共查询到20条相似文献,搜索用时 15 毫秒
1.
S. Akcöltekin E. Akcöltekin H. Lebius 《Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms》2009,267(4):683-686
We have investigated morphological changes of freshly cleaved CaF2(1 1 1) single crystal surfaces before and after ion irradiation. We show that with or without irradiation the surface undergoes serious changes within minutes after the cleavage if the samples are exposed to ambient conditions. This is most likely due to the adsorption of water and could be avoided only if working under clean ultra-high-vacuum conditions. Ion-induced modifications on this surface seem to act as centers for an increased rate of adsorption so that any quantitative numbers obtained by atomic force microscopy in such experiments have to be treated with caution. 相似文献
2.
Yudi Rosandi Thomas Michely 《Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms》2009,267(16):2769-2773
Using molecular-dynamics simulation, we study the sputtering of a Pt(1 1 1) surface under oblique and glancing incidence 5 keV Ar ions. For incidence angles larger than a critical angle ?c, the projectile is reflected off the surface and the sputter yield is zero. We discuss the azimuth dependence of the critical angle ?c with the help of the surface corrugation felt by the impinging ion. If a step exists on the surface, sputtering occurs also for glancing incidence ?>?c. We demonstrate that for realistic step densities, the total sputtering of a stepped surface may be sizable even at glancing incidence. 相似文献
3.
Tousif Hussain I.A. Khan Nida Khalid Shahzad Naseem 《Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms》2009,267(5):768-772
Titanium nitride thin films were deposited on Si(1 0 0) substrates by using a low energy (2.3 KJ) Mather-type plasma focus device. The composition of the deposited films was characterized by X-ray diffraction (XRD). The crystallite size has strong dependence on the numbers of focus shots. The crystallinity of TiN thin films is found to increase with increasing the number of focus shots. The effect of different number of focus shots on micro structural changes of thin films was characterized by Scanning Electron Microscope (SEM) and Atomic Force Microscope (AFM). SEM results showed net-like structure for film deposited for 15 numbers of shots, which are elongated grains of Si3N4 in amorphous form embedded into TiN crystals. The average surface roughness was calculated from AFM images of the thin films. These results indicated that the average surface roughness increased for films deposited with increased number of focus shots. The least crystallite size and roughness are observed for film deposited with 25 focus shots. 相似文献
4.
W.S. Lai J.J. Yu D.J. Bacon 《Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms》2009,267(18):3076-3079
The present study is relevant to the preferential Al sputtering and/or enhancement of the Ni/Al ratio in Ni3Al observed by the scanning transmission electron microscopy fitted with a field emission gun (FEG STEM). Atomic recoil events at the low index (1 0 0), (1 1 0) and (1 1 1) surfaces of Ni3Al through elastic collisions between electrons and atoms are simulated using molecular dynamics (MD) methods. The threshold energy for sputtering, Esp, and adatom creation, Ead, are determined as a function of recoil direction. Based on the MD determined Esp, the sputtering cross-sections for Ni and Al atoms in these surfaces are calculated with the previous proposed model. It is found that the sputtering cross-section for Al atoms is about 7-8 times higher than that for Ni, indicating the preferential sputtering of Al in Ni3Al, in good agreement with experiments. It is also found that the sputtering cross-sections for Ni atoms are almost the same in these three surfaces, suggesting that they are independent of surface orientation. Thus, the sputtering process is almost independent of the surface orientation in Ni3Al, as it is controlled by the sputtering of Ni atoms with a lower sputtering rate. 相似文献
5.
Jun Wang Wei Yang 《Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms》2008,266(16):3583-3587
The effects of short duration irradiation with low dose rate gamma and beta rays on the input resistance and the output Hall voltage of InSb, GaAs, Si, and Ge semiconductor Hall effect devices were systemically studied. Both gamma and beta irradiation can cause the input resistance of Hall effect devices to increase linearly with increasing irradiation time, in the absence of a magnetic field. When the devices were placed in a magnetic field, the output Hall voltage and input resistance increased nonlinearly with increasing gamma irradiation time. The effects of both gamma and beta irradiation persisted long after the irradiation itself, and without annealing. The effects from irradiation in Hall effect devices can be mainly ascribed to the degradation of the charge carriers’ transport properties caused by radiation-induced defects. The radiation resistance of the Hall effect devices was estimated by considering changes of the input resistance under the same irradiation conditions. The Ge and Si Hall effect devices demonstrated a better radiation resistance than the InSb and GaAs Hall effect devices due to their large displacement threshold energy. 相似文献
6.
