The change of solution pH had substantial influence on NOX absorption. In the presence of CO2, the NOX removal efficiency reached 89.2% when the absorbent temperature was raised to 60 °C, and the effective absorption time can be maintained for 8 h, which attribute to the buffering effect in the absorbent. Besides, both the addition of Na2S2O3 and urea can promote the NOX removal efficiency when the absorbent temperature is 25 °C, and the addition of Na2S2O3 had achieved better results. The advantage of adding Na2S2O3 became less evident at higher absorbent temperature and coexistence of CO2. In all experiments, SO2 removal efficiency was always above 99%, and it was basically not affected by the above factors. 相似文献
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Experiments on simultaneous absorption of SO_2 and NO_X from sintering flue gas via a composite absorbent NaClO_2/NaClO were carried out. The effects of various operating parameters such as NaClO_2 concentration(ms), NaClO concentration(mp), molar ratio of NaClO_2/NaClO(M), solution temperature(TR), initial solution pH, gas flow(Vg) and inlet concentration of SO_2(CS) and NO(CN) on the removal efficiencies of SO_2 and NO were discussed. The optimal experimental conditions were determined to be initial solution pH = 6, TR=55 °C and M = 1.3 under which the average efficiencies of desulfurization and denitrification could reach99.7% and 90.8%, respectively. Moreover, according to the analysis of reaction products, it was found that adding NaClO to NaClO_2 aqueous solution is favorable for the generation of ClO_2 and Cl_2 which have significant effect on desulfurization and denitrification. Finally, engineering experiments were performed and obtained good results demonstrating that this method is practicable and promising. 相似文献
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A composite-liquid absorbent (CLA), NaClO/KMnO4, for simultaneous desulfurization and denitrification (SDD) was studied in a homemade bubbling reactor. The experimental results showed that the CLA configured by sodium hypochlorite (NaClO) and potassium permanganate (KMnO4) had a very good synergistic effect on SDD. The effects of NaClO concentration (CNa), KMnO4 concentration (CK), gas space velocity (Vg), initial pH value, and temperature of the absorption liquid (Ts) on efficiencies of the SDD were investigated. Under the optimal reaction conditions, the best removal efficiencies were 100% for sulfur dioxide (SO2) and above 94% for nitric oxide (NO). The ion chromatography and titration were used to analyze the changes of both the ion species and concentrations in the liquid before and after the reaction. According to the experiment results and related literature, the reaction mechanism of the SDD based on the CLA was proposed. 相似文献
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发电锅炉烟气排放基本都需要脱硫脱硝,现在多采用钙基化合物与SO2生成石膏处理烟气,但该工艺不能充分利用产物和同时脱硫脱硝,脱硝采用SCR工艺。研究了炭基材料、金属氧化物和稀土元素作为催化剂在脱硫脱硝中的应用。 相似文献
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介绍一种流光放电烟气脱硫湿法工艺流程,其特征是:(1)采用交直流叠加(AC/DC)方式在工业型反应器发生分布良好的流光放电等离子体;(2)取代传统等离子体干法技术,采用分区湿式反应器系统,大幅降低能耗,无产物粘壁;(3)采用可规模化的流光放电等离子体氧化技术,实现高浓度亚硫酸铵氧化;(4)控制尾气氨逸出;(5)生成液浓缩脱水结晶干燥制得固体硫酸铵。通过半工业试验,在SO2初始浓度500~1000 μl·L-1 条件下,脱硫率≥95%,亚硫酸盐一次氧化率50%~70%,适当处理后达到90%以上,反应器能耗小于3. 5 W·h·m-3,氨逸出在5 μl·L-1以下,副产回收适合农用的铵肥。在吸收液盐浓度3 mol·L-1下还可以获得有实用价值的反应速度,显示出良好的工业应用前景。 相似文献
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燃煤烟气脱硫脱硝一体化技术研究进展 总被引:1,自引:0,他引:1
燃煤烟气是二氧化硫和氮氧化物的最主要来源,对生态环境影响极大。开发技术简单,投资少,运行成本低,具有良好运行性能的脱硫脱硝一体化技术已成为各国控制烟气污染的研发热点。文章重点介绍已成熟或尚在研究的各种固相吸附/再生脱硫脱硝法、气/固催化脱硫脱硝法、液相脱硫脱硝法和高能电子活化氧化法等一体化技术及其最新进展,分析了相关技术原理、优缺点及应用前景。立足于中国基本国情,分析了大力发展和推广燃煤烟气脱硫脱硝一体化技术的必要性和紧迫性。 相似文献
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将氨法脱硫废液用于烟气脱硫系统进行工业化试验.结果表明,新工艺可以增加电厂脱硫溢流液的碱性,提高烟气中SO2的脱除效率,取得较好的应用效果,并且为焦化厂氨法脱硫废液的处理提供了新的途径. 相似文献
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氨法烟气脱硫技术综述 总被引:1,自引:0,他引:1
我国大气污染物的主要来源是以烟尘和SO2为主的烟气。由于氨法烟气脱硫技术是将SO2转化为硫酸铵肥料,该技术得到了越来越广泛的应用。简述了氨法烟气脱硫的技术特点、基本原理,通过与其他常用技术的比较说明了氨法脱硫的技术优势。同时分析了氨法脱硫存在的氨逃逸、亚硫酸铵氧化以及材质腐蚀3个问题,同时提出了相应建议。 相似文献
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《化学工业与工程技术》2017,(2):75-79
采用一定浓度氨水为脱硫剂的氨法湿式烟气脱硫技术,是控制锅炉尾气排放中SO_2浓度的有效方法。介绍了氨法脱硫处理锅炉尾气的原理、工艺改造流程、主要设备及副产品等,简述了工艺改造后烟气脱硫系统、硫酸铵结晶脱水系统及工艺水系统的运行及能耗情况。结果表明:氨法脱硫技术具有反应速度快、脱硫效率高、副产品价值高等一系列优点;脱硫后锅炉装置尾气排放的SO_2和烟尘浓度均达到国家环保标准,系统SO_2脱除率达到95%,烟尘脱除率达到90%;每年还可副产硫酸铵约8 320 t;具有较好的环境效益、经济效益和社会效益。 相似文献
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介绍了我国烟气脱硫技术现状,对氨法烟气脱硫技术进行了分析。提出氨法脱硫技术更符合循环经济的思想,比较适合有氨来源的化肥企业应用,应在化肥企业大力推广。 相似文献
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利用聚丙烯中空纤维双层曝气式膜接触器,对膜曝气-膜吸收耦合式海水烟气脱硫过程开展实验研究,考察了烟气流量、海水流量、海水pH以及曝气量等因素对烟气脱硫参数的影响。结果表明,曝气式膜吸收过程具有更高的脱硫效率和传质性能,相较于非曝气过程,SO2吸收率可提高12.4%。提高烟气流量,使SO2吸收率降低,总传质系数先增大再减小;提高吸收剂流量、pH和曝气量,SO2吸收率和总传质系数均会提高,海水pH较高条件下加入曝气更能有效加强吸收效果;烟气中SO2的吸收通量均随海水pH和曝气量的增加而增加。扫描电镜及接触角测量显示在使用一个月后的膜丝仍具有较高的疏水性能和使用性能。 相似文献