K. Ohhara N. Ishikawa S. Sakai O. Michikami 《Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms》2009,267(6):973-975
CeO2 films were irradiated with 200 MeV Au ions in order to investigate the damages created by electronic energy deposition. In the Raman spectra of the ion-irradiated films, a broad band appears at the higher frequency side of the F2g peak of CeO2. The band intensity increases as ion fluence increases. Furthermore, the F2g peak becomes asymmetric with a low-frequency tail. In order to understand the origin of these spectral changes, an unirradiated CeO2 film was annealed in vacuum at 1000 °C. By comparing the results for the irradiation and for the annealing, it is concluded that the broad band obtained for irradiated samples contains the peak observed for the annealed sample. The F2g peak becomes asymmetric with a low-frequency tail by the irradiation as well as the annealing. Therefore, the above-mentioned changes in the Raman spectra caused by 200 MeV Au irradiation is closely related to the creation of oxygen vacancies. 相似文献
7.
I. Strašík E. Mustafin R. Hinca D. Schardt A. Golubev B. Sharkov G. Fehrenbacher H. Iwase G. Mustafina 《Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms》2008,266(15):3443-3452
As a preparatory work for constructing the FAIR facility at GSI, samples of stainless steel and copper were irradiated by 950 MeV/u 238U ions and depth-profiles of residual activity were measured by gamma-ray spectroscopy. The isotopes with dominating contribution to the residual activity were identified and their contributions were quantified. In contrast to the previous study performed at lower energies, the activities could no longer be determined from the full-assembly target measurements. Depth-profiling of residual activity of all identified isotopes had to be completed by measurements of individual target foils. The activity contributions were then obtained by integration of the depth-profiles. 相似文献
8.
Wataru Takeuchi 《Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms》2009,267(11):1952-1959
The clean Cu(1 0 0) surface and Pt/Cu(1 0 0) surface by Pt deposition at room temperature have been investigated using the computer simulation of coaxial impact-collision ion scattering spectroscopy (CAICISS). The computer simulations employing the ACOCT program code, which treats the atomic collisions three-dimensionally and is based on the binary collision approximation (BCA), were carried out for the case of 3 keV He+ ions incident along the 〈1 0 0〉 and 〈1 1 0〉 azimuths of the clean Cu(1 0 0) and Pt/Cu(1 0 0) surfaces. The comparisons between ACOCT results and experimental CAICISS data show that the experimental results on the clean Cu(1 0 0) surface are relatively well reproduced by the ACOCT simulations including the inward relaxation of 1.2% in the first interlayer spacing and the outward relaxation of 1.6% in the second interlayer spacing, and that the ACOCT simulations for the Pt deposition with coverages of 2.35 ML and 2.75 ML on the Cu(1 0 0) surface appear the concentrations of 0.24 ML of Pt sitting 2.3 Å and 0.25 ML of Pt sitting 2.5 Å above the outermost atomic layer, respectively. 相似文献
9.
J. Ghatak K.G.M. Nair 《Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms》2008,266(8):1282-1286
Thin films of Ag (1.5 nm thick) are grown on Si (1 1 1) substrates using evaporation method in high vacuum condition and due to non-wetting nature of silver, isolated islands of mean size ≈12.0 nm have been formed on the surface. Au2+ (1.5 MeV) ions have been used to irradiate the above systems at various fluences (5 × 1013-1 × 1015 cm−2) at an impact angle of 5° and at a flux of 6.3 × 1012 cm−2 s−1 (corresponding to a beam current density of 2.0 μA cm−2 for Au2+ ions). Ion beam induced embedding is observed to begin at a fluence of 1 × 1014 cm−2 for this high flux whereas low flux irradiations (current density ≈ 0.02 μA cm−2) of Au2+ ions under similar irradiation conditions did not yield embedding (impact angle 5°). High resolution transmission electron microscopy measurement showed no mixing in the form of silicide formation. These results are compared with high flux modifications in Au/Si system. 相似文献
10.
F. Gou Qiu Qian J.Y. Tang 《Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms》2007,265(2):479-484
In this study, Molecular dynamics simulations were performed to investigate F continuously bombarding silicon surfaces at normal incidence and room temperature. The simulated results show that with increasing incident energy and temperature, the etch yield of Si atoms increases, which is in good qualitative agreement with experiments. Accompanying reaching the steady-state F uptake and Si etching, a steady-state SiFx (x = 1-4) reactive layer is formed whose thickness increases with increasing incident energy. In the reaction layer, SiF species are dominant and SiF3 species decrease with increasing incident energy. 相似文献
11.
J.H. Liang S.C. Wang 《Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms》2008,266(24):5116-5119
In this study, n-type <1 0 0> silicon specimens were liquid nitrogen temperature (LT) and room temperature (RT) implanted with 2 × 1015 cm−2 77 keV BSi molecular ions to produce shallow junctions. Post-annealing methods under investigation included furnace annealing (FA) at 550 °C for 0.5, 1, 2, 3 and 5 h and rapid thermal annealing (RTA) at 1050 °C for 25 s. Post-annealing effects on the shallow-junction characteristics were examined using one-step (FA) and two-step (FA + RTA) post-annealing treatments. Secondary ion mass spectrometry (SIMS), cross-sectional transmission electron microscopy (XTEM), a four-point probe and Raman scattering spectroscopy (RSS) were employed to analyze junction depths (xj), damage microstructures, sheet resistance (Rs) and damage characteristics, respectively. The results revealed that the shallow-junction characteristics of the LT implant are better than those of the RT one when post-annealing time in FA exceeds 1 h. A post-annealing time of 3 h in FA is needed in order to obtain the optimal one- or two-step post-annealing effects on the shallow-junction characteristics in both the LT and RT implants. 相似文献
12.
Wang Rong Liu Yunhong 《Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms》2008,266(5):745-749
GaInP/GaAs/Ge triple-junction solar cells were irradiated with 0.28, 0.62 and 2.80 MeV protons with fluences ranging from 1 × 1010 cm−2 to 1 × 1013 cm−2. Their performance degradation is analyzed using current-voltage characteristics and spectral response measurements. The degradation rates of the short circuit current, open circuit voltage, and maximum power output increase with fluence, but decrease with increasing proton energy. It was also observed that the spectral response of the GaAs middle cell degrades more significantly than that of the GaInP top cell. 相似文献
13.
J.A. Valdez I.O. Usov J. Won M. Tang R.M. Dickerson G.D. Jarvinen K.E. Sickafus 《Journal of Nuclear Materials》2009,393(1):126-220
Room temperature ion irradiation damage studies were performed on a ceramic composite intended to emulate a dispersion nuclear fuel. The composite is composed of 90-mole% MgO and 10-mole% HfO2. The as-synthesized composite was found to consist of Mg2Hf5O12 (and some residual HfO2) particles embedded in an MgO matrix. X-ray diffraction revealed that nearly all of the initial HfO2 reacted with some MgO to form Mg2Hf5O12. Ion irradiations were performed using 10 MeV Au3+ ions at room temperature over a fluence range of 5 × 1016-5 × 1020 Au/m2. Irradiated samples were characterized using both grazing incidence X-ray diffraction (GIXRD) and transmission electron microscopy (TEM), the latter using both selected-area electron diffraction (SAED) and micro-diffraction (μD) on samples prepared in cross-sectional geometry. Both GIXRD and TEM electron diffraction measurements on a specimen irradiated to a fluence of 5 × 1020 Au/cm2, revealed that the initial rhombohedral Mg2Hf5O12 phase was transformed into a cubic-Mg2Hf5O12 phase. Finally, it is important to note that at the highest ion fluence used in this investigation (5 × 1020 Au/m2), both the MgO matrix and the Mg2Hf5O12 second phase remained crystalline. 相似文献
14.
Yasuhiro Sakuma Masahiko KatoShinya Yagi Kazuo Soda 《Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms》2011,269(3):257-262
We have measured the energy distributions of the secondary ions sputtered from the Si(1 1 1) and Ge(1 1 1) surfaces and investigated the ionization probabilities of sputtered Si+ and Ge+ ions for clarifying their ionization mechanisms. The observed ionization probabilities depend on the velocity of Si+ and Ge+ ions. This velocity dependence can be successfully analyzed by a theoretical expression, which was proposed originally for the metal surfaces. This implies that the ionization mechanism of Si+ and Ge+ ions is the same as ions sputtered from the metal surface, i.e., the resonant electron transfer in the high velocity regime and the thermal excitation process in the low velocity regime. The difference in the ionization probability between Si+ and Ge+ ions is well explained by the difference in the band gap energy. 相似文献
15.
G. Anandha babu N. Vijayan K. Asokan 《Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms》2008,266(23):5032-5036
4,4′-Dimethylbenzophenone (DMBP) single crystals were irradiated at room temperature and at liquid nitrogen temperature with 50 MeV Li3+ ions at fluences 1 × 1012 and 1 × 1013 ions/cm2. The dielectric constant and dielectric loss as a function of frequency of the applied ac field in the range from 20 Hz to 1 MHz and at temperatures ranging from 313 to 353 K were analyzed. The dielectric constant decreases with increase in frequency for all the temperatures. The dielectric constant and dielectric loss increase with fluence. Optical absorption was measured at different conditions. UV-Vis studies reveal the decrease in bandgap. The unirradiated as well as irradiated crystals were characterized by photoluminescence. Ion-induced changes were also studied with respect to their mechanical response using the Vicker’s microhardness technique and parameters including fracture toughness, brittleness index and yield strength are calculated. 相似文献
16.
M.S. Gravielle J.E. Miraglia 《Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms》2009,267(4):610-614
This work deals with the interference effects recently observed in grazing collisions of few-keV atoms with insulator surfaces. The process is studied within a distorted-wave method, the surface eikonal approximation, based on the use of the eikonal wave function and involving axial channeled trajectories with different initial conditions. The theory is applied to helium atoms impinging on a LiF(0 0 1) surface along the 〈1 1 0〉 direction. The role played by the projectile polarization and the surface rumpling is investigated. We found that when both effects are included, the proposed eikonal approach provides angular projectile spectra in good agreement with the experimental findings. 相似文献
17.
Y. Xin X. Ju T.D. Ma Q.Y. Huang 《Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms》2009,267(18):3166-3169
China Low Activation Martensitic (CLAM) steel was irradiated at room temperature with different doses of He+ and H+ ion beams. TEM indicated that the microstructure of unirradiated CLAM steel consisted of laths, grain boundaries, dislocations and carbides. Electron diffraction patterns revealed that the microstructure of carbides at grain boundaries was primarily dominated by M23C6 carbide. Vacancy clusters were induced into the matrix after irradiation. TEM-EDX of carbides and matrices of unirradiated and post-irradiated samples were performed to investigate the composition of carbides and the effect of irradiation on the composition of carbides. Carbides from unirradiated and irradiated specimens at grain boundaries were found to be enriched with Cr. For irradiated specimens, concentrations of Cr increased as the irradiation dose was increased. Cr enrichment could lead to precipitation of additional phase. 相似文献
18.
M.A. Tagliente M. Massaro 《Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms》2008,266(7):1055-1061
We present an experimental and theoretical study on the structural properties of ZnO nanoparticles embedded in silica. The ZnO-SiO2 nanocomposite was prepared by ion implanting a Zn+ beam in a silica slide and by annealing in oxidizing atmosphere at 800 °C. From an experimental point of view, the structural properties of the ZnO-SiO2 nanocomposite were studied by using glancing incidence X-ray diffraction. According to the results, zinc crystalline nanoclusters with an average diameter of 13 nm are in the as-implanted sample. The annealing in oxidizing atmosphere promotes the total oxidation of the Zn nanoclusters and increases their size until to an average of 22 nm. Moreover, the formed ZnO nanocrystals have a preferential (0 0 2) crystallographic orientation. From a theoretical point of view, the preferential orientation of the ZnO nanoparticles can be explained satisfactory by the minimization of the strain energy of the nanoparticles placed in proximity of the surface of the matrix. 相似文献
19.
N. Matsunami S. Venkatachalam H. Kakiuchida 《Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms》2008,266(8):1522-1526
Aluminum nitride (AlN) thin films have been deposited on Si(1 1 1) substrates by using reactive-rf-magnetron-sputtering at 250 °C. The crystalline quality and orientation of the films have been studied by X-ray diffraction (XRD). We have observed that the films grow with c- or a-axis orientation. The composition, film thickness, impurities and stress are considered to be factors affecting the orientation and have been analyzed by Rutherford backscattering spectroscopy (RBS), nuclear reaction analysis (NRA) and XRD. Their effects on the film growth will be discussed. Surface morphology of the films will be also presented. 相似文献
20.
C. Mansilla P. PhilippT. Wirtz 《Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms》2011,269(9):905-908
Nowadays, the use of low energy ion bombardment in secondary ion mass spectrometry (SIMS) is a mandatory step to obtain high depth resolution for the characterization of ultra shallow junctions. However, increment of roughness during ion bombardment leads to the degradation of depth resolution. The evolution of surface roughening and ripple formation on silicon at ambient temperature under 1 keV Cs+ ion bombardment with and without sample rotation has been studied by means of atomic force microscopy.Ripple formation with a perpendicular orientation with respect to the Cs+ beam direction has been detected, and their wavelength and correlation length have been monitored as a function of the experimental conditions. Roughness and wavelength increased with increasing ion fluence, while variations of ion flux showed little effect. The effect of sample rotation during ion bombardment led to a critical reduction of the surface roughness and disappearance of ripples. 相似文献